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A Complex atom lens

Erik Anciaux

Published Jan 1, 2018• 0 citations
Publisher

Abstract

This dissertation presents progress on an atomic beam brightening and focusing experiment that has been shown to create a beam with higher brightness and greater resolution than that of any previous atomic focusing experiment. Our method of beam brightening relies upon using a permanent magnetic hexapole as a lens in conjunction with transverse laser cooling to focus and collimate a supersonic beam of metastable neon atoms. We then use an adjustable electromagnetic hexapole as a lens to focus the brightened atomic beam. Neutral atom beams have long been used as a tool to spectroscopically probe two dimensional surfaces, however the lack of a means to create bright, high-resolution neutral atom beams has limited their utility as a nanoscale resolution probing mechanism. While optical and electron microscopy have been the workhorses of microscopy for decades, we believe that our scheme for beam brightening and focusing will unleash the promise of neutral atom microscopy. Our scheme of beam brightening and focusing can be repeated in series and reveals a pathway to true high density nanoscale neutral atom focusing. Simulations suggest that when combined with aberration correction, our scheme will be able to produce an atomic beam with sufficient brightness and resolution to be useful as a surface sensitive nanoscale probe.

DOI
10.15781/t29z90x01

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This dissertation presents progress on an atomic beam brightening and focusing experiment that has been shown to create a beam with higher brightness and greater resolution than that of any previous atomic focusing experiment. Our method of beam brightening relies upon using a permanent magnetic hexapole as a lens in conjunction with transverse laser cooling to focus and collimate a supersonic beam of metastable neon atoms. We then use an adjustable electromagnetic hexapole as a lens to focus the brightened atomic beam. Neutral atom beams have long been used as a tool to spectroscopically probe two dimensional surfaces, however the lack of a means to create bright, high-resolution neutral atom beams has limited their utility as a nanoscale resolution probing mechanism. While optical and electron microscopy have been the workhorses of microscopy for decades, we believe that our scheme for beam brightening and focusing will unleash the promise of neutral atom microscopy. Our scheme of beam brightening and focusing can be repeated in series and reveals a pathway to true high density nanoscale neutral atom focusing. Simulations suggest that when combined with aberration correction, our scheme will be able to produce an atomic beam with sufficient brightness and resolution to be useful as a surface sensitive nanoscale probe.
We report on progress towards a neutral atom imaging device that will be used for chemically sensitive surface microscopy and nanofabrication. Our novel technique for improving refractive power and correcting chromatic aberration in atom lenses is based on a fundamental paradigm shift from continuous-beam focusing to a pulsed, three-dimensional approach. Simulations of this system suggest that it will pave the way toward the long-sought goal of true atom imaging on the nanoscale. Using a prototype lens with a supersonic beam of metastable neon, we have imaged complex patterns with lower distortion and higher resolution than has been shown in any previous experiment. Comparison with simulations corroborates the underlying theory and encourages further refinement of the process.
The study of collisions between excited atoms requires high-intensity atomic beams to achieve detector signals of sufficient strength. Producing large densities of excited rare gas atoms R is especially difficult, since with conventional sources metastable atoms R make up a tiny fraction of ≈10-5 of the total beam flux. In such cases, 'brightening' the beam is the only way to achieve a sufficiently large flux. We have followed a scheme proposed by Metcalf to brighten an atomic beam of neon. The setup employs laser cooling on the Ne((3s)3P2 → (3p)3D3) cycling transition, and consists of three stages. First, we collimate all atoms emerging from a discharge source within a half-angle θ0 = 100 mrad. Second, the collimated beam is focused to a point. Third, the now converging beam is re-collimated to form a thin and bright atomic beam.
Summary form only given. Recently it has been demonstrated that neutral atomic beams can be focused by use of a laser as an atom-optical lens. Standing wave atom-optical (SW) lenses have been of particular interest because of the potential for both high-resolution and high-throughput lithography. In this paper, using sub-Doppler optical cooling schemes in conjunction with mechanical collimation, and a SW with /spl sigma/=56 /spl mu/m, we have been able to achieve <20 nm resolution with contrast of at least 10:1, focusing a thermal atomic sodium beam using 589-nm light corresponding to the D/sub 2/ transition.
Neutral Helium atoms have significant potential for use as a probe in a matter-wave microscope. Their low energy scattering interactions with surfaces are well understood within the field of Helium Atom Scattering, where they have been shown to be sensitive to the presence of adsorbates, surface phonons and metalisation of surfaces. A focused probe of neutral Helium atoms could exploit this sensitivity and provide spatially resolved information for surfaces when scanned in two dimensions, thereby realising a Scanning Helium Microscope (SHeM). The ultimate resolution of a SHeM is set by the size of the Helium focus, and is ultimately limited by the sub-angstrom de Broglie wavelength of thermal Helium atoms. This thesis describes progress towards the demonstration of a SHeM using optical potential lenses to focus ground state neutral Helium atoms. The AC Stark effect is exploited to create an optical potential lens to focus a supersonic Helium beam. This is the first experimental demonstration of neutral Helium focusing using far off resonant fields. In addition, a high efficiency detection scheme for neutral Helium atoms (50%) using multiphoton ionisation is developed for use in SHeM. This represents a significant improvement on the very poor efficiency of electron bombardment detection schemes commonly used in Helium experiments. This detection scheme offers potentially sub-micron spatial resolution, and nanosecond temporal resolution.
Intense, highly collimated sources of atoms have many potential applications. Bright beams will be important for competitive high flux and high resolution direct-write techniques in lithography, with the added advantage of parallel writing through laser manipulation. Intense sources will also be useful in other atom optic devices e.g. for loading atoms into hollow fiber waveguides. In atomic physics, many collision processes can only be measured with the sensitivity offered by such high flux sources. We report progress on the development of an intense, collimated beam of metastable helium atoms which improves the brightness generated by conventional nozzle discharge sources by several orders of magnitude. The system uses diode lasers to transversely collimate and then to longitudinally slow the atoms, using Zeeman tuning to compensate for the changing Doppler shift. The slowed, collimated beam is then compressed in a 2D magneto-optic trap before a final collimation stage, to achieve the required increase in intensity. Initial experiments using the helium source for some of the applications above are described.
The evolving field of nanofabrication demands that more precise fabrication and evaluation tools be developed. We describe a method for creating a high quality focused ion beam with enhanced capabilities using an ion source based on laser-cooled neutral atoms in a magneto-optical trap. This technique will improve resolution and brightness beyond the current state of the art, can be used with the full range of atomic species that can be laser cooled and trapped, and will allow unprecedented control over the ion emission, allowing, for example, the production of single ions ``on demand.'' We give estimates for the emittance and present a realistic ray tracing analysis of a basic focusing system demonstrating the feasibility of focusing the beam to a spot size of less than 10nm10\phantom{\rule{0.3em}{0ex}}\mathrm{nm}10nm.