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Acta Physica Sinica

GENERATION OF PHASE CONJUGATED BACKWARD WAVE BY DEGENERATE FOUR-WAVE MIXING IN CHLOROPHYLL SOLUTION

Cunkai Wu, FAN JUN-YIN, WANG ZHI-YING, 中国科学院上海光学精密机械研究所

Published Jan 1, 1980• 2 citations
Publisher

Abstract

In this paper, the first experiment of generating the phase conjugated backward wave by degenerate four-wave mixing in chlorophyll solution is reported. It is demonstrated that the efficiency converting the incident object beam into the phase conjugated backward wave with interaction length 5mm long has approached 22%. This is a four-level system having a high conversion efficiency. The intensity of the complex conjugate reflected wave is proportional to that of the incident object wave as we kept the pumping beam intensity constant. The phase conjugate behaviours of the backward wave have been demonstrated. By using the phase conjugate nature of the reflected wave, good quality reconstructed images of a grid are obtained through a phase distorting media.

DOI
10.7498/aps.29.305

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•Jul 18, 1988•0 citations
In this paper, the first experiment of generating the phase conjugated backward wave by degenerate four-wave mixing in chlorophyll solution is reported. It is demonstrated that the efficiency converting the incident object beam into the phase conjugated backward wave with interaction length 5mm long has approached 22%. This is a four-level system having a high conversion efficiency. The intensity of the complex conjugate reflected wave is proportional to that of the incident object wave as we kept the pumping beam intensity constant. The phase conjugate behaviours of the backward wave have been demonstrated. By using the phase conjugate nature of the reflected wave, good quality reconstructed images of a grid are obtained through a phase distorting media.
Phase conjugation of backward-and forward-wave produced by degenerate four-wave mixing using a nearly resonantly enhanced nonlinearity in four-level organic dye solutions was investigated. The conversion efficiency of 22% had been obtained in a 2.5 X 10-5 - molar solution of Chlorophyll A in methylalcohol with a 5 mm interaction length and a pumping energy of ～ 8 mJ from SH of a Q-switched Nd: YAG. Degene-rate four-wave mixing by two-photon resonant-enhancement in the solution of rhodamine 6G in alcohol was studied. Measurements were performed which described the dependence of nonlinear reflectivities on the molar concentrations of the media and the intensities of the pumping and object waves. Phase conjugation characteristics of forward-wave in four-wave mixing process were theoretically analysed. Experiments have cofirmed the theoretical prediction. The method of quartet degenerate four-wave mixing had been ex-tended to the doublet degenerate case. Using this method image conversion from 1.06 μm to 5320 ? had been realized with a conversion efficiency of 25% in a 5 mm long satu-rable absorber made of organic dye 9740 solution in dichloroethane. Theoretical analy-sis showed that using a medium, which is a near resonant absorber for the infrared object wave but is transparent for the visible reconstruction wave, the conversion efficiency may be well in excess of unity.
Phase conjugation of backward-and forward-wave produced by degenerate four-wave mixing using a nearly resonantly enhanced nonlinearity in four-level organic dye solutions was investigated. The conversion efficiency of 22% had been obtained in a 2.5 X 10-5 - molar solution of Chlorophyll A in methylalcohol with a 5 mm interaction length and a pumping energy of ～ 8 mJ from SH of a Q-switched Nd: YAG. Degene-rate four-wave mixing by two-photon resonant-enhancement in the solution of rhodamine 6G in alcohol was studied. Measurements were performed which described the dependence of nonlinear reflectivities on the molar concentrations of the media and the intensities of the pumping and object waves. Phase conjugation characteristics of forward-wave in four-wave mixing process were theoretically analysed. Experiments have cofirmed the theoretical prediction. The method of quartet degenerate four-wave mixing had been ex-tended to the doublet degenerate case. Using this method image conversion from 1.06 μm to 5320 ? had been realized with a conversion efficiency of 25% in a 5 mm long satu-rable absorber made of organic dye 9740 solution in dichloroethane. Theoretical analy-sis showed that using a medium, which is a near resonant absorber for the infrared object wave but is transparent for the visible reconstruction wave, the conversion efficiency may be well in excess of unity.
Phase conjugation of backward-and forward-wave produced by degenerate four-wave mixing using a nearly resonantly enhanced nonlinearity in four-level organic dye solutions was investigated. The conversion efficiency of 22% has been obtained in a 2.5×10-5-molar solution of chlorophyll A in methylalcohol with a 5mm interaction length and a pumping energy of ～8mj from SH of a Q-switched Nd:YAG. Degenerate four-wave mixing by two-photon resonant-enhancement in the solution of rhodamine 6G in alcohol was investigated. Measurements were performed which described the dependance of nonlinear reflectivities on the molar concentrations of the media and the intensities of the pumping and object waves. Phase conjugation characteristics of forward-wave in four-wave mixing process were theoretically analysed. Experiments have confirmed the theoretical prediction. The method of quartet degenerate four-wave mixing has been extended to the doublet degenerate casa. Using this method, image conversion from 1.06μm to 5320 A has been realized with a conversion efficiency of 25% in a 5 mm long saturable absorber made of organic dye 9740 solution in diehloroethane. Theoretical analysis shows that using a medium, which is a near resonant absorber for the infrared object wave but transparent for the visible reconstruction wave, the conversion efficiency may be well in excess of unity.
Both backward and forward phase conjugate waves have been observed indegenerate four-wave mixing (DFWM) in a LiNbO 3 :Fe crystalline slab. Investigation shows that the observed forward phase conjugate wave consists of two main contributions. The dominant contribution is the phase conjugate wave of the reflected signal beam. The other contribution arises from the reflection of backward phase conjugate wave at the front surface of the crystal. The intensity of the forward phase conjugate wave is comparable with that of the backward phase conjugate wave.
Optical phase conjugation is a process that leads to the correction of wavefront distortions under conditions such that a beam of light passes twice in opposite directions through an aberrating optical medium. Analogously, the state of polarization of an optical beam can become aberrated, (for example, by passing through a stressed optical component), and these polarization aberrations can be removed by the process of polarization conjugation. In polarization conjugation, the polarization unit vector of the incident wave is replaced by its complex conjugate in the generated wave.