Entanglement is an established resource in quantum information processing, and there is a clear imperative to study many-body systems both in quantum technology applications and for probing fundamental physical laws. Ion trap cavity quantum electrodynamics is a highly promising platform for research. Prerequisites are the controlled coupling of many ions to the cavity field along with the ability to initialize the quantum states and drive coherent transitions between them. A coaxial ion trap and high finesse cavity system has been shown to couple strings of up to five ions to the cavity mode with nearly optimal coupling strength thanks to precise control over their positions in the standing wave and their mutual Coulomb interaction. The predictive power of the theoretical model demonstrates that the scheme can be extended to more ions or to higher coupling regimes. In a separate experiment it has been demonstrated that a quantum state can be initialized, before coherently transferring the population to a qubit state through the cavity interaction. The emission of polarized photons in the cavity mode has been measured, taking the system closer to the generation of cluster states for quantum information research and fundamental studies in many-body entanglement. Building on the aforementioned work, an infrastructure has been put in place for the direct observation of vacuum Rabi oscillations between a single ion and the cavity. In this scheme, the contribution to the dynamics from the dominant incoherent channel is minimized through post-selection of the data. As a quantum system coupled to a reservoir with memory, it will provide experimental constraints on theoretical work in the field of non-Markovian dynamics.
Entanglement is an established resource in quantum information processing, and there is a clear imperative to study many-body systems both in quantum technology applications and for probing fundamental physical laws. Ion trap cavity quantum electrodynamics is a highly promising platform for research. Prerequisites are the controlled coupling of many ions to the cavity field along with the ability to initialize the quantum states and drive coherent transitions between them. A coaxial ion trap and high finesse cavity system has been shown to couple strings of up to five ions to the cavity mode with nearly optimal coupling strength thanks to precise control over their positions in the standing wave and their mutual Coulomb interaction. The predictive power of the theoretical model demonstrates that the scheme can be extended to more ions or to higher coupling regimes. In a separate experiment it has been demonstrated that a quantum state can be initialized, before coherently transferring the population to a qubit state through the cavity interaction. The emission of polarized photons in the cavity mode has been measured, taking the system closer to the generation of cluster states for quantum information research and fundamental studies in many-body entanglement. Building on the aforementioned work, an infrastructure has been put in place for the direct observation of vacuum Rabi oscillations between a single ion and the cavity. In this scheme, the contribution to the dynamics from the dominant incoherent channel is minimized through post-selection of the data. As a quantum system coupled to a reservoir with memory, it will provide experimental constraints on theoretical work in the field of non-Markovian dynamics.
Recent technological advances in cavity quantum electrodynamics (CQED) are paving the way to utilize multiple quantum emitters confined in a single optical cavity. In such systems, it is crucially important to control the quantum mechanical coupling of individual emitters to the cavity mode. In this regard, combining ion trap technologies with CQED provides a particularly promising approach due to the well-established motional control over trapped ions. Here, we experimentally demonstrate coupling of up to five trapped ions in a string to a high-finesse optical cavity. By changing the axial position and spacing of the ions in a fully deterministic manner, we systematically characterize their coupling to the cavity mode through visibility measurements of the cavity emission. In good agreement with the theoretical model, the results demonstrate that the geometrical configuration of multiple trapped ions can be manipulated to obtain optimal cavity coupling. Our system presents a new ground for exploring CQED with multiple quantum emitters, enabled by the highly controllable collective light-matter interaction.
Quantum networking is an established and growing field of research, with applications in many other fields of quantum technology, as well as fundamental research in quantum mechanics. A quantum network consists of multiple quantum devices that can interchange quantum information or be entangled with each other. Trapped ions coupled to optical cavities are among the most promising platforms in quantum technology broadly and networking specifically, with the ability to initialise and store quantum states in the ions and, via the cavity, transfer those states onto photons, which can interact with distant systems. This thesis describes two experiments using an ion trap with integrated high finesse optical cavity as a source of single photons. In the first, the photons were converted to a standard telecommunications wavelength through quantum frequency conversion and transmitted over 10 km of optical fibre. The attenuation experienced by the photons in optical fibre without frequency conversion would make transmission over such a long distance impractical. The converted photons were shown to maintain their nonclassical statistics, meaning such a system could be used to create quantum networks over long distances. A novel scheme for producing single photons from the ion-cavity system was demonstrated. This scheme significantly reduces the impact of decoherence in the system compared to commonly used schemes through selection of the initial state of the ion. This scheme may be directly applied to ion-photon entanglement and would lead to improved fidelity in ion-ion entanglement or state transfer. Both experiments represent significant steps towards the building of quantum networks based on ions coupled to optical cavities. They lay the groundwork for future experiments using the same system to entangle ions with photons and eventually with ions in other traps.
Trapped ions are a promising platform for local quantum information processing. In order to distribute this quantum information over long distances, we can take advantage of optical cavities, which ofier a coherent interface between matter and light, enabling the transfer of quantum information from stationary qubits such as ions onto photons. We demonstrate such an interface by coupling trapped ions to a cavity and have recently shown that a quantum state can be faithfully transferred from a single ion onto a single photon. In particular, this transfer can be improved by taking advantage of a collective effect between multiple ions, namely, superradiant emission into the cavity. In this proof-of-principle experiment, we tune the phase of a two-ion entangled state between sub- and superradiance. The superradiant coupling is then used to enhance the transfer of quantum information onto a photon from a logical qubit encoded in the two ions. Finally, prospects for linking together distant ions in cavities via a quantum network are discussed. Toward this goal, we outline a fiber-based ion-cavity experiment which allows access to the single-ion strong-coupling regime.
Cavity quantum electrodynamics (QED) in the strong-coupling regime provides the opportunity to monitor and control the dynamics of a simple quantum system. A single Cesium atom interacts strongly with single-photon fields in the mode of a high-finesse optical cavity. When the resulting coherent coupling rate dominates dissipation in the system, strong coupling is realized and the system displays distinctively quantum behavior. The coupling between atomic internal states and the quantized cavity field allows for diverse protocols in quantum state preparation, quantum communication, and quantum logic. However, the atom's external or motional state must also be taken into account. My research develops cavity QED in the limit where the coherent atom-field coupling dominates the atomic kinetic energy and thus significantly affects the atomic center-of-mass motion. In this regime, the interaction of the atom with the cavity field provides both a means of controlling atomic motion and a signal for detecting that motion in real time with high signal-to-noise. The sensing capability of the ``atom-cavity microscope" is exploited to trap single atoms with single-photon fields and to monitor their orbits in real time as they are bound in the cavity. Such real-time position sensing is the basis for a detailed strategy and ongoing experiment to actively stabilize select aspects of an atom's motion within the cavity. As the cavity-enabled position measurement approaches the standard quantum limit, this work begins to realize a quantum servo for atomic position and to address questions of optimal state estimation and state preparation. In combination with other progress in cavity QED, it furthers the goal of controlled atom-field interactions for quantum information science.
The research undertaken unites two distinct areas of quantum information processing: single ions stored in radio-frequency traps and single photons in optical fibres. Strings of ions are presently the most successful implementation of quantum computing, with elementary quantum algorithm and quantum simulations realised. The principal challenge in the field is to enhance the quantum processing power by scaling up current devices to larger systems. We pursue one of the most promising strategies: distributed quantum computation in which multiple small-scale ion processors are interlinked by exchanging photonic quantum bits via optical fibres. This requires a coherent quantum interface between ions and photons, mapping ionic to photonic quantum states and vice versa. To maximise fidelity and the success rate of the scheme, the interaction of ions and photons must take place in a microscopic optical cavity with high finesse. To this end, single 40Ca+ were trapped in a radio-frequency ion trap whose trapping electrodes are hollow cylinders. Optical fibres with mirrors machined on the facets are inserted into the electrodes to form a Fabry-Pérot cavity. Because the fibres are shielded by the electrodes the detrimental distortion of the trapping field due to their presence is suppressed and ions can be trapped for several hours. 40Ca+ has a -type energy level scheme wherein the ion is cooled on the 42P1/2 ? 42S1/2 transition and the cavity is tuned to the 42P1/2 ? 32D3/2 transition. This thesis reports the successful coupling of single ions to a high finesse optical fibre based cavity, with coupling strength g = 2p · 4:6 MHz. The cavity has length 367 µm, finesse of 40,000 and linewidth 2k = 2p · 9:4 MHz. In this coupling regime, the enhancement of the ion's emission rate through the Purcell effect was observed. Further, anti-correlation was observed in the emission rates between the P1/2 ? D3/2 and P1/2 ? S1/2 transitions with an effective emission rate suppression of up to 60% in the latter transition. The built system offers greater promises. Once the position in the cavity mode has been optimised we expect to reach the long-sought after strong coupling regime with (g, k, y) = 2p · (12:2; 4:7; 11:2) MHz.
Long-range transport of quantum information across a network is most readily achieved through the use of photons as the information carriers. The nodes of such a quantum network are most naturally a quantum memory or information processor, which typically do not rely upon photonic qubits. Realizing a large-scale distributed quantum network therefore requires an efficient interface between the two physical manifestations of the quantum information. The most promising platform for realizing a quantum computer is the manipulation of trapped atomic ions, as this system has demonstrated all the fundamental requirements to realize a quantum computer. Additionally, trapped ions posses long coherence times necessary for quantum memories. The interface between atomic and photonic qubits relies on a high photon emission rate into the collected solid angle. Most methods of photon collection for quantum networks use a high numerical aperture microscope objective, which only collects on the order of 1% of all the emitted photons. This results in a small probability of successfully linking two quantum nodes. In this work, I present the design, simulation, and implementation of a trapped ion cavity QED system capable of improving the photon collection efficiency. A single ytterbium ion is coupled to a high-finesse optical cavity. The photon scatter rate into the cavity mode is enhanced by a factor of 130 over the free-space scatter rate into the cavity solid angle. This represents the first step towards realizing a protocol to entangle the polarization of an emitted photon to the Zeeman sublevels of the ion with high photon collection efficiency. Simulations of the experimental system indicate that with an optical cavity up to 4% of the light emitted by the ion can be collected.