Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Sub-Doppler Spectroscopy by Using Sodium Nanocell

E. Mariotti, Alen Khanbekyan, Alen Khanbekyan, A. Burchianti, David G. Sarkisyan, A. S. Sarkisyan, Y. Pashayan-Leroy, Claude Leroy, K. Khanbekyan, L. Moi

Published Oct 14, 2008• 0 citations
OpenAlex

Abstract

We present for the first time the results of the sub-Doppler spectroscopy realized with a nanocell filled with a Sodium metal. The thickness L of the gap between the windows (which determines the length of the atomic vapor column) has a wedge in the vertical direction varying from 100 to 900 nm. It is demonstrated that the use of a nanocell with the thickness L=lambda/2 and L=lambda, where lambda is the wavelength of the dye laser radiation resonant with D2 line of Sodium, allows one to provide sub-Doppler spectroscopy of the Transmission and Fluorescence spectra of D2 lines of Sodium (lambda ~ 590 nm). A cw dye laser radiation with the linewidth of ~1 MHz and tunable in the range of several GHz has been used

Related papers

Sub-doppler spectroscopy of sodium vapor in an ultrathin cell

K. Khanbekyan, E. Mariotti, Alen Khanbekyan +2 more

The results obtained in a cell with a distance between windows on the order of several hundreds of nanometers (the so-called “nanocell”) are presented. The nanocell thickness L in the vertical direction changes from 100 to 900 nm. It is shown that the use of a nanocell with thickness L = λ /2, where λ is a laser wavelength resonant to the atomic transition D 2 in sodium atoms, provides sub-Doppler resolution of transmission and fluorescence spectra.

Optics and Spectroscopy•May 1, 2016•4 citations

Sub-Doppler Spectroscopy of Room-Temperature Cs Atomic Vapor in a 400-nm-Thick Nanocell

Armen D. Sargsyan, Rodolphe Momier, A. Papoyan +1 more

Abstract The sub-Doppler absorption and fluorescence spectra at the frequencies of D1- and D2-line transitions in Cs atomic vapor, enclosed in a nanocell (NC) with a thickness L ~ 400 nm, have been investigated experimentally at a near-room temperature. It is shown that a decrease in the NC temperature to 35°C causes narrowing of the absorption lines to values smaller than the Doppler width by a factor of 6, due to which the strong spectral broadening induced by laser field can be measured. The high intensity threshold for optical pumping (which limits the fluorescence intensity in centimeter-length cells) made it possible to record fluorescence spectra (using laser power of several milliwatts) at a temperature of 20°C; thus, a frequency marker of transitions in the range of D1,2 lines can be developed based on a room-temperature NC. A comparison with a widely used marker based on saturated absorption is performed.

Journal of Experimental and Theoretical Physics•Oct 1, 2021•2 citations

Magneto-optical processes in atomic vapor cells with radiation wavelength-scale thickness

A. Papoyan, David G. Sarkisyan

Sub-Doppler nature of atomic spectra in alkali metal vapor cells of nanometric thickness L (nanocells) allows one to study peculiarities of magneto-optical processes, which occur in a magnetic field for the case when L is of the order of λ (λ is a laser resonant wavelength). We particularly address the issues of practical implementation of the studied processes. The following results are presented. i) A "λ-Zeeman technique" exploiting velocity-selective optical pumping resonances in L = λ Rb cell placed in a B-field, which allows direct determination frequency shifts and modification of transition probabilities of individual Zeeman transitions in magnetic field and is applicable for development of wide-range (~ 0.1 - 1000 mT) optical magnetometers and tunable frequency reference. ii) A technique for locking the laser radiation frequency, B-field-tunable in ~ 500 MHz range, which is based on selective reflection of a circularly-polarized laser beam from Rb vapor cell with thickness L ≈ λ/2.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Dec 22, 2008•1 citation

Broadening and Shift of the D1 and D2 Lines of Rb Atoms by Neon: Resolving Hyperfine Components in a Half-Wave Cell Using Double Differentiation with Respect to Frequency

Armen D. Sargsyan, T. A. Vartanyan, David G. Sarkisyan

Abstract A cell with a submicron thickness was used to measure the broadening and shift of the D1 and D2 lines of Rb atoms by neon. The resolution of hypefine components is achieved by a combination of two techniques. First, the Rb vapor column thickness in the direction of propagation of the laser radiation was chosen equal to half of its wavelength λ under conditions of resonance with the atomic transition frequency. For rubidium atoms λ/2 ~ 400 nm. At a nanocell thickness L ~ λ/2, in the transmission spectrum A(ν), the spectral lines of atomic transitions are narrowed due to the exclusion of Doppler broadening. Second, further narrowing of the detected signals was achieved by the double differentiation of the transmission spectrum, A''(ν). The transmission spectra of pure rubidium vapor and rubidium vapor with the addition of neon have been measured at different pressures. The measured values of the shift coefficients of the D1 and D2 lines of rubidium in the presence of Ne were –1.1 ± 0.2 MHz/Torr and –2.1 ± 0.2 MHz/Torr, respectively. The broadening coefficients of the D1 and D2 lines coincide and are equal to 10 ± 1 MHz/Torr. Due to its high spectral resolution, this technique allows separate measurements for each individual transition.

Optics and Spectroscopy•Nov 1, 2021•6 citations

Dependence of the cesium absorption D1 linewidth on the thickness of atomic vapor column

Armen D. Sargsyan, David G. Sarkisyan, Y. Pashayan-Leroy +3 more

A new nanocell has been elaborated, where the thickness of the atomic vapor column varies smoothly in the range L = 350–5100 nm. The cell allows studying the behavior of the resonance absorption at the D 1 line of cesium atoms by varying the thickness from L = λ / 2 to L = 5 λ with the step λ / 2 (λ being the resonant wavelength of the laser, 894 nm) and the laser intensity. It is shown that at low laser intensities a narrowing of the resonance absorption spectrum is observed for L = (2 n + 1)λ/2 (with an integer n ) up to L = (7/2)λ, whereas for L = n λ the spectrum broadens. The developed theoretical model well describes the experiment.

Journal of Contemporary Physics (Armenian Academy of Sciences)•Jan 29, 2008•9 citations

Study of atomic spectral lines in a magnetic field with use of a nanocell with the thickness L = λ

T. Varzhapetyan, G. Hakhumyan, V. V. Babushkin +3 more

We propose a technique which we call “ L = λ Zeeman technique” (LZT) for investigation of the transitions between the Zeeman sublevels of the hfs structure of alkali metal atoms in external magnetic fields. The technique is based on the employment of a nanocell with the thickness of the Rb atom vapor column equal to the wavelength of the laser radiation, 780 nm, resonant with the atomic rubidium D 2 transition. At the laser intensities of about 1 mW/cm 2 in the transmission spectrum of the nanocell narrow (∼ 30 MHz) resonant peaks of reduced absorption appear localized exactly on the atomic transitions. In magnetic fields these peaks are split and their amplitudes and frequency positions depend on the magnetic field strength. The theoretical model well describes the experimental results.

Journal of Contemporary Physics (Armenian Academy of Sciences)•Dec 1, 2007•10 citations
We present for the first time the results of the sub-Doppler spectroscopy realized with a nanocell filled with a Sodium metal. The thickness L of the gap between the windows (which determines the length of the atomic vapor column) has a wedge in the vertical direction varying from 100 to 900 nm. It is demonstrated that the use of a nanocell with the thickness L=lambda/2 and L=lambda, where lambda is the wavelength of the dye laser radiation resonant with D2 line of Sodium, allows one to provide sub-Doppler spectroscopy of the Transmission and Fluorescence spectra of D2 lines of Sodium (lambda ~ 590 nm). A cw dye laser radiation with the linewidth of ~1 MHz and tunable in the range of several GHz has been used
Abstract The sub-Doppler absorption and fluorescence spectra at the frequencies of D1- and D2-line transitions in Cs atomic vapor, enclosed in a nanocell (NC) with a thickness L ~ 400 nm, have been investigated experimentally at a near-room temperature. It is shown that a decrease in the NC temperature to 35°C causes narrowing of the absorption lines to values smaller than the Doppler width by a factor of 6, due to which the strong spectral broadening induced by laser field can be measured. The high intensity threshold for optical pumping (which limits the fluorescence intensity in centimeter-length cells) made it possible to record fluorescence spectra (using laser power of several milliwatts) at a temperature of 20°C; thus, a frequency marker of transitions in the range of D1,2 lines can be developed based on a room-temperature NC. A comparison with a widely used marker based on saturated absorption is performed.
Sub-Doppler nature of atomic spectra in alkali metal vapor cells of nanometric thickness L (nanocells) allows one to study peculiarities of magneto-optical processes, which occur in a magnetic field for the case when L is of the order of λ (λ is a laser resonant wavelength). We particularly address the issues of practical implementation of the studied processes. The following results are presented. i) A "λ-Zeeman technique" exploiting velocity-selective optical pumping resonances in L = λ Rb cell placed in a B-field, which allows direct determination frequency shifts and modification of transition probabilities of individual Zeeman transitions in magnetic field and is applicable for development of wide-range (~ 0.1 - 1000 mT) optical magnetometers and tunable frequency reference. ii) A technique for locking the laser radiation frequency, B-field-tunable in ~ 500 MHz range, which is based on selective reflection of a circularly-polarized laser beam from Rb vapor cell with thickness L ≈ λ/2.
Abstract A cell with a submicron thickness was used to measure the broadening and shift of the D1 and D2 lines of Rb atoms by neon. The resolution of hypefine components is achieved by a combination of two techniques. First, the Rb vapor column thickness in the direction of propagation of the laser radiation was chosen equal to half of its wavelength λ under conditions of resonance with the atomic transition frequency. For rubidium atoms λ/2 ~ 400 nm. At a nanocell thickness L ~ λ/2, in the transmission spectrum A(ν), the spectral lines of atomic transitions are narrowed due to the exclusion of Doppler broadening. Second, further narrowing of the detected signals was achieved by the double differentiation of the transmission spectrum, A''(ν). The transmission spectra of pure rubidium vapor and rubidium vapor with the addition of neon have been measured at different pressures. The measured values of the shift coefficients of the D1 and D2 lines of rubidium in the presence of Ne were –1.1 ± 0.2 MHz/Torr and –2.1 ± 0.2 MHz/Torr, respectively. The broadening coefficients of the D1 and D2 lines coincide and are equal to 10 ± 1 MHz/Torr. Due to its high spectral resolution, this technique allows separate measurements for each individual transition.
A new nanocell has been elaborated, where the thickness of the atomic vapor column varies smoothly in the range L = 350–5100 nm. The cell allows studying the behavior of the resonance absorption at the D 1 line of cesium atoms by varying the thickness from L = λ / 2 to L = 5 λ with the step λ / 2 (λ being the resonant wavelength of the laser, 894 nm) and the laser intensity. It is shown that at low laser intensities a narrowing of the resonance absorption spectrum is observed for L = (2 n + 1)λ/2 (with an integer n ) up to L = (7/2)λ, whereas for L = n λ the spectrum broadens. The developed theoretical model well describes the experiment.
We propose a technique which we call “ L = λ Zeeman technique” (LZT) for investigation of the transitions between the Zeeman sublevels of the hfs structure of alkali metal atoms in external magnetic fields. The technique is based on the employment of a nanocell with the thickness of the Rb atom vapor column equal to the wavelength of the laser radiation, 780 nm, resonant with the atomic rubidium D 2 transition. At the laser intensities of about 1 mW/cm 2 in the transmission spectrum of the nanocell narrow (∼ 30 MHz) resonant peaks of reduced absorption appear localized exactly on the atomic transitions. In magnetic fields these peaks are split and their amplitudes and frequency positions depend on the magnetic field strength. The theoretical model well describes the experimental results.