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Journal of Physics Conference Series

Superconducting stripline resonators at frequencies up to 50 GHz for microwave spectroscopy applications

Tobias Wollandt, Markus Thiemann, Martin Dressel, Marc Scheffler

Published Mar 1, 2018• 0 citations
Publisher

Abstract

Planar superconducting microwave resonators are commonly operated for various cryogenic applications, typically at frequencies between 2 and 15 GHz. But for certain applications, e.g. microwave spectroscopy to study the dynamics of charges and spins in solids, a wider spectral range is desired. Driving such microwave resonators at higher frequencies is challenging due to enhanced losses and reduced wavelength. Here we present superconducting stripline resonators operating at multiple frequencies as high as 50 GHz. These resonators are fabricated of Pb and can easily be adjusted to particular applications, including mK temperatures in a dilution refrigerator. Demonstrating such a resonator as a spectroscopic tool, we detect the superconducting transition of a Sn sample in a wide spectral range.

DOI
10.1088/1742-6596/969/1/012082

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Planar superconducting microwave resonators are commonly operated for various cryogenic applications, typically at frequencies between 2 and 15 GHz. But for certain applications, e.g. microwave spectroscopy to study the dynamics of charges and spins in solids, a wider spectral range is desired. Driving such microwave resonators at higher frequencies is challenging due to enhanced losses and reduced wavelength. Here we present superconducting stripline resonators operating at multiple frequencies as high as 50 GHz. These resonators are fabricated of Pb and can easily be adjusted to particular applications, including mK temperatures in a dilution refrigerator. Demonstrating such a resonator as a spectroscopic tool, we detect the superconducting transition of a Sn sample in a wide spectral range.
Abstract We demonstrate the operation of superconducting coplanar microwave resonators in a very large frequency range up to 50 GHz. The resonators are fabricated from niobium thin films on sapphire substrates and have fundamental frequencies of 5 GHz or 10 GHz. We study numerous harmonics of the resonators at temperatures between 1.5 K and 6 K, and we determine quality factors of up to 22 600 at 1.5 K. As an example for spectroscopy applications of such resonators we detect the superconducting transition of a bulk tin sample at multiple probing frequencies.
Planar superconducting microwave transmission line resonators can be operated at multiple harmonic resonance frequencies. This allows covering wide spectral regimes with high sensitivity, as it is desired, e.g., for cryogenic microwave spectroscopy. A common complication of such experiments is the presence of undesired “spurious” additional resonances, which are due to standing waves within the resonator substrate or housing box. Identifying the nature of individual resonances (“designed” vs “spurious”) can become challenging for higher frequencies or if elements with unknown material properties are included, as is common for microwave spectroscopy. Here, we discuss various experimental strategies to distinguish designed and spurious modes in coplanar superconducting resonators that are operated in a broad frequency range up to 20 GHz. These strategies include tracking resonance evolution as a function of temperature, magnetic field, and microwave power. We also demonstrate that local modification of the resonator, by applying minute amounts of dielectric or electron spin resonance-active materials, leads to characteristic signatures in the various resonance modes, depending on the local strength of the electric or magnetic microwave fields.
Superconducting resonators are widely used in fields spanning from quantum computing to electron spin resonance (ESR) spectroscopy. With the goal of realizing superconducting resonators, a broad variety and combination of superconducting materials, substrates and fabrication processes have been used and thoroughly reported in the literature. High temperature superconductors such as YBCO and low temperature superconductors such as Nb, NbN, NbTiN and Al are the major actors in the domain. In this work, we investigate the possibility to extend the family of suitable low temperature superconductors for the realization of planar superconducting microwave resonators for future ESR applications. In particular, this study focuses on NbTi, a widely used material to realize superconducting cables but not investigated for planar resonating structures at GHz frequencies. A 150 nm thick film of NbTi is sputtered and patterned on top of an Al2O3 substrate. For devices resonating around 6.8 GHz quality factors greater than 10,000 are observed at 3 K and in magnetic fields up to 250 mT.
In this master's thesis, I present the design, fabrication, and characterisation of superconducting microwave resonators. These resonators are quarter-wavelength coplanar waveguide resonators, operating at resonance frequencies between 4 GHz and 8 GHz. This kind of resonator is a key component in several applications, ranging from quantum computation devices to parametric amplifiers. Minimising the losses (achieving high internal quality factors) in these resonators is important to maximise performance of the applications they are used for. During the thesis work, we have studied several possible changes to improve the resonator quality.\n\nFabrication of the resonators was done in the Nanofabrication Laboratory at Chalmers University of Technology, and consist of the following steps: cleaning a sapphire or silicon wafer, depositing a layer of superconducting niobium, photolithography, and etching the waveguide. We then measured the resonators in a cryogen-free dilution refrigerator, at a temperature of 10 mK. The measurements consisted of a power sweep, in order to quantify the quality factor at high and low excitation powers. As an example, the first resonator we fabricated had a quality factor of 4.3 x 10^4 at high power (about 10^5 photons in the resonator), and quality factor of 3.7 x 10^4 at the single-photon level.\n\nWe then investigated different loss mechanisms that we expect to negatively affect the quality factor, and how to reduce this loss. Firstly, to reduce radiation losses and magnetic vortex losses, we reduced the lateral dimensions of the resonator. Secondly, as two-level system (TLS) losses are believed to mainly reside at the surfaces of the materials and interfaces between them, we etched into the substrate to selectively move a part of the TLS away from the resonator. We also studied the effect of the meandering of the resonator on the quality factor, as well as using two different etching gasses.\n\nBy gathering all this data, we were then able to compare the different combinations to see the effect of the changing parameters. In conclusion, the reduced lateral dimensions and the removal of part of the substrate indeed reduce the losses, as expected from the theory. We also found interesting behaviour with regards to the meandering, namely that having a meandered structure negatively affects the quality factor.\n\nCombining all results, we can give a guideline for the fabrication of resonators in the future, which gave us a quality factor up to 4.9 x 10^5 at high excitation power, and 3.0 x 10^5 at the single photon level.
The complex dielectric constant ε^=ε1+iε2\hatε = ε_1 + i ε_2ε^=ε1​+iε2​ of SrTiO3_33​ reaches high values ε1≈2∗104ε_1 \approx 2*10^{4}ε1​≈2∗104 at cryogenic temperatures, while the dielectric losses (ε2ε_2ε2​) are much stronger than for other crystalline dielectrics. SrTiO3_33​ is a common substrate for oxide thin films, like the superconducting LaAlO3_33​/SrTiO3_33​ system, but the large ε1ε_1ε1​ and ε2ε_2ε2​ restrict high-frequency quantum devices on SrTiO3_33​. Here we present superconducting coplanar Nb resonators on SrTiO3_33​, which we successfully operate in a distant-flip-chip geometry at frequencies that exceed 1 GHz. We find a pronounced and unexpected increase in resonator quality factor QQQ at temperatures below 1 K, reaching up to Q≈800Q \approx 800Q≈800. We attribute this to substantial changes of the dielectric losses in SrTiO3_33​ at mK temperatures, and we also detect non-monotonous changes in the temperature-dependent ε1ε_1ε1​. These findings challenge our present understanding of the dielectric properties of SrTiO3_33​ and at the same time demonstrate that cryogenic high-frequency devices on SrTiO3_33​ are more feasible than previously assumed.
We have fabricated a superconducting resonator capable of generating a strong microwave magnetic field in a small (100 μm) volume for low temperature magnetic resonance experiments. While the resonator was specifically developed for use at millikelvin temperatures in a dilution refrigerator, where the total cooling power is limited to a few hundred microwatts, it is also useful at temperatures up to 5 K. The resonator consists of a 220 μm diameter, 2-1/2 turn niobium coil resonating with a short section of niobium microstripline. At a resonance frequency of 3 GHz, the loaded Q of the resonator was 780. The field strength was characterized by performing electron spin nutations. Operating at 100 mK with 320 μW of dissipated power, the resonator generated a field of 4 G at a distance of 100 μm from the coil.