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Nature Communications

Neutral beam microscopy with a reciprocal space approach using magnetic beam spin encoding

Morgan Lowe, Yosef Alkoby, Helen Chadwick, Gil Alexandrowicz

Published Aug 15, 2024• 2 citations
Publisher

Abstract

The emerging technique of neutral beam microscopy offers a non-perturbative way of imaging surfaces of various materials which cannot be studied using conventional microscopes. Current neutral beam microscopes use either diffractive focusing or pin-hole scanning to achieve spatial resolution, and are characterised by a strong dependence of the imaging time on the required resolution. In this work we introduce an alternative method for achieving spatial resolution with neutral atom beams which is based on manipulating the magnetic moments of the beam particles in a gradient field, and is characterised by a much weaker dependence of the imaging time on the image resolution. The validity of the imaging approach is demonstrated experimentally by reconstructing one dimensional profiles of the beam which are in good agreement with numerical simulation calculations. Numerical simulations are used to demonstrate the dependence of the signal to noise on the scan resolution and the topography of the sample, and assess the broadening effect due to the spread of velocities of the beam particles. The route towards implementing magnetic encoding in high resolution microscopes is discussed.

DOI
10.1038/s41467-024-51175-2

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•Jan 1, 2017•0 citations
The emerging technique of neutral beam microscopy offers a non-perturbative way of imaging surfaces of various materials which cannot be studied using conventional microscopes. Current neutral beam microscopes use either diffractive focusing or pin-hole scanning to achieve spatial resolution, and are characterised by a strong dependence of the imaging time on the required resolution. In this work we introduce an alternative method for achieving spatial resolution with neutral atom beams which is based on manipulating the magnetic moments of the beam particles in a gradient field, and is characterised by a much weaker dependence of the imaging time on the image resolution. The validity of the imaging approach is demonstrated experimentally by reconstructing one dimensional profiles of the beam which are in good agreement with numerical simulation calculations. Numerical simulations are used to demonstrate the dependence of the signal to noise on the scan resolution and the topography of the sample, and assess the broadening effect due to the spread of velocities of the beam particles. The route towards implementing magnetic encoding in high resolution microscopes is discussed.
The recently developed magnetic encoding beam microscopy approach to imaging with neutral atomic beams has a spatial resolution that is limited by the spread of velocities within the beam. Here we present a solution for overcoming this restriction which is based on adding a homogeneous magnetic field and resolving both the spatial resolution and the de Broglie wavelength of the particles using sequential Fourier transforms. Numerical simulations are used to demonstrate the enhanced resolution obtained with this approach, and how features which were lost in the spatial reconstruction due to the spread of velocities can be recovered. Wavelength/velocity resolved profiles that were reconstructed from experimental data are presented, demonstrating how the scheme can be applied in practice.
Matter-wave microscopy can be dated back to 1932 when Max Knoll and Ernst Ruska published the first image obtained with a beam of focussed electrons. In this paper a new step in the development of matter-wave microscopy is presented. We have created an instrument where a focussed beam of neutral, ground-state atoms (helium) is used to image a sample. We present the first 2D images obtained using this new technique. The imaged sample is a free-standing hexagonal copper grating (with a period of about 36 microm and rod thickness of about 8 microm). The images were obtained in transmission mode by scanning the focussed beam, which had a minimum spot size of about 2.0 microm in diameter (full width at half maximum) across the sample. The smallest focus achieved was 1.9 +/- 0.1 microm. The resolution for this experiment was limited by the speed ratio of the atomic beam through the chromatic aberrations of the zone plate that was used to focus. Ultimately the theoretical resolution limit is set by the wavelength of the probing particle. In praxis, the resolution is limited by the source and the focussing optics.
The most efficient method for controlling the motion of material particles in experimental physics is the use of interaction potentials with electromagnetic fields. The static magnetic and electric interaction potentials are used in the optics of charged particles. In the optics of neutral atoms, the various interaction potentials of atoms with laser and electromagnetic fields are used in addition to the static fields. The effective methods of diffraction, interference, mirror reflection of atoms are implemented in atom optics. The most difficult problem in atom optics is the problem of high-resolution focusing of neutral atoms, which is promising for the nondestructive method for probing the surface at the atomic level, as well as for the creation of nanostructures on the surface. Although there are many proposals for focusing of atomic beams, this problem is experimentally unsolved. The main difficulty is the creation of the interaction potential of the atom with the electromagnetic field that is close to an ideal lens for atoms.In this paper, we experimentally implement another approach to the problem of focusing and construction of an image in atom optics, which is based on a well known idea of optical pinhole camera. The pinhole camera in optics is a camera without lens. Light forming an image passes through a small hole. In our experiment with the atom pinhole camera the Cr atomic beam passes through a set of holes in a metal mask and thereby forms, by analogy with optics, a glowing object of a given geometry. The atoms pass through the holes in the mask, propagate in vacuum along rectilinear trajectories, similar to light rays, and are incident on a thin film (thickness 5 mum) placed at a distance of 90 mm from the mask with a large number (n =107-108/cm2) of nanoholes (50 nm diameter). Each hole of the film is a pinhole camera for atoms, which forms its individual image of the object on the substrate surface placed at a distance of l = 5mum behind the film.
Surface based geometries of microfabricated wires or patterned magnetic films can be used to magnetically trap and manipulate ultracold neutral atoms or Bose-Einstein condensates. We investigate the magnetic properties of such atom chips using a scanning magnetoresistive (MR) microscope with high spatial resolution and high field sensitivity. By comparing MR scans of a permanent magnetic atom chip to field profiles obtained using ultracold atoms, we show that MR sensors are ideally suited to observe small variations of the magnetic field caused by imperfections in the wires or magnetic materials which ultimately lead to fragmentation of ultracold atom clouds. Measurements are also provided for the magnetic field produced by a thin current-carrying wire with small geometric modulations along the edge. Comparisons of our measurements with a full numeric calculation of the current flow in the wire and the subsequent magnetic field show excellent agreement. Our results highlight the use of scanning MR microscopy as a convenient and powerful technique for precisely characterizing the magnetic fields produced near the surface of atom chips.
In 2008 we presented the first images obtained with a new type of matter wave microscope: NEutral Helium Atom MIcroscopy (NEMI). The main features in NEMI are the low energy of the atoms (<0.1 eV) and the fact that they are neutral. This means that fragile and/or insulating samples can be imaged without surface damage and charging effects. The ultimate resolution limit is given by the de Broglie wavelength (about 0.06 nm for a room-temperature beam), but reaching a small focus spot is still a major challenge. The best result previously was about 2 μ m. The main result of this paper is the focusing of a helium atom beam to a diameter below 1 μ m. A particular challenge for neutral helium microscopy is the optical element for focusing. The most promising option is to manipulate neutral helium via its de Broglie wavelength, which requires optical elements structured to nanometre precision. Here we present an investigation of the helium focusing properties of nanostructured Fresnel zone-plates. Experiments were performed by varying the illuminated area and measuring the corresponding focused spot sizes and focused beam intensities. The results were fitted to a theoretical model. There is a deviation in the efficiency of the larger zone plate, which indicates a distortion in the zone-plate pattern, but nevertheless there is good agreement between model and experiments for the focus size. This together with the demonstration of focusing to below 1 μ m is an important step towards nanometre resolution neutral helium microscopy.
Neutral Helium atoms have significant potential for use as a probe in a matter-wave microscope. Their low energy scattering interactions with surfaces are well understood within the field of Helium Atom Scattering, where they have been shown to be sensitive to the presence of adsorbates, surface phonons and metalisation of surfaces. A focused probe of neutral Helium atoms could exploit this sensitivity and provide spatially resolved information for surfaces when scanned in two dimensions, thereby realising a Scanning Helium Microscope (SHeM). The ultimate resolution of a SHeM is set by the size of the Helium focus, and is ultimately limited by the sub-angstrom de Broglie wavelength of thermal Helium atoms. This thesis describes progress towards the demonstration of a SHeM using optical potential lenses to focus ground state neutral Helium atoms. The AC Stark effect is exploited to create an optical potential lens to focus a supersonic Helium beam. This is the first experimental demonstration of neutral Helium focusing using far off resonant fields. In addition, a high efficiency detection scheme for neutral Helium atoms (50%) using multiphoton ionisation is developed for use in SHeM. This represents a significant improvement on the very poor efficiency of electron bombardment detection schemes commonly used in Helium experiments. This detection scheme offers potentially sub-micron spatial resolution, and nanosecond temporal resolution.