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Physical Review Letters

Nonequilibrium Precondensation of Classical Waves in Two Dimensions Propagating through Atomic Vapors

Neven Šantić, Adrien Fusaro, Sabeur Salem, Josselin C. Garnier, Antonio Picozzi, Robin Kaiser

Published Feb 2, 2018• 72 citations
Publisher

Abstract

The nonlinear Schrödinger equation, used to describe the dynamics of quantum fluids, is known to be valid not only for massive particles but also for the propagation of light in a nonlinear medium, predicting condensation of classical waves. Here we report on the initial evolution of random waves with Gaussian statistics using atomic vapors as an efficient two dimensional nonlinear medium. Experimental and theoretical analysis of near field images reveal a phenomenon of nonequilibrium precondensation, characterized by a fast relaxation towards a precondensate fraction of up to 75%. Such precondensation is in contrast to complete thermalization to the Rayleigh-Jeans equilibrium distribution, requiring prohibitive long interaction lengths.

DOI
10.1103/physrevlett.120.055301

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The nonlinear Schrödinger equation, used to describe the dynamics of quantum fluids, is known to be valid not only for massive particles but also for the propagation of light in a nonlinear medium, predicting condensation of classical waves. Here we report on the initial evolution of random waves with Gaussian statistics using atomic vapors as an efficient two dimensional nonlinear medium. Experimental and theoretical analysis of near field images reveal a phenomenon of nonequilibrium precondensation, characterized by a fast relaxation towards a precondensate fraction of up to 75%. Such precondensation is in contrast to complete thermalization to the Rayleigh-Jeans equilibrium distribution, requiring prohibitive long interaction lengths.
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The propagation of light in nonlinear media is well described by a 222D nonlinear Schrödinger equation (NLSE) within the paraxial approximation, which is equivalent to the Gross-Pitaesvskii equation (GPE), the mean-field description for the dynamics of Bose-Einstein condensates (BECs). Due to this similarity, many theoretical and experimental investigations of phenomena which have already been studied and realized in BECs have been recently analysed in alternative experimental platforms such as hot atomic vapours. In this work, we study the formation of droplets of light in these media, attempting to establish a mapping between the experimental parameters normally used in BEC experiments and those needed to observe the analogous phenomenon in hot atomic vapours. We obtain the energy functional for the susceptibility of the medium in the χ(3)χ^{(3)}χ(3) , χ(3)+χ(5)χ^{(3)}+χ^{(5)}χ(3)+χ(5) and saturating regimes for a two-level atomic configuration considering the focusing (attractive) regime. We apply a Gaussian variational approach and check its predictions through numerical simulations of the NLSE for each regime. Finally, we study the real-time dynamics of the system for both the χ(3)+χ(5)χ^{(3)}+χ^{(5)}χ(3)+χ(5) and saturating nonlinearities, focusing our attention on the behaviour of the breathing mode and on the analysis of droplet formation for realistic experimental conditions.
Quantum noise correlations have been employed in several areas in physics including condensed matter, quantum optics and ultracold atom to reveal non-classical states of the systems. So far, such analysis mostly focused on systems in equilibrium. In this paper, we show that quantum noise is also a useful tool to characterize and study the non-equilibrium dynamics of one dimensional system. We consider the Ramsey sequence of one dimensional, two-component bosons, and obtain simple, analytical expressions of time evolutions of the full distribution functions for this strongly-correlated, many-body system. The analysis can also be directly applied to the evolution of interference patterns between two one dimensional quasi-condensates created from a single condensate through splitting. Using the tools developed in this paper, we demonstrate that one dimensional dynamics in these systems exhibits the phenomenon known as "prethermalization", where the observables of non-equilibrium, long-time transient states become indistinguishable from those of thermal equilibrium states.