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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Magneto-optical processes in atomic vapor cells with radiation wavelength-scale thickness

A. Papoyan, David G. Sarkisyan

Published Dec 22, 2008• 1 citation
Publisher

Abstract

Sub-Doppler nature of atomic spectra in alkali metal vapor cells of nanometric thickness L (nanocells) allows one to study peculiarities of magneto-optical processes, which occur in a magnetic field for the case when L is of the order of λ (λ is a laser resonant wavelength). We particularly address the issues of practical implementation of the studied processes. The following results are presented. i) A "λ-Zeeman technique" exploiting velocity-selective optical pumping resonances in L = λ Rb cell placed in a B-field, which allows direct determination frequency shifts and modification of transition probabilities of individual Zeeman transitions in magnetic field and is applicable for development of wide-range (~ 0.1 - 1000 mT) optical magnetometers and tunable frequency reference. ii) A technique for locking the laser radiation frequency, B-field-tunable in ~ 500 MHz range, which is based on selective reflection of a circularly-polarized laser beam from Rb vapor cell with thickness L ≈ λ/2.

DOI
10.1117/12.822451

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•Jul 5, 2010•0 citations
Sub-Doppler nature of atomic spectra in alkali metal vapor cells of nanometric thickness L (nanocells) allows one to study peculiarities of magneto-optical processes, which occur in a magnetic field for the case when L is of the order of λ (λ is a laser resonant wavelength). We particularly address the issues of practical implementation of the studied processes. The following results are presented. i) A "λ-Zeeman technique" exploiting velocity-selective optical pumping resonances in L = λ Rb cell placed in a B-field, which allows direct determination frequency shifts and modification of transition probabilities of individual Zeeman transitions in magnetic field and is applicable for development of wide-range (~ 0.1 - 1000 mT) optical magnetometers and tunable frequency reference. ii) A technique for locking the laser radiation frequency, B-field-tunable in ~ 500 MHz range, which is based on selective reflection of a circularly-polarized laser beam from Rb vapor cell with thickness L ≈ λ/2.
We describe the so-called "Lambda-Zeeman method" to investigate individual hyperfine transitions between Zeeman sublevels of atoms in an external magnetic field of 0.1 mT - 0.25 T. Atoms are confined in a nanocell with thickness L = Lambda, where Lambda is the resonant wavelength (794 nm or 780 nm for D1 or D2 line of Rb). Narrow resonances in the transmission spectrum of the nanocell are split into several components in a magnetic field; their frequency positions and probabilities depend on the B-field. Possible applications are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references.
The features of the effect of selective reflection from rubidium vapor in a nanocell with the thickness L ≈ λ/2 and L ≈ λ/4, where λ = 795 nm is the wavelength of laser radiation resonant with the Rb D 1 line, are studied. It is shown that, because of the behavior of the nanocell as a low-Q-factor Fabry–Pérot etalon, the sign of the derivative of the selective reflection spectra changes near L ≈ λ/2 from negative at L > λ/2 to positive at L < λ/2. The simplicity of the experimental implementation, large amplitude, and sub-Doppler width (40MHz) of a detected signal at an atomic transition frequency are appropriate for applications in metrology and magnetometry. In particular, selective reflection from the nanocell is a convenient frequency marker of atomic transitions; in this case, the amplitudes of peaks are proportional to the transition probabilities. The remote optical monitoring of a magnetic field with a spatial resolution L = λ/4 ≈ 199 of nm is possible on the basis of the splitting of selective reflection peaks in a strong magnetic field (up to 3 kG). A theoretical model describes well the experimental results.
We describe the so-called λ-Zeeman method to investigate individual hyperfine transitions between Zeeman sublevels of atoms in an external magnetic field of 0.1mT–0.25T. Atoms are confined in a nanocell with thickness L=λ, where λ is the resonant wavelength (794 or 780nm for D1 or D2 line, respectively, of Rb). Narrow resonances in the transmission spectrum of the nanocell are split into several components in a magnetic field; their frequency positions and transition probabilities depend on the B field. Possible applications are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references.
We propose a technique which we call “ L = λ Zeeman technique” (LZT) for investigation of the transitions between the Zeeman sublevels of the hfs structure of alkali metal atoms in external magnetic fields. The technique is based on the employment of a nanocell with the thickness of the Rb atom vapor column equal to the wavelength of the laser radiation, 780 nm, resonant with the atomic rubidium D 2 transition. At the laser intensities of about 1 mW/cm 2 in the transmission spectrum of the nanocell narrow (∼ 30 MHz) resonant peaks of reduced absorption appear localized exactly on the atomic transitions. In magnetic fields these peaks are split and their amplitudes and frequency positions depend on the magnetic field strength. The theoretical model well describes the experimental results.
Recently unique extremely thin cells (ETC) containing atomic vapour of alkali metals with the column thickness L of an order and much less than optical light wavelength λ have been developed. It has been demonstrated that these ETC are a very promising tool for a fundamental study of atom-light, atom-atom, atom-surface and atom-external magnetic field interactions. Particularly, a dramatically different behaviour of resonant absorption, fluorescence and resonant magneto-optical processes compared to that obtained with the help of cm-long ordinary cells has been demonstrated. Possible applications based on ETC are described, such as magnetometers with nanometric spatial resolution and tunable atomic frequency references. For the study of buffer gas influence, a multi-region cell (MRC) has been developed. MRC consists of an ETC cell having a wedged thickness of the gap between the windows that allows one to form atomic vapour column thickness in the range of 0.1 ÷ 4 μm. The ETC is connected through a sapphire tube with a 1cm-long sapphire tube having sapphire windows. The 1cm-long cell has a sapphire side-arm containing Rb metal. MRC's are filled with 6 Torr and 20 Torr Neon gas, thus there is Rb vapour and buffer gas inside the MRC. The construction of the MRC allows one to compare absorption and fluorescence processes simultaneously in the case of the ETC use as well as in the case of 1cm-long ordinary cell use. The comparison of the resonant absorption and fluorescence in the extremely thin cell (ETC) filled with pure Rb with another one filled with Rb and Neon gas with the pressures of 6 Torr and 20 Torr is provided. The effect of the collapse and revival of Dicke-type narrowing is still observable for the thicknesses L = λ/2, and L = λ, with λ being the resonant laser wavelength 794 nm (D1 line of Rb), i.e. the spectra of the resonant absorption and fluorescence demonstrate strong sub-Doppler narrowing for the thickness L = λ/2 and broadening for the thickness L = λ. It is important to note that in an ordinary Rb cell with the thickness L in the range of 1mm - 10 cm filled with buffer gas, with the pressure higher than 1 Torr, in the well-known Saturation Absorption scheme, any sub-Doppler features are absent. For L = λ the so called velocity selective optical pumping/saturating resonance (VSOP) located at the atomic transition is still observable when Ne pressure is 6 Torr, while the linewidth is increased by 4 times in comparison with that obtained in a pure Rb ETC. It is also demonstrated that the use of the fluorescence spectra at L = λ/2 allows one to use ETC for the buffer gas pressure measurements. Comparison with the theory will be presented.
The energy levels of atoms placed in an external magnetic field undergo frequency shifts and changes in their transition probabilities. It is demonstrated that using fluorescence spectra from a submicron thin vapour cell (STC) with the thickness L = λ/2, it is possible to efficiently study the above mentioned changes (“half-λ Zeeman technique” (HLZT)). The circularly polarized beam of extended-cavity diode laser (λ = 794 nm, laser bandwidth γL < 1 MHz) resonant with 87Rb D1 transition, after passing through Faraday isolator is directed onto the Rb STC with the thickness L = λ/2. The temperature of the STC is 120 °C, corresponding to N ~ 1013 atom/cm3. STC was provided by a special oven with 3 openings: 2 inlets for laser beam passage, and one orthogonal inlet for side fluorescence detection. This geometry allows simultaneous recording of fluorescence and transmission spectra. STC with the oven is placed between two strong permanent ring magnets and by changing the distance between them it is possible to form a strong magnetic field up to 4500 G. In [1], “λ-Zeeman technique” (LZT) is shown to be efficient to study individual transitions between the Zeeman sublevels of hyperfine levels in an external magnetic field up to 2400 G. LZT uses STC with thickness L = λ, where λ is 794 nm (780 nm) for D1 line (D2 line) of Rb. Narrow velocity selective optical pumping/saturation (VSOP) resonances in the transmission spectrum of the STC are split into several components in the magnetic field; their frequency positions and probabilities depend on the B-field. We present comparison of HLZT and LZT in a wide region of magnetic fields up to 4500 G. We present the fluorescence spectrum for L = λ/2 and the transmission spectrum for L = λ. The VSOP resonances in the LZT-curve are narrower meanwhile the advantage of HLZT is that the fluorescence appears on a flat background. Applications such as magnetometer with high spatial resolution and the theoretical model describing well the experiment will be presented.