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Optics and Spectroscopy

Sub-doppler spectroscopy of sodium vapor in an ultrathin cell

K. Khanbekyan, E. Mariotti, Alen Khanbekyan, L. Moi, Aleksandr Khanbekyan

Published May 1, 2016• 4 citations
Publisher

Abstract

The results obtained in a cell with a distance between windows on the order of several hundreds of nanometers (the so-called “nanocell”) are presented. The nanocell thickness L in the vertical direction changes from 100 to 900 nm. It is shown that the use of a nanocell with thickness L = λ /2, where λ is a laser wavelength resonant to the atomic transition D 2 in sodium atoms, provides sub-Doppler resolution of transmission and fluorescence spectra.

DOI
10.1134/s0030400x16050143

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Journal of Experimental and Theoretical Physics Letters•Aug 1, 2016•25 citations
The results obtained in a cell with a distance between windows on the order of several hundreds of nanometers (the so-called “nanocell”) are presented. The nanocell thickness L in the vertical direction changes from 100 to 900 nm. It is shown that the use of a nanocell with thickness L = λ /2, where λ is a laser wavelength resonant to the atomic transition D 2 in sodium atoms, provides sub-Doppler resolution of transmission and fluorescence spectra.
We present for the first time the results of the sub-Doppler spectroscopy realized with a nanocell filled with a Sodium metal. The thickness L of the gap between the windows (which determines the length of the atomic vapor column) has a wedge in the vertical direction varying from 100 to 900 nm. It is demonstrated that the use of a nanocell with the thickness L=lambda/2 and L=lambda, where lambda is the wavelength of the dye laser radiation resonant with D2 line of Sodium, allows one to provide sub-Doppler spectroscopy of the Transmission and Fluorescence spectra of D2 lines of Sodium (lambda ~ 590 nm). A cw dye laser radiation with the linewidth of ~1 MHz and tunable in the range of several GHz has been used
Abstract The sub-Doppler absorption and fluorescence spectra at the frequencies of D1- and D2-line transitions in Cs atomic vapor, enclosed in a nanocell (NC) with a thickness L ~ 400 nm, have been investigated experimentally at a near-room temperature. It is shown that a decrease in the NC temperature to 35°C causes narrowing of the absorption lines to values smaller than the Doppler width by a factor of 6, due to which the strong spectral broadening induced by laser field can be measured. The high intensity threshold for optical pumping (which limits the fluorescence intensity in centimeter-length cells) made it possible to record fluorescence spectra (using laser power of several milliwatts) at a temperature of 20°C; thus, a frequency marker of transitions in the range of D1,2 lines can be developed based on a room-temperature NC. A comparison with a widely used marker based on saturated absorption is performed.
On the basis of density matrix equations, we theoretically investigated narrow sub-Doppler resonances in the spectral distribution of a number of atomic particles (atoms or molecules) optically excited in a metastable state in an ultrathin gas cell with the inner thickness less than or of the order of the wavelength λ ≤ 1 μm of the monochromatic light wave incident in the normal direction. Essential dependence of these resonances (on the center of the optical transition) was analyzed versus the inner thickness and transversal size of such a gas cell and also versus the intensity of the incident wave. Investigated resonances may be applied as references in high-accuracy optical frequency standards and for high precision measurements.
Sub-Doppler nature of atomic spectra in alkali metal vapor cells of nanometric thickness L (nanocells) allows one to study peculiarities of magneto-optical processes, which occur in a magnetic field for the case when L is of the order of λ (λ is a laser resonant wavelength). We particularly address the issues of practical implementation of the studied processes. The following results are presented. i) A "λ-Zeeman technique" exploiting velocity-selective optical pumping resonances in L = λ Rb cell placed in a B-field, which allows direct determination frequency shifts and modification of transition probabilities of individual Zeeman transitions in magnetic field and is applicable for development of wide-range (~ 0.1 - 1000 mT) optical magnetometers and tunable frequency reference. ii) A technique for locking the laser radiation frequency, B-field-tunable in ~ 500 MHz range, which is based on selective reflection of a circularly-polarized laser beam from Rb vapor cell with thickness L ≈ λ/2.
Theoretical studies have been conducted on sub-Doppler resonances of fluorescence of an ultrathin gas layer in a cell with an internal weakness less than or on the order of the wavelength of a monochromatic light beam incident on the given cell in the normal direction. The features of these resonances are analyzed both under steady-state action of the incident radiation and immediately following abrupt termination of its action. The essential dependence of these resonances (at the centers of optical transitions with sufficiently small radiation spectral linewidths) on the transversal dimensions of the gas cell (using the example of a rectangular parallelepiped shape). The main focus is on analyzing the linear optics case when the examined resonances are narrowest. The possibility is noted of using such sub-Doppler fluorescence resonances in nanometer gas cells as references for optical frequency standards.
The features of the effect of selective reflection from rubidium vapor in a nanocell with the thickness L ≈ λ/2 and L ≈ λ/4, where λ = 795 nm is the wavelength of laser radiation resonant with the Rb D 1 line, are studied. It is shown that, because of the behavior of the nanocell as a low-Q-factor Fabry–Pérot etalon, the sign of the derivative of the selective reflection spectra changes near L ≈ λ/2 from negative at L > λ/2 to positive at L < λ/2. The simplicity of the experimental implementation, large amplitude, and sub-Doppler width (40MHz) of a detected signal at an atomic transition frequency are appropriate for applications in metrology and magnetometry. In particular, selective reflection from the nanocell is a convenient frequency marker of atomic transitions; in this case, the amplitudes of peaks are proportional to the transition probabilities. The remote optical monitoring of a magnetic field with a spatial resolution L = λ/4 ≈ 199 of nm is possible on the basis of the splitting of selective reflection peaks in a strong magnetic field (up to 3 kG). A theoretical model describes well the experimental results.