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Micro and Nano Engineering

Fabrication and characterization of NbTi microwave superconducting resonators

Roberto Russo, André Chatel, Nergiz Şahin Solmaz, Reza Farsi, H. Furci, Juergen Brügger, Giovanni Boero

Published May 10, 2023• 7 citations
Publisher

Abstract

Superconducting resonators are widely used in fields spanning from quantum computing to electron spin resonance (ESR) spectroscopy. With the goal of realizing superconducting resonators, a broad variety and combination of superconducting materials, substrates and fabrication processes have been used and thoroughly reported in the literature. High temperature superconductors such as YBCO and low temperature superconductors such as Nb, NbN, NbTiN and Al are the major actors in the domain. In this work, we investigate the possibility to extend the family of suitable low temperature superconductors for the realization of planar superconducting microwave resonators for future ESR applications. In particular, this study focuses on NbTi, a widely used material to realize superconducting cables but not investigated for planar resonating structures at GHz frequencies. A 150 nm thick film of NbTi is sputtered and patterned on top of an Al2O3 substrate. For devices resonating around 6.8 GHz quality factors greater than 10,000 are observed at 3 K and in magnetic fields up to 250 mT.

DOI
10.1016/j.mne.2023.100203

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Superconducting resonators are widely used in fields spanning from quantum computing to electron spin resonance (ESR) spectroscopy. With the goal of realizing superconducting resonators, a broad variety and combination of superconducting materials, substrates and fabrication processes have been used and thoroughly reported in the literature. High temperature superconductors such as YBCO and low temperature superconductors such as Nb, NbN, NbTiN and Al are the major actors in the domain. In this work, we investigate the possibility to extend the family of suitable low temperature superconductors for the realization of planar superconducting microwave resonators for future ESR applications. In particular, this study focuses on NbTi, a widely used material to realize superconducting cables but not investigated for planar resonating structures at GHz frequencies. A 150 nm thick film of NbTi is sputtered and patterned on top of an Al2O3 substrate. For devices resonating around 6.8 GHz quality factors greater than 10,000 are observed at 3 K and in magnetic fields up to 250 mT.
Abstract We systematically study the performance of compact lumped element planar microwave Nb70Ti30N (NbTiN) resonators operating at 5 GHz in external in-plane magnetic fields up to 440 mT, a broad temperature regime from 2.2 K up to 13 K, as well as mK temperatures. For comparison, the resonators have been fabricated on thermally oxidized and pristine, (001) oriented silicon substrates. When operating the resonators in the multi-photon regime at T = 2.2 K, we find internal quality factors Q int ≃ 2 × 105 for NbTiN resonators grown on pristine Si substrates. In addition, we investigate the Q-factors of the resonators on pristine Si substrates at millikelvin temperatures to assess their applicability for quantum applications. We find Q int ≃ 2 × 105 in the single photon regime and Q int ≃ 5 × 105 in the high power regime at T = 7 mK. From the excellent performance of our resonators over a broad temperature and magnetic field range, we conclude that NbTiN deposited on Si (100) substrates, where the surface oxide has been removed, constitutes a promising material platform for electron spin resonance and ferromagnetic resonance experiments using superconducting planar microwave resonators.
Microwave superconducting resonators are extensively studied in fields such as quantum computing and electron spin resonance (ESR) spectroscopy. However, the integration of superconducting resonators with feedback mechanisms to create ultra-low noise oscillators is a relatively unexplored area, and the application of such oscillators in ESR spectroscopy has not yet been demonstrated. In this work, we report the design, fabrication, and application of microwave oscillators based on superconducting resonators for ESR spectroscopy, illustrating an alternative way for the improvement of the performance of oscillator based ESR sensors. Specifically, ESR spectra are obtained by measuring the oscillator's frequency shift induced by the ESR effect as a function of the applied static magnetic field. The oscillators are composed of a single heterojunction bipolar transistor or high electron mobility transistor coupled with NbTi or YBa2Cu3O7 (YBCO) superconducting resonators. The fabricated oscillators operate at frequencies of 0.6 and 1.7 GHz and temperatures up to 80 K (for YBCO resonators) and 8 K (for NbTi resonators). The lowest measured frequency noise is about 9 mHz/Hz1/2 (−139 dBc/Hz), the best spin sensitivity is about 1×1010 spins/Hz1/2, and the best concentration sensitivity is about 3×1018 spins/Hz1/2m3. The approach proposed in this work should allow for significantly better spin and concentration sensitivities compared to those achievable with normal conductors, up to operating frequencies, magnetic fields, and temperatures, where superconductors exhibit substantially lower effective microwave resistance than normal conductors.
Superconducting microwave resonators are of interest for a wide range of applications, including for their use as microwave kinetic inductance detectors (MKIDs) for the detection of faint astrophysical signatures, as well as for quantum computing applications and materials characterization. In this paper, procedures are presented for the fabrication and characterization of thin-film superconducting microwave resonators. The fabrication methodology allows for the realization of superconducting transmission-line resonators with features on both sides of an atomically smooth single-crystal silicon dielectric. This work describes the procedure for the installation of resonator devices into a cryogenic microwave testbed and for cool-down below the superconducting transition temperature. The set-up of the cryogenic microwave testbed allows one to do careful measurements of the complex microwave transmission of these resonator devices, enabling the extraction of the properties of the superconducting lines and dielectric substrate (e.g., internal quality factors, loss and kinetic inductance fractions), which are important for device design and performance.
Superconducting microwave resonators are of interest for a wide range of applications, including for their use as microwave kinetic inductance detectors (MKIDs) for the detection of faint astrophysical signatures, as well as for quantum computing applications and materials characterization. In this paper, procedures are presented for the fabrication and characterization of thin-film superconducting microwave resonators. The fabrication methodology allows for the realization of superconducting transmission-line resonators with features on both sides of an atomically smooth single-crystal silicon dielectric. This work describes the procedure for the installation of resonator devices into a cryogenic microwave testbed and for cool-down below the superconducting transition temperature. The set-up of the cryogenic microwave testbed allows one to do careful measurements of the complex microwave transmission of these resonator devices, enabling the extraction of the properties of the superconducting lines and dielectric substrate (e.g., internal quality factors, loss and kinetic inductance fractions), which are important for device design and performance.
Titanium nitride is an attractive material for a range of superconducting quantum-circuit applications owing to its low microwave losses, high surface inductance, and chemical stability. The physical properties and device performance, nevertheless, depend strongly on the quality of the materials. In this paper, we focus on the highly crystalline and epitaxial titanium nitride thin films deposited on sapphire substrates using magnetron sputtering at an intermediate temperature (${300}^{\ensuremath{\circ}}\mathrm{C}$). We performed a set of systematic and comprehensive material characterizations to thoroughly understand the structural, chemical, and transport properties. Microwave losses at low temperatures were studied using patterned microwave resonators, where the best internal quality factor in the single-photon regime is measured to be $3.3\ifmmode\times\else\texttimes\fi{}{10}^{6}$ and that in the high-power regime $>1.0\ifmmode\times\else\texttimes\fi{}{10}^{7}$. Adjusted with the material filling factor of the resonators, the microwave loss-tangent here compares well with the previously reported best values for superconducting resonators. This work lays the foundation of using epitaxial titanium nitride for low-loss superconducting quantum circuits.
Abstract Amorphous NbTiN is widely applied in superconducting electronic devices owing to its merits of wide energy gap, high T c , and mitigated requirement in fabrication. Its highly disordered feature yields considerable kinetic inductance, making it an ideal material for parametric amplification. To build up the correspondence between the fabrication conditions and the desirable electrical performance, we designed, fabricated, and measured NbTiN microstrip resonators at microwave frequencies. The principal result is that the unloaded Q factor of the resonators does not depend on the film normal state resistivity, which largely depends on the sputtering pressure. This result is consistent with the dirty superconductor theories.