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Quantum Optics Journal of the European Optical Society Part B

Experimental study of the forward phase-conjugate wave in degenerate four-wave mixing in LiNbO3:Fe

Sing Hai Tang, Xue Hua He, Heyi Zhang

Published Jun 1, 1991• 1 citation
Publisher

Abstract

Both backward and forward phase conjugate waves have been observed indegenerate four-wave mixing (DFWM) in a LiNbO 3 :Fe crystalline slab. Investigation shows that the observed forward phase conjugate wave consists of two main contributions. The dominant contribution is the phase conjugate wave of the reflected signal beam. The other contribution arises from the reflection of backward phase conjugate wave at the front surface of the crystal. The intensity of the forward phase conjugate wave is comparable with that of the backward phase conjugate wave.

DOI
10.1088/0954-8998/3/3/004

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Both backward and forward phase conjugate waves have been observed indegenerate four-wave mixing (DFWM) in a LiNbO 3 :Fe crystalline slab. Investigation shows that the observed forward phase conjugate wave consists of two main contributions. The dominant contribution is the phase conjugate wave of the reflected signal beam. The other contribution arises from the reflection of backward phase conjugate wave at the front surface of the crystal. The intensity of the forward phase conjugate wave is comparable with that of the backward phase conjugate wave.
DFWM as an useful tool to generate phase conjugate waves has recently been the subject of intensive study. In particular photorefractive crystals such as LiNbO3, KNbO3, BaTiO3 and SBN are widely used[1]. Among the published papers on DFWM most are concerned with backward phase conjugate waves and only a few with forward phase conjugate, waves.[2,3] In both of these papers the intensity of the forward phase conjugate wave has not been investigated. We report here a systematic study of the intensity of forward phase conjugate wave.
Stationary photorefractive self-pumped phase-conjugation with one four-wave-mixing interaction region, stimulated by the photorefractive amplified backward scattering, is obtained in LiNbO 3 :Fe crystals, in which the strong backward scattered light is gotten by putting a scattering particle on the backface of the sample. Even though its reflectivities are not high (its temporal and stationary reflectivities are 10% and 3%, respectively), due to the low electrooptic coefficients of LiNbO 3 :Fe crystals, our experimental results prove that this mechanism is effective and simple comparing with the "cat" self-pumped phase-conjugator.
Degenerate four-wave mixing (DFWM) spectroscopy is a potentially powerful technique for quantitative measurement of minor species in gas-phase media [1-3]. In this paper we compare the DFWM signal levels and lineshapes obtained using two different phase-matching geometries: the phase-conjugate geometry and the forward phase-matched geometry. DFWM signal levels are calculated by solving the time-dependent density matrix equations using direct numerical integration (DNI) [4, 5] for a two-level system interacting with three laser beams. This numerical analysis includes the effects of molecular motion, intermolecular collisions, and high laser intensities, all of which have been shown to affect the DFWM signal level.