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Radio-frequency atomic magnetometers: an analysis of interrogation regimes

Jenelle Rajroop

Published Jun 28, 2018• 0 citations
OpenAlex

Abstract

An atomic magnetometer is a sensor which is used to measure a magnetic field through its interaction with the atomic sample. Significant research into atomic magnetometry has led to the development of very sensitive atomic sensors capable of matching the sensitivity of the most sensitive magnetometers, superconducting quantum interference devices (SQUIDs). Because SQUIDS require cryogenics to operate, atomic magnetometers provide a sensitive, yet low-cost alternative. They have found use in many areas such as medicine, security, explosives detection and fundamental physics research. One of the primary factors influencing sensitivity is the detuning of the probe beam from the resonant transitions of the atomic ground state. A caesium room temperature radio-frequency (rf) magnetometer is constructed and used to investigate the influence of the probe beam detuning on the magnetometer signal of the F = 3 and F = 4 ground states. The results of probing near and far from resonance revealed an off-resonant regime and two absorptive regimes. In the off-resonant regime, the atomic spins are unperturbed by the probe beam; it is a quantum non-demolition (QND) interaction. The two absorptive regimes, found when the probe beam is in the vicinity of either the 62S1 2 F = 3 → 6 2P3 2 F 0 = 2,3,4 or the 62S1 2 F = 4 → 6 2P3 2 F 0 = 3,4,5 transitions, is characterised as a non-QND interaction in which the probe beam influences the measurement. The sensitivity of the rf magnetometer is determined to be ≈ 1.98 fT/ √ Hz. In addition, the exploration of the relationship between the signal to noise ratio (SNR) and probe beam detuning revealed that the SNR is constant with detuning but the larger the detuning, the higher the probe beam power needs to be to reach the optimum SNR.

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Physical Review Letters•Aug 3, 2005•312 citations
An atomic magnetometer is a sensor which is used to measure a magnetic field through its interaction with the atomic sample. Significant research into atomic magnetometry has led to the development of very sensitive atomic sensors capable of matching the sensitivity of the most sensitive magnetometers, superconducting quantum interference devices (SQUIDs). Because SQUIDS require cryogenics to operate, atomic magnetometers provide a sensitive, yet low-cost alternative. They have found use in many areas such as medicine, security, explosives detection and fundamental physics research. One of the primary factors influencing sensitivity is the detuning of the probe beam from the resonant transitions of the atomic ground state. A caesium room temperature radio-frequency (rf) magnetometer is constructed and used to investigate the influence of the probe beam detuning on the magnetometer signal of the F = 3 and F = 4 ground states. The results of probing near and far from resonance revealed an off-resonant regime and two absorptive regimes. In the off-resonant regime, the atomic spins are unperturbed by the probe beam; it is a quantum non-demolition (QND) interaction. The two absorptive regimes, found when the probe beam is in the vicinity of either the 62S1 2 F = 3 → 6 2P3 2 F 0 = 2,3,4 or the 62S1 2 F = 4 → 6 2P3 2 F 0 = 3,4,5 transitions, is characterised as a non-QND interaction in which the probe beam influences the measurement. The sensitivity of the rf magnetometer is determined to be ≈ 1.98 fT/ √ Hz. In addition, the exploration of the relationship between the signal to noise ratio (SNR) and probe beam detuning revealed that the SNR is constant with detuning but the larger the detuning, the higher the probe beam power needs to be to reach the optimum SNR.
We propose and demonstrate a radio-frequency (rf) atomic magnetometer based on parametric resonances. Previously, most rf atomic magnetometers are based on magnetic resonances and their sensitivities are often limited by spin-exchange relaxation. Here, we introduce a novel scheme for an rf magnetometer where the rf magnetic field is measured by exciting the parametric resonances instead of magnetic resonances using parametric modulation fields. In this way, the spin-exchange relaxation is almost eliminated. Benefiting from the low spin relaxation rate, the parametric resonance scheme exhibits a narrower linewidth and stronger signal, which results in a higher sensitivity. With a 6×6×3 mm^{3} Rb atomic vapor cell, we developed an rf atomic magnetometer with a noise floor of 2 fT/Hz^{1/2}, which is about one order of magnitude higher than the sensitivity achieved in the magnetic-resonance-based scheme. The presented rf detection scheme holds promise in advancing rf atomic magnetometers and brings new insight into their various applications.
Optically pumped radio frequency (RF) atomic magnetometers have been shown to have an improved sensitivity over standard tuned coils for frequencies less than 50 MHz, making these RF magnetometers attractive for the detection of nuclear quadrupole resonance (NQR) and low-field nuclear magnetic resonance (NMR) signals. In an atomic magnetometer a linearly polarized probe beam measures, through Faraday rotation, the transverse atomic magnetization induced by the resonant RF signal. The resonance, or Larmor, frequency of the magnetometer is easily tuned with a small magnetic field. We construct an atomic magnetometer based on a potassium vapor cell with a measured sensitivity of 0.22 ± 0.02 fT/ √ Hz and a detection bandwidth of 334 ± 11 Hz when tuned to 423 kHz, giving a Q of over 1200. While high Q magnetometers are sensitive to weak magnetic fields, they are also sensitive to magnetic transients, such as those associated with the excitation pulses needed for magnetic resonance. The ringing created by such transients can obscure the signal of interest. This is particularly detrimental for magnetic resonance signals that decay faster than the transverse relaxation rate. We demonstrate that by feeding back part of the optical signal to orthogonal electromagnetic coils, this unwanted ringing can be quickly damped out leaving the magnetometer ready for the detection of the signal. This negative feedback as applied to the K spins is called spin-damping and can be used to relax the K atoms faster by more than two orders of magnitude. Using spin-damping we reduce the dead-time before data acquisition from 0.8 to 0.2 ms in the detection of NQR signals from ammonium nitrate, one of the so-called fertilizer bomb explosives with an NQR frequency of 423 kHz. Furthermore, we discover that spin-damping can not only be used to suppress signals, it can also be used to suppress noise. We show that it can be used to suppress both environmental noise and more fundamental quantum noise, such as photon shot and spin projection noise. The latter suppression opens the door for its use in quantum control to initialize spin systems before measurements. For phase-sensitive detection, as is often used in magnetic resonance, spin-damping suppresses signal and noise in such a way as to increase the sensitivity bandwidth of the magnetometer. We prove, both theoretically and experimentally, that it is possible to increase the magnetometer detection bandwidth by a factor of 3 or more without significant loss in sensitivity. Such gains in bandwidth for a high Q magnetometer translate into savings in detection time, particularly for substance detection where the frequency of the signal of interest may not be completely known.
Abstract The magnetic field is one of the most fundamental and ubiquitous physical observables, carrying information about all electromagnetic phenomena. For the past 30 years, superconducting quantum interference devices (SQUIDs) operating at 4 K have been unchallenged as ultrahigh-sensitivity magnetic field detectors1, with a sensitivity reaching down to 1 fT Hz-1/2 (1 fT = 10-15 T). They have enabled, for example, mapping of the magnetic fields produced by the brain, and localization of the underlying electrical activity (magnetoencephalography). Atomic magnetometers, based on detection of Larmor spin precession of optically pumped atoms, have approached similar levels of sensitivity using large measurement volumes2, 3, but have much lower sensitivity in the more compact designs required for magnetic imaging applications4. Higher sensitivity and spatial resolution combined with non-cryogenic operation of atomic magnetometers would enable new applications, including the possibility of mapping non-invasively the cortical modules in the brain. Here we describe a new spin-exchange relaxation-free (SERF) atomic magnetometer, and demonstrate magnetic field sensitivity of 0.54 fT Hz-1/2 with a measurement volume of only 0.3 cm3. Theoretical analysis shows that fundamental sensitivity limits of this device are below 0.01 fT Hz-1/2. We also demonstrate simple multichannel operation of the magnetometer, and localization of magnetic field sources with a resolution of 2 mm.
Spin-exchange relaxation-free (SERF) atomic magnetometers are the promising non-cryogenic sensors to potentially replace the superconducting quantum interference device (SQUID) in the ultra-weak magnetic-field measurements. Although the SERF magnetometers have achieved a sensitivity of sub-femtotesla, the bandwidth is limited at a narrow range. In this work, we developed a closed-loop SERF magnetometer under proportional-integral (PI) control, the bandwidth could be adaptively tuned and extended above 1.2 kHz. A nearly 40-fold enhancement of the typical bandwidth was achieved in comparison with the open-loop system and the sensitivity was maintained at 15 fT/Hz1/2from 30 Hz to 750 Hz. Moreover, the magnetic field dynamic range could also be greatly improved. This proposed atomic magnetometer with higher bandwidth, sensitivity, and dynamic range has a good prospect in developing a compact, portable, and non-cryogenic magnetic field sensor and may find more applications in biomedical, nuclear magnetic resonance, and fundamental physics research.
We describe an alkali-metal magnetometer for detection of weak magnetic fields in the radio-frequency (rf) range. High sensitivity is achieved by tuning the Zeeman resonance of alkali atoms to the rf frequency and partially suppressing spin-exchange collisions in the alkali-metal vapor. We demonstrate magnetic field sensitivity of 2 fT/Hz(1/2) at a frequency of 99 kHz with a resonance width of 400 Hz. We also derive a simple analytic expression for the fundamental limit on the sensitivity of the rf magnetometer and show that a sensitivity of about 0.01 fT/Hz(1/2) can be achieved in a practical system with a measurement volume of 200 cm3.