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Fibonacci sequences and valence bond entanglement entropy in doped quantum spin ladders

Sudipto Singha Roy, Himadri Shekhar Dhar, Aditi Sen De, Ujjwal Sen

Published Dec 7, 2017• 0 citations
OpenAlex

Abstract

An interesting aspect of antiferromagnetic quantum spin ladders, with complete dimer coverings, is that the wave function can be recursively generated by estimating the number of coverings in the valence bond basis, which follow the fabled Fibonacci sequence. In this work, we show that generalized forms of such sequences can also be derived for multi-legged and doped quantum spin ladders, which allows the corresponding dimer covered state to be recursively generated. This simplifies the investigation and estimation of several important quantities in these many-body quantum systems. In particular, we show that the valence bond entanglement entropy, which is a substantial figure of merit for understanding critical behavior, can be conveniently derived for large spin ladders.

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An interesting aspect of antiferromagnetic quantum spin ladders, with complete dimer coverings, is that the wave function can be recursively generated by estimating the number of coverings in the valence bond basis, which follow the fabled Fibonacci sequence. In this work, we show that generalized forms of such sequences can also be derived for multi-legged and doped quantum spin ladders, which allows the corresponding dimer covered state to be recursively generated. This simplifies the investigation and estimation of several important quantities in these many-body quantum systems. In particular, we show that the valence bond entanglement entropy, which is a substantial figure of merit for understanding critical behavior, can be conveniently derived for large spin ladders.
Using a recursive method we construct dimer and nondimer variational ansatzs of the ground state for the two-legged ladder, and compute the number of dimer coverings, the energy density, and the spin-correlation functions. The number of dimer coverings are given by the Fibonacci numbers for the dimer-resonating-valence-bond state and their generalization for the nondimer states. Our method relies on the recurrent relations satisfied by the overlaps of the states with different lengths, which can be solved using generating functions. The recurrent-relation method is applicable to other short-range systems. Based on our results we make a conjecture about the bond amplitudes of the two-legged ladder.
We introduce for SU(2) quantum spin systems the valence bond entanglement entropy as a counting of valence bond spin singlets shared by two subsystems. For a large class of antiferromagnetic systems, it can be calculated in all dimensions with quantum Monte Carlo simulations in the valence bond basis. We show numerically that this quantity displays all features of the von Neumann entanglement entropy for several one-dimensional systems. For two-dimensional Heisenberg models, we find a strict area law for a valence bond solid state and multiplicative logarithmic corrections for the Néel phase.
We formulate an analytical recursive method to generate the wave function of doped short-range resonating valence bond (RVB) states as a tool to efficiently estimate multisite entanglement as well as other physical quantities in doped quantum spin ladders. We prove that doped RVB ladder states are always genuine multipartite entangled. Importantly, our results show that within specific doping concentration and model parameter regimes, the doped RVB state essentially characterizes the trends of genuine multiparty entanglement in the exact ground states of the Hubbard model with large on-site interactions, in the limit that yields the $t\text{\ensuremath{-}}J$ Hamiltonian.
The valence-bond structure of spin-1/2 Heisenberg antiferromagnets is closely related to quantum entanglement. We investigate measures of entanglement entropy based on transition graphs, which characterize state overlaps in the overcomplete valence-bond basis. The transition graphs can be generated using projector Monte Carlo simulations of ground states of specific Hamiltonians or using importance sampling of valence-bond configurations of amplitude-product states. We consider definitions of entanglement entropy based on the bonds or loops shared by two subsystems (bipartite entanglement). Results for the bond-based definition agree with a previously studied definition using valence-bond wave functions (instead of the transition graphs, which involve two states). For the one-dimensional Heisenberg chain, with uniform or random coupling constants, the prefactor of the logarithmic divergence with the size of the smaller subsystem agrees with exact results. For the ground state of the two-dimensional Heisenberg model (and also N\'eel-ordered amplitude-product states), there is a similar multiplicative violation of the area law. In contrast, the loop-based entropy obeys the area law in two dimensions while still violating it in one dimension---both behaviors in accord with expectations for proper measures of entanglement entropy.
We present a direct comparison of the recently proposed valence bond entanglement entropy and the von Neumann entanglement entropy on spin-1/2 Heisenberg systems using quantum Monte Carlo and density-matrix renormalization group simulations. For one-dimensional chains we show that the valence bond entropy can be either less or greater than the von Neumann entropy; hence, it cannot provide a bound on the latter. On ladder geometries, simulations with up to seven legs are sufficient to indicate that the von Neumann entropy in two dimensions obeys an area law, even though the valence bond entanglement entropy has a multiplicative logarithmic correction.
We calculate the bipartite von Neumann and second R\'enyi entanglement entropies of the ground states of spin-1/2 dimerized Heisenberg antiferromagnets on a square lattice. Two distinct dimerization patterns are considered: columnar and staggered. In both cases, we concentrate on the valence bond solid (VBS) phase and describe such a phase with the bond-operator representation. Within this formalism, the original spin Hamiltonian is mapped into an effective interacting boson model for the triplet excitations. We study the effective Hamiltonian at the harmonic approximation and determine the spectrum of the elementary triplet excitations. We then follow an analytical procedure, which is based on a modified spin-wave theory for finite systems and was originally employed to calculate the entanglement entropies of magnetic ordered phases, and calculate the entanglement entropies of the VBS ground states. In particular, we consider one-dimensional (line) subsystems within the square lattice, a choice that allows us to consider line subsystems with sizes up to ${L}^{\ensuremath{'}}\phantom{\rule{0.16em}{0ex}}=\phantom{\rule{0.16em}{0ex}}1000$. We combine such a procedure with the results of the bond-operator formalism at the harmonic level and show that, for both dimerized Heisenberg models, the entanglement entropies of the corresponding VBS ground states obey an area law as expected for gapped phases. For both columnar-dimer and staggered-dimer models, we also show that the entanglement entropies increase but they seem to not diverge as the dimerization decreases and the system approaches the N\'eel-VBS quantum phase transition. Finally, the entanglement spectra associated with the VBS ground states are presented.