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Nonlinear dynamics in quantum fluids of light

Heitor Victor Santos da SILVA

Published Jul 25, 2023• 0 citations
OpenAlex

Abstract

The propagation of light in nonlinear media is well described by a 2D nonlinear Schrödinger equation (NLSE) within the paraxial approximation, which is equivalent to the GrossPitaevskii equation (GPE), the mean-field description for the dynamics of Bose-Einstein condensates (BECs). As a product of this similarity, we can establish the figure of a quantum fluid of light. Quantum fluids of light have been used for theoretical and experimental investigations of phenomena already studied and realised in BECs. In this thesis, we describe the mechanisms that make the conception of a quantum fluid of light possible for different experimental platforms. Furthermore, we present a study on the formation of self-bound droplets of light in hot atomic vapours, our chosen nonlinear medium, in an attempt to obtain a mapping between experimental parameters typically used in BEC experiments and those needed to observe the analogous phenomenon in atomic vapours. We investigate the static properties of the system, providing a phase diagram for the different and possible solutions for the optical regimes of interest. Finally, we systematically study droplet dynamics, focusing on the behaviour of the collective monopole excitation and the dynamic formation of these objects under realistic experimental conditions.

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The propagation of light in nonlinear media is well described by a $2$D nonlinear Schrödinger equation (NLSE) within the paraxial approximation, which is equivalent to the Gross-Pitaesvskii equation (GPE), the mean-field description for the dynamics of Bose-Einstein condensates (BECs). Due to this similarity, many theoretical and experimental investigations of phenomena which have already been studied and realized in BECs have been recently analysed in alternative experimental platforms such as hot atomic vapours. In this work, we study the formation of droplets of light in these media, attempting to establish a mapping between the experimental parameters normally used in BEC experiments and those needed to observe the analogous phenomenon in hot atomic vapours. We obtain the energy functional for the susceptibility of the medium in the $χ^{(3)}$ , $χ^{(3)}+χ^{(5)}$ and saturating regimes for a two-level atomic configuration considering the focusing (attractive) regime. We apply a Gaussian variational approach and check its predictions through numerical simulations of the NLSE for each regime. Finally, we study the real-time dynamics of the system for both the $χ^{(3)}+χ^{(5)}$ and saturating nonlinearities, focusing our attention on the behaviour of the breathing mode and on the analysis of droplet formation for realistic experimental conditions.

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Static and dynamic properties of self-bound droplets of light in hot vapors

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Paraxial fluid of light in hot atomic vapors

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Quantum fluids of light are the photonic counterpart of Bose gases. They currently attract increasing interest since they are versatile and highly tunable systems for probing many-body physics quantum phenomena, such as superfluidity. Superfluid flow of light has already been reported in microcavity exciton-polariton condensates but clear observation of this phenomenon in cavityless systems, that is, for propagating photon fluids, remains elusive. In this thesis, we study the hydrodynamical properties of light propagating close to resonance in hot rubidium vapors. Whereas photons in air are not interacting with each other, the situation is different in rubidium vapors, as an effective interaction between them, mediated by the atomic ensemble, appears. The light behaves therefore as a fluid flowing in the plane perpendicular to the optical axis. The primary purpose of this thesis was to show that light in those systems can behave as a superfluid. The first step toward the observation of superfluidity is to measure the dispersion relation of small amplitude density waves travelling onto the propagating photon fluid. I show that this dispersion exhibits a linear trend for small excitation wave-vectors, which is, according to the Landau criterion, a sufficient condition for guaranteeing superfluidity. I present then an all-optical defect experiment - where the photon fluid flows against an optically induced obstacle (namely, a local change of refractive index) - designed to measure the drag force cancellation at the fluid/superfluid threshold.

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An Investigation of the Collective Modes and Phases of Bose-Einstein Condensates

Priyam Das

Bose-Einstein condensate (BEC) is a new state of matter, experimentally realized in a dilute alkali gas of weakly interacting bosons. The gas is cooled to very low temperatures, of the order of nano-Kelvin, at which point a large fraction of the atoms occupy the lowest quantum state. Under such conditions, the quantum effects become apparent on a macroscopic scale. Many fundamental ideas of quantum mechanics have been realized and proven to be true in experiments, by studying the Bose-Einstein condensates. Amongst them, the observation of macroscopic matter wave interference, the creation of vortices, dark and bright solitons etc, find special mention. The dynamics of this system in presence of an optical lattice reveals a superfluid to Mott insulator quantum phase transition. This has opened a new avenue for research on BEC and its applications. From a theoretical standpoint, the dynamics of BEC can be described by means of an effective mean-field theory. This formalism is much simpler than the many-body Schr¨odinger equation and based on a classical nonlinear evolution equation, known as Gross-Pitaevskii equation. The nonlinear nature of the GPE leads to several interesting phenomena like soliton propagation, vortices, four wave mixing etc., which are closely related to nonlinear fiber optics. The present thesis deals with nonlinear excitations and different phases of BEC and is organized as follows: after a brief introduction, in chapter two, we start with BEC in a one-dimensional shallow optical lattice, experiencing both cubic and quintic nonlinearity. A superfluid density wave, of twice the periodicity of lattice potential, is identified. This indicates matter redistribution, where atoms from neighbouring sites have been depleted leading to a density wave behaviour. Interestingly, it ceases to exist when only one of these interactions is operative. We predict the loss of superfluidity through a classical dynamical phase transition, where modulational instability leads to the loss of phase coherence. In presence of pure two-body interaction, the superfluid density shows a periodicity commensurate with the lattice potential. Apart from the superfluid state, a density wave insulating phase is also found to exist, possessing two frequency modulations commensurate with the lattice potential. A dynamical phase transition connects the superfluid phase with an insulating phase, which in turn, is connected with the density wave insulating phase. The solutions are found to be marginally stable, as per the Vakhitov-Kolokolov (VK) criterion. Chapter three describes the dynamics of the atomic-molecular Bose-Einstein condensate (AMBEC) by mean-field Gross-Pitaevskii equation (GPE), taking into account the atom-molecular interaction, as well as atom-molecule inter-conversion. The two-body atom-atom, atom-molecule and molecule-molecule interactions are analogous to the cubic nonlinearity of the standard GPE, whereas, the quadratic nonlinear term arising from the inter-conversion between atoms and molecules is identical to the scenario in strongly coupled BEC in one dimension. The presence of both weak and strong interactions adds further richness to this system. We find the molecular BEC possesses a complex dark (grey) soliton, while the atomic condensate is a bright one. The energy and momentum of this system is computed in order to see the effect of the both weak and strong interactions on Lieb mode profile and compare it with the pure atomic condensate profile. Another class of solutions exist in this system, where both atomic and molecular condensates possess bright solitons. In chapter four, we investigate the effect of a harmonic trap on the dynamics of grey solitons in Bose-Einstein condensates. It is observed that, these nonlinear excitations of the cigar-shaped Bose-Einstein condensate have strong coupling with the trap at low momenta and hence can be effectively isolated from the Bogoliubov sound modes, which respond weakly to harmonic confinement. This strong coupling with the trap also makes the grey soliton amenable for control and manipulation through trap modulation and temporal variation of the two-body interaction. We have shown that in presence of an expulsive oscillator trap, the grey soliton gets amplified, while having a compression in its width. Exact solutions are also obtained in case of the two component Bose-Einstein condensates (TBECs), where one component is a grey soliton and the other a bright one. The presence of the trap and inter-species interaction significantly affects the grey soliton dynamics. Similar to the single component, in the present case, we have shown that both grey and bright soliton can be compressed simultaneously. A detailed study of the energy and momentum of the soliton is reported, in order to find the effect of the trap on the Lieb mode. In chapter five, we study a BEC-defect complex in a quasi-one dimensional scenario, where the defect atom moves in the condensate with constant velocity. Explicit solutions of the coupled mean-field equations, describing defect-grey soliton dynamics are obtained, demonstrating the coexistence of grey soliton and a localized defect. Unlike the case of dark soliton, where the defect trapping center has vanishing superfluid density, the moving grey soliton necessarily possesses a finite superfluid component at the defect location. The presence of the defect can lower the grey soliton’s maximum velocity, as compared to the defect free case, where the maximum velocity is the sound velocity. We have also carried out the stability analysis of the obtained solutions using renormalized momentum formalism and Vakhitov-Kolokolov criteria and find that the obtained solutions are stable through both the methods. The grey soliton’s energy gets substantially modified through its interaction with the defect, opening up the possibility of its control through defect dynamics. Chapter six describes a parametrically forced Bose-Einstein condensate in the presence of a general moving optical lattice. The interaction between the atoms in the condensate and the time dependent lattice potential leads to a novel propagating superfluid matter wave, which can be controlled through chirp management. This system, when placed in a trap, accelerates and undergoes rapid nonlinear compression, controlled by the chirp. The density achieves its maximum, when the matter wave changes direction. It is also shown that this system exhibits dynamical superfluid insulator transition, where superfluidity breaks down and the condensate transits to an insulating phase. The stability has been investigated using Vakhitov-Kolokolov criterion and found that it depends on the chirp, as well as on the nature of the atom-atom interaction. The exact expression for energy is obtained and analyzed in detail to gain physical understanding of the chirp management of the sinusoidal excitations and also the dynamical phase transition.

•Jul 1, 2011•0 citations

Investigation of Quantum Liquid in Quasi One Dimensional Bose-Einstein Condensate

Argha Debnath, Ayan Khan

Recent observations of droplets in dipolar and binary Bose-Einstein condensate (BEC) motivates us to study the theory of droplet formation in details. Precisely, we are interested in investigating the possibility of droplet formation in a quasi one dimensional geometry. The recent observation have concluded that the droplets are stabilized by the competition between effective mean-filed and beyond mean-field interaction. Hence, it is possible to map the effective equation of motion to a cubic-quartic nonlinear Schr\odinger equation (CQNLSE). We obtain two analytical solutions of the modified Gross-Pitaevskii equation or CQNLSE and based on their stability we investigate the parameter regime for which droplets can form. The effective potential allows us to conclude about the regions of soliton domination and self bound droplet formations.

•Aug 2, 2020•0 citations
The propagation of light in nonlinear media is well described by a 2D nonlinear Schrödinger equation (NLSE) within the paraxial approximation, which is equivalent to the GrossPitaevskii equation (GPE), the mean-field description for the dynamics of Bose-Einstein condensates (BECs). As a product of this similarity, we can establish the figure of a quantum fluid of light. Quantum fluids of light have been used for theoretical and experimental investigations of phenomena already studied and realised in BECs. In this thesis, we describe the mechanisms that make the conception of a quantum fluid of light possible for different experimental platforms. Furthermore, we present a study on the formation of self-bound droplets of light in hot atomic vapours, our chosen nonlinear medium, in an attempt to obtain a mapping between experimental parameters typically used in BEC experiments and those needed to observe the analogous phenomenon in atomic vapours. We investigate the static properties of the system, providing a phase diagram for the different and possible solutions for the optical regimes of interest. Finally, we systematically study droplet dynamics, focusing on the behaviour of the collective monopole excitation and the dynamic formation of these objects under realistic experimental conditions.
The propagation of light in nonlinear media is well described by a 222D nonlinear Schrödinger equation (NLSE) within the paraxial approximation, which is equivalent to the Gross-Pitaesvskii equation (GPE), the mean-field description for the dynamics of Bose-Einstein condensates (BECs). Due to this similarity, many theoretical and experimental investigations of phenomena which have already been studied and realized in BECs have been recently analysed in alternative experimental platforms such as hot atomic vapours. In this work, we study the formation of droplets of light in these media, attempting to establish a mapping between the experimental parameters normally used in BEC experiments and those needed to observe the analogous phenomenon in hot atomic vapours. We obtain the energy functional for the susceptibility of the medium in the χ(3)χ^{(3)}χ(3) , χ(3)+χ(5)χ^{(3)}+χ^{(5)}χ(3)+χ(5) and saturating regimes for a two-level atomic configuration considering the focusing (attractive) regime. We apply a Gaussian variational approach and check its predictions through numerical simulations of the NLSE for each regime. Finally, we study the real-time dynamics of the system for both the χ(3)+χ(5)χ^{(3)}+χ^{(5)}χ(3)+χ(5) and saturating nonlinearities, focusing our attention on the behaviour of the breathing mode and on the analysis of droplet formation for realistic experimental conditions.
Turbulence in the quantum (superfluid) regime, similarly to its classical counterpart, continues to attract a great deal of scientific inquiry due to the yet high number of unresolved problems. While turbulent states can be routinely created in degenerate atomic gases, there is no generic scheme to produce turbulence in fluids of light. Under paraxial propagation, light in bulk nonlinear media behaves as a two-dimensional superfluid, described by a nonlinear Schr\"odinger equation formally equivalent to the Gross-Pitaevskii model of a weakly interacting Bose gas, where photon-photon interactions are mediated by a third-order (Kerr) nonlinearity. Here we develop the theory describing the onset of a kinetic instability when two paraxial optical fluids with different streaming velocities interact via the optical nonlinearity. From numerical simulations of the nonlinear Schr\"odinger equation, we further characterize the onset of the instability and describe its saturation in the form of vortex nucleation and excitation of turbulence. The experimental observation of such effects is also discussed. The class of instabilities described here thus provide a natural route towards the investigation of quantum (superfluid) turbulence, structure formation, and out-of-equilibrium dynamics in superfluids of light.
Quantum fluids of light are the photonic counterpart of Bose gases. They currently attract increasing interest since they are versatile and highly tunable systems for probing many-body physics quantum phenomena, such as superfluidity. Superfluid flow of light has already been reported in microcavity exciton-polariton condensates but clear observation of this phenomenon in cavityless systems, that is, for propagating photon fluids, remains elusive. In this thesis, we study the hydrodynamical properties of light propagating close to resonance in hot rubidium vapors. Whereas photons in air are not interacting with each other, the situation is different in rubidium vapors, as an effective interaction between them, mediated by the atomic ensemble, appears. The light behaves therefore as a fluid flowing in the plane perpendicular to the optical axis. The primary purpose of this thesis was to show that light in those systems can behave as a superfluid. The first step toward the observation of superfluidity is to measure the dispersion relation of small amplitude density waves travelling onto the propagating photon fluid. I show that this dispersion exhibits a linear trend for small excitation wave-vectors, which is, according to the Landau criterion, a sufficient condition for guaranteeing superfluidity. I present then an all-optical defect experiment - where the photon fluid flows against an optically induced obstacle (namely, a local change of refractive index) - designed to measure the drag force cancellation at the fluid/superfluid threshold.
Bose-Einstein condensate (BEC) is a new state of matter, experimentally realized in a dilute alkali gas of weakly interacting bosons. The gas is cooled to very low temperatures, of the order of nano-Kelvin, at which point a large fraction of the atoms occupy the lowest quantum state. Under such conditions, the quantum effects become apparent on a macroscopic scale. Many fundamental ideas of quantum mechanics have been realized and proven to be true in experiments, by studying the Bose-Einstein condensates. Amongst them, the observation of macroscopic matter wave interference, the creation of vortices, dark and bright solitons etc, find special mention. The dynamics of this system in presence of an optical lattice reveals a superfluid to Mott insulator quantum phase transition. This has opened a new avenue for research on BEC and its applications. From a theoretical standpoint, the dynamics of BEC can be described by means of an effective mean-field theory. This formalism is much simpler than the many-body Schr¨odinger equation and based on a classical nonlinear evolution equation, known as Gross-Pitaevskii equation. The nonlinear nature of the GPE leads to several interesting phenomena like soliton propagation, vortices, four wave mixing etc., which are closely related to nonlinear fiber optics. The present thesis deals with nonlinear excitations and different phases of BEC and is organized as follows: after a brief introduction, in chapter two, we start with BEC in a one-dimensional shallow optical lattice, experiencing both cubic and quintic nonlinearity. A superfluid density wave, of twice the periodicity of lattice potential, is identified. This indicates matter redistribution, where atoms from neighbouring sites have been depleted leading to a density wave behaviour. Interestingly, it ceases to exist when only one of these interactions is operative. We predict the loss of superfluidity through a classical dynamical phase transition, where modulational instability leads to the loss of phase coherence. In presence of pure two-body interaction, the superfluid density shows a periodicity commensurate with the lattice potential. Apart from the superfluid state, a density wave insulating phase is also found to exist, possessing two frequency modulations commensurate with the lattice potential. A dynamical phase transition connects the superfluid phase with an insulating phase, which in turn, is connected with the density wave insulating phase. The solutions are found to be marginally stable, as per the Vakhitov-Kolokolov (VK) criterion. Chapter three describes the dynamics of the atomic-molecular Bose-Einstein condensate (AMBEC) by mean-field Gross-Pitaevskii equation (GPE), taking into account the atom-molecular interaction, as well as atom-molecule inter-conversion. The two-body atom-atom, atom-molecule and molecule-molecule interactions are analogous to the cubic nonlinearity of the standard GPE, whereas, the quadratic nonlinear term arising from the inter-conversion between atoms and molecules is identical to the scenario in strongly coupled BEC in one dimension. The presence of both weak and strong interactions adds further richness to this system. We find the molecular BEC possesses a complex dark (grey) soliton, while the atomic condensate is a bright one. The energy and momentum of this system is computed in order to see the effect of the both weak and strong interactions on Lieb mode profile and compare it with the pure atomic condensate profile. Another class of solutions exist in this system, where both atomic and molecular condensates possess bright solitons. In chapter four, we investigate the effect of a harmonic trap on the dynamics of grey solitons in Bose-Einstein condensates. It is observed that, these nonlinear excitations of the cigar-shaped Bose-Einstein condensate have strong coupling with the trap at low momenta and hence can be effectively isolated from the Bogoliubov sound modes, which respond weakly to harmonic confinement. This strong coupling with the trap also makes the grey soliton amenable for control and manipulation through trap modulation and temporal variation of the two-body interaction. We have shown that in presence of an expulsive oscillator trap, the grey soliton gets amplified, while having a compression in its width. Exact solutions are also obtained in case of the two component Bose-Einstein condensates (TBECs), where one component is a grey soliton and the other a bright one. The presence of the trap and inter-species interaction significantly affects the grey soliton dynamics. Similar to the single component, in the present case, we have shown that both grey and bright soliton can be compressed simultaneously. A detailed study of the energy and momentum of the soliton is reported, in order to find the effect of the trap on the Lieb mode. In chapter five, we study a BEC-defect complex in a quasi-one dimensional scenario, where the defect atom moves in the condensate with constant velocity. Explicit solutions of the coupled mean-field equations, describing defect-grey soliton dynamics are obtained, demonstrating the coexistence of grey soliton and a localized defect. Unlike the case of dark soliton, where the defect trapping center has vanishing superfluid density, the moving grey soliton necessarily possesses a finite superfluid component at the defect location. The presence of the defect can lower the grey soliton’s maximum velocity, as compared to the defect free case, where the maximum velocity is the sound velocity. We have also carried out the stability analysis of the obtained solutions using renormalized momentum formalism and Vakhitov-Kolokolov criteria and find that the obtained solutions are stable through both the methods. The grey soliton’s energy gets substantially modified through its interaction with the defect, opening up the possibility of its control through defect dynamics. Chapter six describes a parametrically forced Bose-Einstein condensate in the presence of a general moving optical lattice. The interaction between the atoms in the condensate and the time dependent lattice potential leads to a novel propagating superfluid matter wave, which can be controlled through chirp management. This system, when placed in a trap, accelerates and undergoes rapid nonlinear compression, controlled by the chirp. The density achieves its maximum, when the matter wave changes direction. It is also shown that this system exhibits dynamical superfluid insulator transition, where superfluidity breaks down and the condensate transits to an insulating phase. The stability has been investigated using Vakhitov-Kolokolov criterion and found that it depends on the chirp, as well as on the nature of the atom-atom interaction. The exact expression for energy is obtained and analyzed in detail to gain physical understanding of the chirp management of the sinusoidal excitations and also the dynamical phase transition.
Recent observations of droplets in dipolar and binary Bose-Einstein condensate (BEC) motivates us to study the theory of droplet formation in details. Precisely, we are interested in investigating the possibility of droplet formation in a quasi one dimensional geometry. The recent observation have concluded that the droplets are stabilized by the competition between effective mean-filed and beyond mean-field interaction. Hence, it is possible to map the effective equation of motion to a cubic-quartic nonlinear Schr\odinger equation (CQNLSE). We obtain two analytical solutions of the modified Gross-Pitaevskii equation or CQNLSE and based on their stability we investigate the parameter regime for which droplets can form. The effective potential allows us to conclude about the regions of soliton domination and self bound droplet formations.