Quantum communication and quantum computation are anticipated quantum technologies which enable us to tackle problems which are hard or even impossible to solve by classical means. A major challenge in implementing real life applications for quantum communication and quantum computation is to implement efficient interfaces between different kinds of quantum systems which serve as carriers of quantum information, such as single photons and single material quantum systems (i.e. atoms, ions ...). These different kinds of quantum systems have different advantages and disadvantages if it comes to practical applications. Single photons, which may serve as flying qubits, can be transmitted over larger distances without suffering from too much decoherence while single material quantum systems may be used as matter qubits to store and process quantum information locally. For many applications, the particular advantages of both kinds of systems are needed. Hence, we require interfaces between flying qubits and matter qubits. In the first part of this thesis, we develop suitable protocols for implementing interfaces between these flying qubits and matter qubits. The key challenge is to design the interactions to allow the efficient coupling of single photons to single material quantum systems, such as atoms and ions. This is not only of interest for possible practical applications of quantum mechanics but also drives fundamental research, as it is directly connected to a precise control and enhancement of matter-field interactions. The second part of this thesis is concerned with the applications of quantum technologies for simulating complex quantum systems, which cannot be treated by classical means. In many cases, the simulation of complex quantum systems turns out to be a difficult task due to the basic structure of quantum mechanics. The same aspects of quantum mechanics, which allow us to tackle computationally hard problems by using quantum algorithms, create difficulties in understanding the behavior of complex quantum systems. However, the understanding of complex quantum systems is not only of fundamental importance but might also enable us to give answers to problems of practical significance, such as an explanation for high-temperature superconductivity. Here, we develop protocols for implementing such quantum simulations based on ions trapped in state of the art ion traps. The applications of these kinds of quantum simulations are ranging from fundamental research to process design, control, and optimization.
Quantum communication and quantum computation are anticipated quantum technologies which enable us to tackle problems which are hard or even impossible to solve by classical means. A major challenge in implementing real life applications for quantum communication and quantum computation is to implement efficient interfaces between different kinds of quantum systems which serve as carriers of quantum information, such as single photons and single material quantum systems (i.e. atoms, ions ...). These different kinds of quantum systems have different advantages and disadvantages if it comes to practical applications. Single photons, which may serve as flying qubits, can be transmitted over larger distances without suffering from too much decoherence while single material quantum systems may be used as matter qubits to store and process quantum information locally. For many applications, the particular advantages of both kinds of systems are needed. Hence, we require interfaces between flying qubits and matter qubits. In the first part of this thesis, we develop suitable protocols for implementing interfaces between these flying qubits and matter qubits. The key challenge is to design the interactions to allow the efficient coupling of single photons to single material quantum systems, such as atoms and ions. This is not only of interest for possible practical applications of quantum mechanics but also drives fundamental research, as it is directly connected to a precise control and enhancement of matter-field interactions. The second part of this thesis is concerned with the applications of quantum technologies for simulating complex quantum systems, which cannot be treated by classical means. In many cases, the simulation of complex quantum systems turns out to be a difficult task due to the basic structure of quantum mechanics. The same aspects of quantum mechanics, which allow us to tackle computationally hard problems by using quantum algorithms, create difficulties in understanding the behavior of complex quantum systems. However, the understanding of complex quantum systems is not only of fundamental importance but might also enable us to give answers to problems of practical significance, such as an explanation for high-temperature superconductivity. Here, we develop protocols for implementing such quantum simulations based on ions trapped in state of the art ion traps. The applications of these kinds of quantum simulations are ranging from fundamental research to process design, control, and optimization.
Precise control over quantum systems can enable the realization of fascinating applications such as powerful computers, secure communication devices, and simulators that can elucidate the physics of complex condensed matter systems. However, the fragility of quantum effects makes it very difficult to harness the power of quantum mechanics. In this thesis, we present novel systems and tools for gaining fundamental insights into the complex quantum world and for bringing practical applications of quantum mechanics closer to reality. We first optimize and show equivalence between a wide range of techniques for storage of photons in atomic ensembles. We describe experiments demonstrating the potential of our optimization algorithms for quantum communication and computation applications. Next, we combine the technique of photon storage with strong atom-atom interactions to propose a robust protocol for implementing the two-qubit photonic phase gate, which is an important ingredient in many quantum computation and communication tasks.
Experiments in quantum optics are motivated by fundamental questions about the quantum mechanical description of matter and light as well as by applications in quantum technologies such as quantum information processing. Exploiting the quantum character of both matter and light has turned out to be extremely rewarding for novel technological applications in the emerging fields of quantum communication and computation. Here we consider the implementation of quantum information technology with trapped ions and single photons, focusing on two key issues: the entanglement of distant atoms and the controlled interaction of a single photon with a single atom.
This thesis describes the construction of a double ion trap apparatus including the necessary frequency-stabilized laser systems, and first experiments to investigate the generation of distant atomic entanglement, the implementation of a simple quantum network and controlled single-atom single-photon interaction. The experimental setup comprises two ion traps at a distance of one meter, which are independent but identical in construction. We introduce novel realizations of a photoionization method for calcium atoms, a laser frequency stabilization scheme and a radio frequency pulse sequencer. Linear Paul traps are used to load individual or strings of calcium ions. High-numerical aperture objectives mounted on sub-micrometer positioning systems allow us to address and manipulate a single ion with strongly focused light fields and collect the emitted fluorescence photons from a large solid angle. With these bidirectional single-atom single-photon interfaces the essential building blocks of a quantum network with atoms and photons are available. One of the main objectives we pursue with the double-trap apparatus is the generation of entanglement between ions in different traps, which is one of the key tasks in a quantum network. We compare single- and two-photon schemes for probabilistic entanglement creation and analyze how the performance of the schemes depends on photon detection efficiency. As a first step towards the experimental realization of such schemes we measure the second order correlation function of fluorescence photons emitted from two distant trapped ions. We observe high-contrast quantum (Hong-Ou-Mandel) interference, proving the indistinguishability of photons emitted from different ions, which is a prerequisite for the considered entanglement schemes. To investigate the interaction of single photons and a single atom in free space we combine the ion trap apparatus with a tunable, narrowband spontaneous parametric down-conversion source. The high-numerical aperture objectives allow us to efficiently couple bandwidth-tunable photons to a single trapped ion. Such atom-photon interaction at the single-particle level is the most fundamental process in quantum optics and lies literally at the focus of many experimental implementations of quantum information processing protocols and of studies of the (quantum) limits of matter -light interaction, which were so far restricted to weak coherent light fields. Here we observe individual atomic absorption events of one photon of an entangled pair by employing a quantum jump detection scheme. To characterize and control the interaction process we modify the spectral properties of the down conversion photons and perform single-photon spectroscopy of a single ion. To go beyond experiments with cohe rent fields we study temporal correlations between the absorption of photons from the spontaneous parametric down conversion source by a single ion and the detection of the corresponding partner photon.
For the applied scheme we observe promising indications that the quantum correlations of photons produced in spontaneous parametric down conversion are preserved in the resonant interaction with a single atom. The implementation of more efficient atom-light coupling and entanglement transfer schemes with our apparatus is outlined.
Devices that harness the surprising properties of quantum systems at scale hold the possibility of revolutionary advances in information technology. Algorithms for quantum computers can take advantage of quantum parallelism to solve problems that are intractable with classical hardware, including prime factorization and simulating chemical processes. A quantum communication network that carries qubits instead of bits can leverage the irreversibility of projective measurement to guarantee secure communication. Because quantum states are fragile, building such devices requires exquisite control over many isolated quantum systems. One of the most critical capabilities is the interaction of stationary and flying qubits. In this thesis we consider how to engineer atom-light interactions as an interface for networked quantum systems. Quantum atom-light couplers require the efficient and reversible interaction of atomic and optical qubits, but the natural interaction of atoms and photons is weak. It is this very lack of interaction between light and its environment that makes light such an excellent carrier of quantum information. There are three promising strategies for stronger coherent atom-light interactions. First, the light field may be confined to a cavity so that it interacts with the atom over a longer time. Second, the light field may be focussed to a small spot with high aperture optics and matched to the natural atomic radiation pattern. Third, we may pass the light field through an ensemble of many atoms and store the qubit in a distributed state. In practice, atom-light couplers employ some combination of all three strategies. We will focus our research on the second two approaches: first by coupling one and two trapped ions with high aperture optics, and then operating a quantum optical memory with an ensemble of approximately 10 billion neutral atoms. Atoms that have been ionized and trapped in a common electromagnetic potential are an advanced few-qubit computation platform. Qubit states are associated with an electronic excitation at each atom, controlled coherently with lasers, and made to interact in two (or many) qubit gates by mutual Coulomb repulsion. One path to quantum advantage with ion-trap quantum processors is to scale small qubit registers by distributing entanglement with photonic interconnects. We consider the feasible efficiency of free-space atom-light couplers for atomic dipole transitions, and derive the atomic image by common free-space couplers. We couple a trapped-ion register with high-aperture lenses and operate a single trapped ion as a photon source. We model the dynamic character of the source and show spin-orbit coupling in the single-photon spatial mode. Although the total collection efficiency is only approximately 0.01, the source has exceptional photon-number purity A = (1.9 +/- 0:2) * 10^-3 such that the higher-order quantum nature of the field persists even after most of the field has been discarded. We derive an efficient quantum non-Gaussian witness and surpass it, the first such demonstration for a trapped-atom single-photon source. We entangle two trapped atoms by single-photon detection, and observe an interference pattern in the spatial mode of the bipartite state. Constructive interference between the entangled components enhances the emission probability by up to 29%, an example of collective enhancement by a two-atom ensemble. The efficiency of free-space atom-light couplers is limited by our capability to engineer high-precision, high-aperture optics. We fabricate ultra-precise hemispheric mirrors with numerical aperture 0.996 by single point diamond turning. The mirrors are amongst the smoothest hemispheric surfaces ever manufactured with root-mean-square (RMS) errors consistently below 25 nm. The smoothest of our mirrors has a RMS error of 14 nm and peak-to-valley error of 88 nm. A mirror with this surface is capable of suppressing or enhancing the spontaneous emission of an atom into free space by 96% in a proposed quantum electrodynamics experiment. We show how these mirrors, with a simple modification, can shape the spatial mode of a trapped atom by similar vacuum-mode engineering. We derive a near-hemispheric mirror coupling scheme that should be 72% efficient with mirrors as precise as ours. We design an ion trap for use with such high-aperture optics. With careful conditioning and control, ensembles of many atoms can be made to store and release photonic qubits on demand. Such optical quantum memories leverage the collective interaction of a light field with many billions of atoms to achieve storage and recall efficiencies approaching unity. We show how stationary light fields for photonic phase gates can be generated in optically deep ensembles, an effect which has since been observed. We implement the gradient echo memory (GEM) scheme in an ultra-high optical depth cold-atom ensemble. The performance of a practical quantum memory is contingent on the chosen qubit encoding. We extend the GEM protocol to allow the simultaneous storage of frequency separated signals and demonstrate that this `dual-rail' memory is suitable for high-fidelity frequency qubits. Dual-rail signals are recalled with 35% efficiency, 82% interference fringe visibility and 6 degrees of phase stability. We describe how the fidelity of the scheme is limited by frequency-dependent polarization rotation and how this may be addressed in an improved configuration. Finally, we demonstrate single-rail storage by GEM with 87% efficiency and 1 ms memory lifetime. Our memory surpasses the no-cloning limit for up to 600 us of storage, out-performing an optical fibre delay line by a factor of six. This is the first quantum memory to beat this important benchmark.
Quantum technologies harness the properties of controlled quantum mechanical systems for applications in computation, communication and metrology, and enable us to further our understanding of fundamental physics. Quantum hardware is designed to manipulate complex and fragile many-particle quantum states, which requires exquisite control machinery, advanced software and near-complete isolation from the surrounding environment. With sufficient capabilities, quantum computers with large registers of quantum bits will perform classically intractable calculations such as quantum chemistry simulations. Quantum key distribution will provide completely secure communications across the world and quantum metrology will enable measurement precision beyond today's capabilities. While quantum technologies are far from surpassing classical hardware today, the vision and potential impact has sparked a world-wide research effort, both theoretical and experimental, to develop a quantum computer. The most sophisticated current quantum technologies have control over small numbers of quantum bits and are limited by environmental decoherence processes. While progress in developing quantum hardware is ongoing, designing and demonstrating new algorithms and protocols for quantum information is a thriving research field. Photonics provides an ideal platform for small-scale proof-of-concept quantum experiments, which are the focus of this thesis. In the coming decades, we will see the realisation of quantum hardware capable of applications that outperform any classical computer. In this thesis, I present several protocols and algorithms for quantum information science and technology, which are implemented in quantum photonic experiments. The applications of these works include robust quantum tomography, quantum state relocation, quantum enhanced data recovery and probing fundamental causality in quantum mechanics. The works presented here are based on two photon experiments from a prototypical spontaneous parametric down-conversion source, which provides an excellent test-bed for quantum information experiments. Photons can be used to encode quantum information in a range of different degrees of freedom. This versatility, along with compatibility with existing technology gives photonics a great advantage in the development of quantum hardware.
An extensively pursued current direction of research in physics aims at the development of practical technologies that exploit the effects of quantum mechanics. As part of this ongoing effort, devices for quantum information processing, secure communication, and high-precision sensing are being implemented with diverse systems, ranging from photons, atoms, and spins to mesoscopic superconducting and nanomechanical structures. Their physical properties make some of these systems better suited than others for specific tasks; thus, photons are well suited for transmitting quantum information, weakly interacting spins can serve as long-lived quantum memories, and superconducting elements can rapidly process information encoded in their quantum states. A central goal of the envisaged quantum technologies is to develop devices that can simultaneously perform several of these tasks, namely, reliably store, process, and transmit quantum information. Hybrid quantum systems composed of different physical components with complementary functionalities may provide precisely such multitasking capabilities. This article reviews some of the driving theoretical ideas and first experimental realizations of hybrid quantum systems and the opportunities and challenges they present and offers a glance at the near- and long-term perspectives of this fascinating and rapidly expanding field.
During the last decades the development of laser cooling and trapping has revolutionized the field of quantum optics. Now we master techniques to control the quantum properties of atoms and light, even at a single atom and single photon level. Understanding and controlling interactions of atoms and light both on the microscopic single particle and on the macroscopic collective levels, are two of the very active directions of the current research in this field. The goal is to engineer quantum systems with tailored properties designed for specific applications. One of the ambitious applications on this way is interfacing quantum information for quantum communication and quantum computing. We summarize here theoretical ideas and experimental methods for interfacing atom-based quantum memories with single flying photons.