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The Journal of Chemical Physics

Communication: Neutral atom imaging using a pulsed electromagnetic lens

Jamie Ryan Gardner, Erik Anciaux, Mark G. Raizen

Published Feb 22, 2017• 13 citations
Publisher

Abstract

We report on progress towards a neutral atom imaging device that will be used for chemically sensitive surface microscopy and nanofabrication. Our novel technique for improving refractive power and correcting chromatic aberration in atom lenses is based on a fundamental paradigm shift from continuous-beam focusing to a pulsed, three-dimensional approach. Simulations of this system suggest that it will pave the way toward the long-sought goal of true atom imaging on the nanoscale. Using a prototype lens with a supersonic beam of metastable neon, we have imaged complex patterns with lower distortion and higher resolution than has been shown in any previous experiment. Comparison with simulations corroborates the underlying theory and encourages further refinement of the process.

DOI
10.1063/1.4976986

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We report on progress towards a neutral atom imaging device that will be used for chemically sensitive surface microscopy and nanofabrication. Our novel technique for improving refractive power and correcting chromatic aberration in atom lenses is based on a fundamental paradigm shift from continuous-beam focusing to a pulsed, three-dimensional approach. Simulations of this system suggest that it will pave the way toward the long-sought goal of true atom imaging on the nanoscale. Using a prototype lens with a supersonic beam of metastable neon, we have imaged complex patterns with lower distortion and higher resolution than has been shown in any previous experiment. Comparison with simulations corroborates the underlying theory and encourages further refinement of the process.
This dissertation presents progress on an atomic beam brightening and focusing experiment that has been shown to create a beam with higher brightness and greater resolution than that of any previous atomic focusing experiment. Our method of beam brightening relies upon using a permanent magnetic hexapole as a lens in conjunction with transverse laser cooling to focus and collimate a supersonic beam of metastable neon atoms. We then use an adjustable electromagnetic hexapole as a lens to focus the brightened atomic beam. Neutral atom beams have long been used as a tool to spectroscopically probe two dimensional surfaces, however the lack of a means to create bright, high-resolution neutral atom beams has limited their utility as a nanoscale resolution probing mechanism. While optical and electron microscopy have been the workhorses of microscopy for decades, we believe that our scheme for beam brightening and focusing will unleash the promise of neutral atom microscopy. Our scheme of beam brightening and focusing can be repeated in series and reveals a pathway to true high density nanoscale neutral atom focusing. Simulations suggest that when combined with aberration correction, our scheme will be able to produce an atomic beam with sufficient brightness and resolution to be useful as a surface sensitive nanoscale probe.
The imaging of a neutral atomic beam by electrostatic force has been demonstrated. An ultracold neon atomic beam in the 1s3[(2p)53s:1P0]{1s}_{3}[{(2p)}^{5}{3s:}^{1}{P}_{0}]1s3​[(2p)53s:1P0​] state illuminated a transparent object, passed through a set of three electrostatic lenses, and formed the image on a microchannel plate detector with the magnification of unity. Each lens consisted of two parallel cylinders that functioned as a concave lens along one axis and as a convex lens along the other axis. The atomic polarizability of neon in the 1s3{1s}_{3}1s3​ state has been also determined to be $2.8(\ifmmode\pm\else\textpm\fi{}0.1)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}39} {\mathrm{Fm}}^{2}.$
In the field of atom optics, there has been much interests in developing components such as lenses, mirrors, beam splitters and waveguides to manipulate neutral atoms. Especially many clever methods to focus neutral atoms have been developed. The lenses have been constructed using the static electrical and magnetic fields, Fresnel zone plates, and radiation pressure forces. Before the laser cooling and trapping techniques were invented, the electrostatic fields could not be used for manipulating neutral atoms because of its weak interaction energy with atoms. After the cold atoms were available, it has been possible to manipulate atoms with weak electrostatic interaction energy. We developed an atom lens system using electrostatic fields.
Matter-wave microscopy can be dated back to 1932 when Max Knoll and Ernst Ruska published the first image obtained with a beam of focussed electrons. In this paper a new step in the development of matter-wave microscopy is presented. We have created an instrument where a focussed beam of neutral, ground-state atoms (helium) is used to image a sample. We present the first 2D images obtained using this new technique. The imaged sample is a free-standing hexagonal copper grating (with a period of about 36 microm and rod thickness of about 8 microm). The images were obtained in transmission mode by scanning the focussed beam, which had a minimum spot size of about 2.0 microm in diameter (full width at half maximum) across the sample. The smallest focus achieved was 1.9 +/- 0.1 microm. The resolution for this experiment was limited by the speed ratio of the atomic beam through the chromatic aberrations of the zone plate that was used to focus. Ultimately the theoretical resolution limit is set by the wavelength of the probing particle. In praxis, the resolution is limited by the source and the focussing optics.
The emerging technique of neutral beam microscopy offers a non-perturbative way of imaging surfaces of various materials which cannot be studied using conventional microscopes. Current neutral beam microscopes use either diffractive focusing or pin-hole scanning to achieve spatial resolution, and are characterised by a strong dependence of the imaging time on the required resolution. In this work we introduce an alternative method for achieving spatial resolution with neutral atom beams which is based on manipulating the magnetic moments of the beam particles in a gradient field, and is characterised by a much weaker dependence of the imaging time on the image resolution. The validity of the imaging approach is demonstrated experimentally by reconstructing one dimensional profiles of the beam which are in good agreement with numerical simulation calculations. Numerical simulations are used to demonstrate the dependence of the signal to noise on the scan resolution and the topography of the sample, and assess the broadening effect due to the spread of velocities of the beam particles. The route towards implementing magnetic encoding in high resolution microscopes is discussed.
The most efficient method for controlling the motion of material particles in experimental physics is the use of interaction potentials with electromagnetic fields. The static magnetic and electric interaction potentials are used in the optics of charged particles. In the optics of neutral atoms, the various interaction potentials of atoms with laser and electromagnetic fields are used in addition to the static fields. The effective methods of diffraction, interference, mirror reflection of atoms are implemented in atom optics. The most difficult problem in atom optics is the problem of high-resolution focusing of neutral atoms, which is promising for the nondestructive method for probing the surface at the atomic level, as well as for the creation of nanostructures on the surface. Although there are many proposals for focusing of atomic beams, this problem is experimentally unsolved. The main difficulty is the creation of the interaction potential of the atom with the electromagnetic field that is close to an ideal lens for atoms.In this paper, we experimentally implement another approach to the problem of focusing and construction of an image in atom optics, which is based on a well known idea of optical pinhole camera. The pinhole camera in optics is a camera without lens. Light forming an image passes through a small hole. In our experiment with the atom pinhole camera the Cr atomic beam passes through a set of holes in a metal mask and thereby forms, by analogy with optics, a glowing object of a given geometry. The atoms pass through the holes in the mask, propagate in vacuum along rectilinear trajectories, similar to light rays, and are incident on a thin film (thickness 5 mum) placed at a distance of 90 mm from the mask with a large number (n =107-108/cm2) of nanoholes (50 nm diameter). Each hole of the film is a pinhole camera for atoms, which forms its individual image of the object on the substrate surface placed at a distance of l = 5mum behind the film.