Semiconductor quantum dots (QDs) are promising artificial atoms for quantum information processing: they can generate single photons flying quantum bits; they show single photon sensitivity promising to develop quantum gates and the spin of a carrier in a QD can be a quantum memory. The scalability of a quantum network requires efficient interfaces between stationary and flying quantum bits. In the last few years, our group has made important progresses in this direction using cavity quantum electrodynamics. With a deterministic positioning of a single QD in a microcavity, we control the QD spontaneous emission on demand [1]. With such technique highly efficient single photon sources with brightness as large as 80% are demonstrated [2]. By minimizing the charge noise around the QD in a gated structure [3], we demonstrate the generation of fully indistinguishable photon. The source brightness is shown to exceed by one or two orders of magnitude the one of a parametric down-conversion source of same quality [4]. Symmetrically, these devices perform as excellent interfaces between a flying quantum bit and a stationary one, where coherent control of a quantum bit can be done when only few photons [5]. References [1] A. Dousse, et al. , Phys. Rev. Lett. 101, 267404 (2008) [2] O. Gazzano, et al. , Nature Communications 4, 1425 (2013) [3] A. Nowak. et al., Nature Communications 5, 3240 (2014) [4] N. Somaschi, et al. Nature Photonics 10.1038/nphoton.2016.23 (2016). [5] V. Giesz, et al., Nature Communications doi:10.1038/ncomms11986 (2016)
Semiconductor quantum dots (QDs) are promising artificial atoms for quantum information processing: they can generate single photons flying quantum bits; they show single photon sensitivity promising to develop quantum gates and the spin of a carrier in a QD can be a quantum memory. The scalability of a quantum network requires efficient interfaces between stationary and flying quantum bits. In the last few years, our group has made important progresses in this direction using cavity quantum electrodynamics. With a deterministic positioning of a single QD in a microcavity, we control the QD spontaneous emission on demand [1]. With such technique highly efficient single photon sources with brightness as large as 80% are demonstrated [2]. By minimizing the charge noise around the QD in a gated structure [3], we demonstrate the generation of fully indistinguishable photon. The source brightness is shown to exceed by one or two orders of magnitude the one of a parametric down-conversion source of same quality [4]. Symmetrically, these devices perform as excellent interfaces between a flying quantum bit and a stationary one, where coherent control of a quantum bit can be done when only few photons [5]. References [1] A. Dousse, et al. , Phys. Rev. Lett. 101, 267404 (2008) [2] O. Gazzano, et al. , Nature Communications 4, 1425 (2013) [3] A. Nowak. et al., Nature Communications 5, 3240 (2014) [4] N. Somaschi, et al. Nature Photonics 10.1038/nphoton.2016.23 (2016). [5] V. Giesz, et al., Nature Communications doi:10.1038/ncomms11986 (2016)
Quantum light is a key resource for the development of quantum-enhanced technologies such as secure communications, quantum networks, distributed quantum computing, metrology, etc. The development of these technologies requires light sources emitting single photons in a pure quantum state as well as efficient photon-photon gates. Such sources and gates can be obtained making use of the single-photon sensitivity of an atomic transition. We study artificial atoms in the form of semiconductor quantum dots to develop building blocks for optical quantum technologies. We use the tools of opto-electronics and nanotechnology to fabricate close to ideal atom-photon interfaces, where a single artificial atom interacts with a single mode of the optical field. We show that cavity quantum electrodynamics allows to largely isolate the artificial atoms from all sources of decoherence such as charge noise and crystal vibrations. We obtain bright solid-state sources of single photons with very high quantum purity, not only in the frequency basis, but for the first time also in the photon number basis. Finally, we have made progresses toward the development of efficient two-photon gates, with devices performing as nonlinear switches at the single-photon level. Some references: High-performances quantum light sources Somaschi et al., Nature Photonics 10, 340 (2016) Grange et al, Phys. Rev. Lett. 118, 253602 (2017) Senellart, Solomon and White, Nature Nanotechnology 12, 1026 (2017) J. C. Loredo, C. Anton, et. al, arXiv:1810.05170 Scaling-up optical quantum computing Loredo et al., Optica 3, 433 (2016) Loredo et al., Phys. Rev. Lett. 118, 130503 (2017) Toward efficient photon-photon gates Giesz et al., Nat. Comm 7, 11986 (2016) De Santis et al, Nature Nanotechnology 12, 663 (2017)
A fascinating dream in quantum information science is to build quantum computers with super-performance and quantum networks with unconditional security [1]. Quantum networks utilize static (matter) quantum bits (qubits) to store and process quantum information at local nodes, and photons as flying qubits for long-distance quantum state transmission between different nodes. To realize a quantum network, it is crucial to achieve light-matter entanglement and reversible quantum-state transfer between light and matter, i.e., the light-matter quantum interface, and the quantum repeater for large-scale quantum communications [2]. Recent experiments have shown that both electrons and holes confined in semiconductor quantum dots (QDs) have long spin relaxation time (T1e, T1h ~ ms) and long spin coherence time (T2e ~ microseconds, T2h > 100 ns). Moreover, fast spin cooling and ultra-fast spin manipulation as well as spin echoes to preserve the spin coherence have also been demonstrated. Undoubtedly these rapid progresses imply that the QD spin is a good candidate for matter qubit in quantum information processing. Furthermore, QD-based single photon sources have been also developed. Therefore, semiconductor QDs offer a good platform for solid-state quantum networking and quantum computation. Here we present two types of conditional quantum gates, i.e., the photon-spin entangling gates [3-4] using a single QD spin in a single-sided or double-sided optical microcavity. Both gates are universal and deterministic (if they are optimized). The spin-selective coherent photon-spin interaction enhanced by the cavity QED lead to giant circular birefringence, which allows us to build these gates. We will show the versatile spin-cavity systems can be applied in all aspects of quantum information science and technology, not only for large-scale quantum communication networks (solid-state quantum repeaters) [5], but also for scalable quantum computing with either photons or spins as qubits. We will also discuss other applications using these gates, such as photon-number resolving detection, quantum feed-back control, loss-resistant quantum metrology, and loophole-free Bell test [6], and other devices based on optical nonlinearity at single-photon levels in these gate structures. All these schemes are feasible with current semiconductor technology [7], and we have recently seen conditional phase shifts in uncharged QD-cavity systems [8]. References [1] H.J. Kimble, Nature (London) 453, 1023 (2008). [2] H.-J. Briegel et al., Phys. Rev. Lett. 81, 5932 (1998). [3] C.Y. Hu et al., Phys. Rev. B 78, 085307 (2008); ibid. 78, 125318 (2008). [4] C.Y. Hu et al., Phys. Rev. B 80, 205326 (2009). [5] C.Y. Hu and J.G. Rarity, Phys. Rev. B 83, 115303 (2011). [6] N. Brunner et al., Arxiv: quant-phys 1303.6522 (2013). [7] S. Reitzenstein et al., Appl. Phys. Lett. 90, 251109 (2007). [8] A.B. Young et al., Phys. Rev. A 84, 011803 (2011).
The ability to generate and manipulate light in pure quantum states is central to the development of quantum enhanced technologies, be it for optical quantum computing or for quantum secure communications. Recently, artificial atoms in the form of semiconductor quantum dots have emerged as an excellent platform to develop efficient components for optical quantum technologies. Using the tools of cavity quantum electrodynamics to harness the quantum light emission and to reduce the decoherence phenomena, single photon wavepackets with very high quantum purity can now be generated. This new generation of devices show unprecedented efficiency and allows scaling-up linear quantum optical technologies [3,4]. The high quality of the artificial atoms also allows to observe new phenomena, such as the generation of light pulses in a pure quantum superposition in the photon number basis [5], or to explore optical non-linearities at the single photon level [6] [1] N. Somaschi, et al. Nature Photonics, 10, 340 (2016) [2] P Senellart, G Solomon, A White, Nature Nanotechnology 12 (11), (2017) [3] C Antón, et al., Optica 6 (12), 1471-1477 (2019) [4] D. Istrati, arXiv 1912.04375 [5] J. C. Loredo, C. Antón, et., Nature Photonics 13 (11), 803 (2019) [6] L. De Santis, et al, Nature Nanotechnology 12, 663 (2017)
Entanglement between particles is a crucial resource in quantum information processing, an important example of which is the exploitation of entangled photons in quantum communication protocols. Among the different available sources of entangled photons, semiconductor quantum dots (QDs) excel owing to their deterministic emission properties, potential for electrical injections, and direct compatibility with semiconductor manufacturing techniques. Despite the great promises, QD-based sources are far from being ideal. In particular, such sources present several critical issues, which require the overcoming of challenges pertaining to spectral tunability, entanglement fidelity, photon indistinguishability and brightness. In this article, we will discuss the potential solutions to these problems and review the recent progress in the field.
The interaction of light with matter is at the heart of quantum optics, which itself enables insight into the fundamental aspects of quantum mechanics. First experimental access to this research field has been realized by coupling atoms to light. Here, the transition between discrete energy states of the atom is associated with the absorption and emission of a photon, a single quantum of the electromagnetic field. As a central aspect of quantum optics, the light-emitter interaction can be significantly enhanced by placing the emitter in optical cavity that is on resonance with the emitter. In recent years, this has led to a rapidly evolving research field known as cavity quantum electrodynamics (CQED). In CQED two different regimes are distinguished: the strong and the weak coupling regimes. In the strong coupling regime, the emitted photon is reflected from the cavity mirrors and eventually reabsorbed by the emitter. In contrast, the weak coupling regime describes the irreversible emission, where the photon leaks out of the cavity before it can be reabsorbed. Both the weak and strong coupling regimes enabled fundamental experiments for a better understanding of quantum optical phenomena. \n \n \n \nCQED grants access to the quantum world and hence offers potentially revolutionizing applications, particularly in the field of quantum information processing. A central aspect for the successful implementation of quantum applications is the system's scalability. Unfortunately, placing atoms deterministically inside a cavity remains technologically elaborate and hence minimizes the prospect of scaling a atom-CQED system. \n \nA possibility to address this issue is to implement CQED in the solid state, where sophisticated fabrication strategies allow miniaturization and scalability of the system. Particularly the development of self-assembled quantum dots (QD) in semiconductors represent a promising route. QDs can be considered as artificial atoms that mimic the atomic two-level system. These structures interact strongly with light and therefore have the potential for replacing atoms in CQED. As a central advantage, QDs are naturally trapped, which greatly simplifies the deterministic incorporation into the cavity. \n \nIn recent years, many efforts have been made to couple self-assembled QDs to microcavities. Generally, the successful implementation of CQED requires a cavity with a high quality factor Q and a low mode volume. In a majority of the approaches, the high Q/small mode volume cavities were monolithically defined around the QD, embedding the QD at a fixed position inside the cavity. Both the weak and strong coupling regimes have been reached with these systems. However, for future applications they suffer from several disadvantages. The fixed position of the QD inside the cavity minimizes the prospects for spectral tunability and spatial positioning the QD inside the cavity. Furthermore, prospects for further increasing of the cavity Q-factor and minimization of the mode volume remain limited in these systems. \n \nIn this thesis the mentioned disadvantages are addressed by developing a fully tunable miniaturized Fabry-Pérot microcavity with low mode volume. The design enables both spatial positioning of the emitter inside the cavity and spectral tunability. Successful coupling of a single QD to the microcavity is demonstrated including the strong coupling regime. Further a new approach to decrease the cavity mode volume is presented, where we demonstrate weak coupling is achieved
A single photon source is an enabling technology in device-independent quantum communication, quantum simulation, linear optics-based and measurement-based quantum computing. These applications employ many photons and place stringent requirements on the efficiency of single photon creation. The scaling on efficiency is typically an exponential function of the number of photons. Schemes taking full advantage of quantum superposition also depend sensitively on the coherence of the photons, i.e. their indistinguishability. \nThis thesis reports a single-photon source with a high end-to-end efficiency. We employ gated quantum dots in an open, tunable microcavity. The gating provides control of the charge and electrical tuning of the emission frequency, the high-quality material and careful design of the system ensures low noise, and the tunability of the microcavity compensates for the lack of control in quantum dot position and emission frequency. Transmission through the top mirror is the dominant escape route for photons from the microcavity, and this output is well-matched to a single-mode fiber. With this design, we can create a single photon at the output of the final optical fiber on-demand with a probability of 57% and with an average two-photon interference visibility of 97.5%. Coherence persists in trains of thousands of photons with single photon creation at a repetition rate of 1 GHz.