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arXiv:1705.00453 · Physical Review A

Doppler cooling thermometry of a multilevel ion in the presence of micromotion

Tomáš Šikorský, Ziv Meir, Nitzan Akerman, Ruti Ben-shlomi, Roee Ozeri

Published Jul 28, 2017• 27 citations
arXivHTMLPDF

Abstract

We study the time-dependent fluorescence of an initially hot, multilevel, single atomic ion trapped in a radio-frequency Paul trap during Doppler cooling. We have developed an analytical model that describes the fluorescence dynamics during Doppler cooling which is used to extract the initial energy of the ion. While previous models of Doppler cooling thermometry were limited to atoms with a two-level energy structure and neglected the effect of the trap oscillating electric fields, our model applies to atoms with multilevel energy structure and takes into account the influence of micromotion on the cooling dynamics. This thermometry applies to any initial energy distribution. We experimentally test our model with an ion prepared in coherent, thermal, and Tsallis energy distributions.

DOI
10.1103/physreva.96.012519

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We study the time-dependent fluorescence of an initially hot, multilevel, single atomic ion trapped in a radio-frequency Paul trap during Doppler cooling. We have developed an analytical model that describes the fluorescence dynamics during Doppler cooling which is used to extract the initial energy of the ion. While previous models of Doppler cooling thermometry were limited to atoms with a two-level energy structure and neglected the effect of the trap oscillating electric fields, our model applies to atoms with multilevel energy structure and takes into account the influence of micromotion on the cooling dynamics. This thermometry applies to any initial energy distribution. We experimentally test our model with an ion prepared in coherent, thermal, and Tsallis energy distributions.
We investigate the temporal dynamics of Doppler cooling of an initially hot single trapped atom in the weak-binding regime using a semiclassical approach. We develop an analytical model for the simplest case of a single vibrational mode for a harmonic trap, and show how this model allows us to estimate the initial energy of the trapped particle by observing the time-dependent fluorescence during the cooling process. The experimental implementation of this temperature measurement provides a way to measure atom heating rates by observing the temperature rise in the absence of cooling. This method is technically relatively simple compared to conventional sideband detection methods, and the two methods are in reasonable agreement. We also discuss the effects of rf micromotion, relevant for a trapped atomic ion, and the effect of coupling between the vibrational modes on the cooling dynamics.
We report on observations of the thermal motion of a single, Doppler-cooled ion along the axis of a linear radio-frequency quadrupole trap. We show that for a harmonic potential the thermal occupation of energy levels leads to a Gaussian distribution of the ion's axial position. The dependence of the spatial thermal spread on the trap potential is used for precise calibration of our imaging system's point spread function and sub-millikelvin thermometry. We employ this technique to investigate the laser detuning dependence of the Doppler temperature.
We study the probability distribution of an atomic ion being laser-cooled in a radio-frequency Paul trap, in terms of Hamiltonian action-angle coordinates appropriate for the time-dependent potential. Close to the effective minimum in many Paul traps, the periodically-driven potential is approximately quadratic in the coordinates. We find that despite the microscopic nonequilibrium forces, a stationary thermal-like exponential distribution in the action is reached after coarse-graining the angles, with a mean action corresponding to the Doppler cooling limit. However, residual electric fields can push the ion from the origin of the quadrupole potential and set it into a large-amplitude oscillation. Above a threshold amplitude of such excess micromotion, the action distribution for motion expanded about the driven oscillation broadens and becomes distinctly nonthermal. We find that by a proper choice of the laser detuning the distribution can be made exponential again, with a mean action close to the Doppler cooling limit. This is important for quantum information processing and other applications, and in particular the derived approach can be immediately applied to crystals of trapped ions in planar configurations, where the driven motion of ions is unavoidable.
We investigate the problem of a single ion in a radio-frequency trap and immersed in an ultracold Bose gas either in condensed or non-condensed phase. We develop master equation formalism describing the sympathetic cooling and we determine the cooling rates and final energies of ions. We show that cold atomic reservoir modifies the stability diagram of the ion in the Paul trap creating the regions where the ion is either cooled or heated due to the energy quanta exchanged with the time-dependent potential. Our calculation indicates that micromotion constitutes an important source of heating limiting the final temperature of ions to values higher than 100μ\muμK for parameters of present experiments.
Micromotion of ions in Paul traps has several adverse effects, including alterations of atomic transition line shapes, significant second-order Doppler shifts in high-accuracy studies, and limited confinement time in the absence of cooling. The ac electric field that causes the micromotion may also induce significant Stark shifts in atomic transitions. We describe three methods of detecting micromotion. The first relies on the change of the average ion position as the trap potentials are changed. The second monitors the amplitude of the sidebands of a narrow atomic transition, caused by the first-order Doppler shift due to the micromotion. The last technique detects the Doppler shift induced modulation of the fluorescence rate of a broad atomic transition. We discuss the detection sensitivity of each method to Doppler and Stark shifts, and show experimental results using the last technique.
We investigate the dynamics of an ion sympathetically cooled by another laser-cooled ion or small ion crystal. To this end, we develop simple models of the cooling dynamics in the limit of weak Coulomb interactions. Experimentally, we create a two-ion crystal of Ca + and Al + by photo-ionization of neutral atoms produced by laser ablation. We characterize the velocity distribution of the laser-ablated atoms crossing the trap by time-resolved fluorescence spectroscopy. We observe neutral atom velocities much higher than the ones of thermally heated samples and find as a consequence long sympathethic cooling times before crystallization occurs. Our key result is a new technique for detecting the loading of an initially hot ion with energy in the eV range by monitoring the motional state of a Doppler-cooled ion already present in the trap. This technique not only detects the ion but also provides information about the dynamics of the sympathetic cooling process.