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Physical Review A

Laser cooling of trapped ions with polarization gradients

J. I. Cirac, R. Blatt, A. S. Parkins, P. Zoller

Published Aug 1, 1993• 20 citations
Publisher

Abstract

Laser cooling of a single trapped ion with Zeeman substructure below the Doppler limit is considered theoretically. The laser field consists of two counterpropagating beams linearly polarized in different directions, and the internal atomic transition is ${\mathit{J}}_{\mathit{g}}$=1/2\ensuremath{\rightarrow}${\mathit{J}}_{\mathit{e}}$=3/2. The ion is assumed to be localized to spatial dimensions smaller than the optical wavelength (Lamb-Dicke limit) and placed at a specific position with respect to the laser beams. Under the assumption that the rate for optical pumping between the atomic ground states defines the smallest time constant in the system, analytic expressions for the final energy and the cooling rates are derived, with both a semiclassical and a full quantum treatment. The results show that laser cooling of a trapped ion using polarization gradients leads to very low energies. These energies are insensitive to the precise localization of the ion with respect to the lasers, the angle between the direction of the polarizations of the laser beams, and the detuning of the cooling laser.

DOI
10.1103/physreva.48.1434

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Abstract We implement three-dimensional polarization gradient cooling (PGC) of trapped ions. Counter-propagating laser beams near 393 nm impinge in lin ⊥ lin configuration, at a frequency below the S 1/2 to P 3/2 resonance in 40 Ca + . Our measurements demonstrate that cooling with laser beams detuned to lower frequencies from the resonance is robust against an elevated phonon occupation number and works continuously in the crossover from regular Doppler cooling to detunings of tens of linewidths. It is thus robust against heating events and also works well for an initial ion motion far out of the Lamb–Dicke regime. We show that PGC performance strongly depends on residual micromotion (MM) and find PGC working for a MM modulation index β ⩽ 0.1. Still, we find that the spectral impurity of the laser field affects both, cooling rates and cooling limits. Thus, a Fabry–Pérot cavity filter is employed to efficiently suppress amplified spontaneous emission of the diode laser. We demonstrate mean phonon numbers for a single ion of 5.4(4) at a trap frequency of 2 π × 285 kHz and 3.3(4) at 2 π × 480 kHz, in the axial and radial directions, respectively.

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Laser cooling of a single trapped ion with Zeeman substructure below the Doppler limit is considered theoretically. The laser field consists of two counterpropagating beams linearly polarized in different directions, and the internal atomic transition is Jg{\mathit{J}}_{\mathit{g}}Jg​=1/2\ensuremath{\rightarrow}Je{\mathit{J}}_{\mathit{e}}Je​=3/2. The ion is assumed to be localized to spatial dimensions smaller than the optical wavelength (Lamb-Dicke limit) and placed at a specific position with respect to the laser beams. Under the assumption that the rate for optical pumping between the atomic ground states defines the smallest time constant in the system, analytic expressions for the final energy and the cooling rates are derived, with both a semiclassical and a full quantum treatment. The results show that laser cooling of a trapped ion using polarization gradients leads to very low energies. These energies are insensitive to the precise localization of the ion with respect to the lasers, the angle between the direction of the polarizations of the laser beams, and the detuning of the cooling laser.
We present two cooling mechanisms that lead to temperatures well below the Doppler limit. These mechanisms are based on laser polarization gradients and work at low laser power when the optical-pumping time between different ground-state sublevels becomes long. There is then a large time lag between the internal atomic response and the atomic motion, which leads to a large cooling force. In the simple case of one-dimensional molasses, we identify two types of polarization gradient that occur when the two counterpropagating waves have either orthogonal linear polarizations or orthogonal circular polarizations. In the first case, the light shifts of the ground-state Zeeman sublevels are spatially modulated, and optical pumping among them leads to dipole forces and to a Sisyphus effect analogous to the one that occurs in stimulated molasses. In the second case (σ+−σ− configuration), the cooling mechanism is radically different. Even at very low velocity, atomic motion produces a population difference among ground-state sublevels, which gives rise to unbalanced radiation pressures. From semiclassical optical Bloch equations, we derive for the two cases quantitative expressions for friction coefficients and velocity capture ranges. The friction coefficients are shown in both cases to be independent of the laser power, which produces an equilibrium temperature proportional to the laser power. The lowest achievable temperatures then approach the one-photon recoil energy. We briefly outline a full quantum treatment of such a limit.
A theoretical analysis is given for one-dimensional laser cooling below the Doppler limit of J=1/2 ground-state atoms. The laser field consists of a pair of counterpropagating, linearly polarized, low-power beams, whose polarization directions differ by an angle \ensuremath{\theta} (0\ensuremath{\le}\ensuremath{\theta}\ensuremath{\le}\ensuremath{\pi}/2). For \ensuremath{\theta}\ensuremath{\ll}1, the effective optical-pumping time is shown to increase strongly near the nodes of the standing wave, and the cooling force can be much larger than that for \ensuremath{\theta}=\ensuremath{\pi}/2. Moreover, for \ensuremath{\theta}\ensuremath{\ll}1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for \ensuremath{\theta}=\ensuremath{\pi}/2. As a consequence it is possible to achieve an equilibrium atomic distribution that, for \ensuremath{\theta}\ensuremath{\ll}1, is characterized by a mean kinetic energy that is lower than that predicted to occur for \ensuremath{\theta}=\ensuremath{\pi}/2. The equilibrium velocity distribution is not necessarily Maxwellian, and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms may be trapped in the vicinity of the laser-field nodes.
We present a semiclassical laser-cooling theory for an ion bound in a quadratic potential well, allowing for an arbitrary internal level scheme of the ion and an arbitrary polarization of the light field. The special case that the ion moves in a region much smaller than the wavelength of the exciting light (Lamb-Dicke limit), as well as an additional low-intensity limit, are worked out in detail. Explicit general expressions are given for the damping and diffusion tensors of the center-of-mass motion of the ion, and the light-induced renormalization of the mechanical oscillation frequencies is discussed. The formalism is implemented analytically using a computer program mathematica for an ion with a j=1/2\ensuremath{\rightarrow}j=3/2 transition moving in a one-dimensional optical molasses consisting of two counterpropagating laser beams with perpendicular linear polarizations (lin \ensuremath{\perp} lin). For a weakly bound ion at negligible saturation, the greatest lower limit of excitation energy turns out to be (33/20)1/2{)}^{1/2})1/2-1/2\ensuremath{\approxeq}0.78 vibrational quanta above the zero-point energy.
Laser cooling of trapped ions in a standing- and running-wave configuration is discussed theoretically. The ions are assumed to be spatially localized on the scale provided by the wavelength of the laser (Lamb-Dicke limit). A master equation for the center-of-mass distribution of the ion is derived for a multilevel system, and explicit results are presented for two- and three-level systems and harmonic trapping potentials. For the two-level system located at the node of the standing wave, we find final temperatures that are a factor of 2 lower than the limit for a running wave and cooling rates that do not saturate with the laser intensity. At the point of maximum gradient of the standing wave, blue detuned cooling is found that is analogous to the Sisyphus cooling of free atoms. For a three-level system we compare our results with those of Wineland, Dalibard, and Cohen-Tannoudji [J. Opt. Soc. Am. B 9, 32 (1992)].
A theoretical analysis is given for 1-D laser cooling below the Doppler limit of J = 1/2 ground- state atoms. The laser field consists of a pair of counterpropagating, linearly polarized low- power beams, whose polarization directions differ by an angle θ (0 ≤ θ ≤ π/2). For θ ≪ 1, the effective optical pumping time is shown to increase strongly near the nodes of the standing wave and the cooling force can be much larger than that for θ ~1. Moreover, for θ ≪ 1, it can be shown that the stimulated part of the atomic diffusion is reduced considerably as compared with that for θ ~ 1. As a consequence it is possible to achieve an equilibrium atomic distribution that, for θ ≪ 1, is characterized by a mean kinetic energy lower than that predicted to occur for θ = π/2. The equilibrium velocity distribution is not necessarily Maxwellian and thus the temperature of the atomic ensemble may not be well defined. The achievable kinetic energy is so small that the cooled atoms are trapped in the vicinity of the laser field nodes. An explanation for these effects is given in terms of Sisyphus cooling.
Abstract We implement three-dimensional polarization gradient cooling (PGC) of trapped ions. Counter-propagating laser beams near 393 nm impinge in lin ⊥ lin configuration, at a frequency below the S 1/2 to P 3/2 resonance in 40 Ca + . Our measurements demonstrate that cooling with laser beams detuned to lower frequencies from the resonance is robust against an elevated phonon occupation number and works continuously in the crossover from regular Doppler cooling to detunings of tens of linewidths. It is thus robust against heating events and also works well for an initial ion motion far out of the Lamb–Dicke regime. We show that PGC performance strongly depends on residual micromotion (MM) and find PGC working for a MM modulation index β ⩽ 0.1. Still, we find that the spectral impurity of the laser field affects both, cooling rates and cooling limits. Thus, a Fabry–Pérot cavity filter is employed to efficiently suppress amplified spontaneous emission of the diode laser. We demonstrate mean phonon numbers for a single ion of 5.4(4) at a trap frequency of 2 π × 285 kHz and 3.3(4) at 2 π × 480 kHz, in the axial and radial directions, respectively.