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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Deterministic giant photon phase shift from a single charged quantum dot

Petros Androvitsaneas, A. B. Young, J. M. Lennon, Christian Schneider, Stefan Alexander Maier, J.J. Hinchliff, George S. Atkinson, Edmund Harbord, Martin Kamp, Sven Höfling, John Rarity, Ruth Oulton

Published Jun 1, 2017• 0 citations
Publisher

Abstract

Quantum dots (QDs) can be incorporated into solid state photonic devices such as cavities or waveguides that enhance the light-matter interaction. A near unit efficiency light-matter interaction is essential for deterministic, scalable quantum information devices [1]. In this limit, a single photon input into the device will undergo a large rotation of the polarization of the light field due to the strong interaction with the QD. In the past preliminary results have indicated that a low quality-factor (Q~290) pillar microcavity possesses a high ß-factor and that the instantaneous interactions should be deterministic and with high fidelity [2].

DOI
10.1109/cleoe-eqec.2017.8087327

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Quantum dots (QDs) can be incorporated into solid state photonic devices such as cavities or waveguides that enhance the light-matter interaction. A near unit efficiency light-matter interaction is essential for deterministic, scalable quantum information devices [1]. In this limit, a single photon input into the device will undergo a large rotation of the polarization of the light field due to the strong interaction with the QD. In the past preliminary results have indicated that a low quality-factor (Q~290) pillar microcavity possesses a high ß-factor and that the instantaneous interactions should be deterministic and with high fidelity [2].
Quantum dots have long been considered systems that could deliver a significant advantage for practical quantum information applications. Their atomic dipolelike transitions and their compatibility to be integrated into a variety of photonic structures has highlighted this fact. Here, the authors measure an unexpectedly high single-photon level phase shift (~6${}^{\ensuremath{\circ}}$), induced upon reflection from a singly negatively charged quantum dot incorporated in a low-QQQ-factor cavity (QQQ~290). This measurement provides the first evidence for a system with unit fidelity and a high efficiency in its interactions. The result opens a new road to realistic spin-photon entanglement devices, in a simple and easy to fabricate photonic structure.
The interaction of light with matter is at the heart of quantum optics, which itself enables insight into the fundamental aspects of quantum mechanics. First experimental access to this research field has been realized by coupling atoms to light. Here, the transition between discrete energy states of the atom is associated with the absorption and emission of a photon, a single quantum of the electromagnetic field. As a central aspect of quantum optics, the light-emitter interaction can be significantly enhanced by placing the emitter in optical cavity that is on resonance with the emitter. In recent years, this has led to a rapidly evolving research field known as cavity quantum electrodynamics (CQED). In CQED two different regimes are distinguished: the strong and the weak coupling regimes. In the strong coupling regime, the emitted photon is reflected from the cavity mirrors and eventually reabsorbed by the emitter. In contrast, the weak coupling regime describes the irreversible emission, where the photon leaks out of the cavity before it can be reabsorbed. Both the weak and strong coupling regimes enabled fundamental experiments for a better understanding of quantum optical phenomena. \n \n \n \nCQED grants access to the quantum world and hence offers potentially revolutionizing applications, particularly in the field of quantum information processing. A central aspect for the successful implementation of quantum applications is the system's scalability. Unfortunately, placing atoms deterministically inside a cavity remains technologically elaborate and hence minimizes the prospect of scaling a atom-CQED system. \n \nA possibility to address this issue is to implement CQED in the solid state, where sophisticated fabrication strategies allow miniaturization and scalability of the system. Particularly the development of self-assembled quantum dots (QD) in semiconductors represent a promising route. QDs can be considered as artificial atoms that mimic the atomic two-level system. These structures interact strongly with light and therefore have the potential for replacing atoms in CQED. As a central advantage, QDs are naturally trapped, which greatly simplifies the deterministic incorporation into the cavity. \n \nIn recent years, many efforts have been made to couple self-assembled QDs to microcavities. Generally, the successful implementation of CQED requires a cavity with a high quality factor Q and a low mode volume. In a majority of the approaches, the high Q/small mode volume cavities were monolithically defined around the QD, embedding the QD at a fixed position inside the cavity. Both the weak and strong coupling regimes have been reached with these systems. However, for future applications they suffer from several disadvantages. The fixed position of the QD inside the cavity minimizes the prospects for spectral tunability and spatial positioning the QD inside the cavity. Furthermore, prospects for further increasing of the cavity Q-factor and minimization of the mode volume remain limited in these systems. \n \nIn this thesis the mentioned disadvantages are addressed by developing a fully tunable miniaturized Fabry-Pérot microcavity with low mode volume. The design enables both spatial positioning of the emitter inside the cavity and spectral tunability. Successful coupling of a single QD to the microcavity is demonstrated including the strong coupling regime. Further a new approach to decrease the cavity mode volume is presented, where we demonstrate weak coupling is achieved
Solid-state quantum emitters have long been recognized as the ideal platform to realize integrated quantum photonic technologies. We demonstrate that a self-assembled negatively charged quantum dot (QD) in a low Q-factor photonic micropillar is a suitable design for deterministic polarization switching and spin-photon entanglement. We show this by measuring a shift in phase of an input single photon of at least 2π/3. As we explain in the text, this is strong experimental proof that input photons can interact with the emitter deterministically. A deterministic photon-emitter interaction is a viable and scalable means to achieve several vital functionalities such as single photon switches and entanglement gates. Our experimentally determined value is limited by mode mismatch between the input laser and the cavity, QD spectral fluctuations, and spin relaxation. When on-resonance we estimate that up to ∼80% of the collected photons couple into the cavity mode and have interacted with the QD and undergone a phase shift of π.
Semiconductor quantum dots (QDs) are promising artificial atoms for quantum information processing: they can generate single photons flying quantum bits; they show single photon sensitivity promising to develop quantum gates and the spin of a carrier in a QD can be a quantum memory. The scalability of a quantum network requires efficient interfaces between stationary and flying quantum bits. In the last few years, our group has made important progresses in this direction using cavity quantum electrodynamics. With a deterministic positioning of a single QD in a microcavity, we control the QD spontaneous emission on demand [1]. With such technique highly efficient single photon sources with brightness as large as 80% are demonstrated [2]. By minimizing the charge noise around the QD in a gated structure [3], we demonstrate the generation of fully indistinguishable photon. The source brightness is shown to exceed by one or two orders of magnitude the one of a parametric down-conversion source of same quality [4]. Symmetrically, these devices perform as excellent interfaces between a flying quantum bit and a stationary one, where coherent control of a quantum bit can be done when only few photons [5]. References [1] A. Dousse, et al. , Phys. Rev. Lett. 101, 267404 (2008) [2] O. Gazzano, et al. , Nature Communications 4, 1425 (2013) [3] A. Nowak. et al., Nature Communications 5, 3240 (2014) [4] N. Somaschi, et al. Nature Photonics 10.1038/nphoton.2016.23 (2016). [5] V. Giesz, et al., Nature Communications doi:10.1038/ncomms11986 (2016)
Though QD arrays have initially been mostly studied in an attempt to improve semiconductor lasers, much attention has been recently devoted to the revolutionary prospects opened by the unique properties of single QDs. These artificial atoms allow to mimic in solid-state systems some of the quantum optics experiments performed on atoms since the early 80’s. Recent demonstrations of coherent control experiments on QDs illustrate this fruitful analogy [10]. We will focus here our discussion on the impact of QDs on two other fields, solid-state cavity quantum electrodynamics (CQED) and the generation of quantum states of light. A single QD can be used to emit triggered single photon pulses and photon pairs, whereas its narrow emission spectrum permits to implement microcavities very efficiently to tailor its emission properties. By combining both kind of effects, it is possible to control simultaneously the number of emitted photons as well as their quantum state and to build a solid-state singlemode source of single photons (singlemode S4P) as proposed [11] and demonstrated recently by our group [12]. This novel device represents the ultimate step in a field which has been extremely active in the last 15 years, spontaneous emission (SE) control in optoelectronic devices using confined electronic and/or photonic systems [13]. Before reviewing the development of this single mode S4P, based on a single QD in a pillar microcavity, we will briefly discuss its potential applications in the field of quantum information processing and quantum communications (QIPC).