In this thesis, we study the diffraction processes of a Bose-Einstein condensate of 87Rb atoms and outline our progress toward the realisation of an atom laser. The experiments are carried out with a condensate that is produced ‘all-optically’; this is covered in the first part of the thesis. For our diffraction processes, we expose the condensate to an intense, pulsed optical standing wave. We perform mean energy measurements and interpret our results with two different theories: one treating the condensed atoms as particles, the other focusing on the atoms’ wave properties. The first interpretation requires knowledge of the theoretical background of the atom-optics -kicked rotor (AOKR); in our experiments, we focus on the resonances in the early-time behaviour of the kicked atoms. The second interpretation retrieves an observation of the temporal Talbot effect—the atomic analogue to the optical Talbot effect. From this point of view, the full resonances represent the integer Talbot effect, whereas the early-time behaviour corresponds to the observation of the fractional Talbot effect. We find for both theoretical interpretations an excellent qualitative agreement between our experimental results and the results of our computer simulation of the AOKR. Furthermore, we outline our future work on the realisation of an atom laser as a tool for coherence measurements of the condensate via atom-counting statistics. In this context, the most current progress in our laboratory is given. We aim for a Bragg-scattering process of our condensate as a modified version of our prospective outcoupling technique for the atom laser; this process is modelled in a semi-classical approach, and our first experimental implementations are presented.
In this thesis, we study the diffraction processes of a Bose-Einstein condensate of 87Rb atoms and outline our progress toward the realisation of an atom laser. The experiments are carried out with a condensate that is produced ‘all-optically’; this is covered in the first part of the thesis. For our diffraction processes, we expose the condensate to an intense, pulsed optical standing wave. We perform mean energy measurements and interpret our results with two different theories: one treating the condensed atoms as particles, the other focusing on the atoms’ wave properties. The first interpretation requires knowledge of the theoretical background of the atom-optics -kicked rotor (AOKR); in our experiments, we focus on the resonances in the early-time behaviour of the kicked atoms. The second interpretation retrieves an observation of the temporal Talbot effect—the atomic analogue to the optical Talbot effect. From this point of view, the full resonances represent the integer Talbot effect, whereas the early-time behaviour corresponds to the observation of the fractional Talbot effect. We find for both theoretical interpretations an excellent qualitative agreement between our experimental results and the results of our computer simulation of the AOKR. Furthermore, we outline our future work on the realisation of an atom laser as a tool for coherence measurements of the condensate via atom-counting statistics. In this context, the most current progress in our laboratory is given. We aim for a Bragg-scattering process of our condensate as a modified version of our prospective outcoupling technique for the atom laser; this process is modelled in a semi-classical approach, and our first experimental implementations are presented.
This thesis reports on the experimental investigation of several applications of the atom-optical quantum kicked rotor (AOQKR) using a Bose-Einstein condensate (BEC) of 87Rb atoms. The AOQKR was achieved by exposing a BEC to short periodic pulses from a horizontal optical standing wave formed from the interference of two off-resonant laser beams. In the first set of experiments the fidelity or overlap between the kicked rotor states with a reference state was studied. The fidelity resonance widths in pulse period and in acceleration were found to scale as the inverse cube of the kick numbers, a sub-Fourier behavior with possible application in precision measurement experiments. The sensitivity of the fidelity to acceleration was experimentally and theoretically investigated and found to depend on the magnitude and direction of the applied acceleration. The asymmetry between positive and negative acceleration was found to be related to the temperature of the atomic sample. In the second set of experiments, the phenomenon of a quantum ratchet (which is manifested by a directed current of particles in the absence of a net bias force) both at resonance and away from resonance was studied. It was confirmed that the current direction can be controlled by changing experimental parameters which leave the underlying symmetries of the system unchanged. It was demonstrated that this behavior can be understood using a single variable containing many of the experimental parameters. These experiments confirmed that such a ratchet behavior can under certain circumstances be the same in both the true classical and quantum regimes. The final application of the AOQKR discussed in this thesis is the quantum accelerator mode. Both the formation and decay mechanism of these modes were studied.
The field of atom optics has progressed rapidly over the past 20 years since the realisation of Bose-Einstein condensation, such that the wave behaviour of atomic gases is now routinely demonstrated. Furthermore, the study of quantum atom optics, which goes beyond a ‘mean-field’ description of quantum systems to consider the behaviour of single particles, has demonstrated both the similarities between photons and massive species, and their differences as a result of the internal structure and external interactions of atoms. An important class of observable quantities which allow such effects to be measured are nth order correlation functions, which can be interpreted as a result of either particle or wave behaviour. These functions provide a statistical description of fluctuations in n-tuples of particles in a source, which rigorously defines concepts such as coherence. The quantum statistics of a Bose-Einstein condensate should be the same as that for an optical laser, while an ideal thermal Bose gas matches the behaviour of incoherent light. However, correlation measurements can also be used to quantify the influence of interactions, dimensionality, confining potentials and waveguides, and the difference in quantum statistics between fermions and bosons, which illustrates the rich range of behaviour exhibited by atomic gases. In this thesis, several aspects of quantum atom optics are explored with experiments using ultracold metastable helium, a species with the unique advantage of facilitating simple single-atom detection with high resolution, while still allowing Bose-Einstein condensates to be formed. The coherence of atomic systems is shown to be maintained when outcoupled as pulsed atom lasers, and the long-range order characteristic of Bose-Einstein condensates is demonstrated to third order for the first time. Conversely, thermal bunching is observed for a variety of atomic systems, including the measurement of correlation functions up to sixth order with near-ideal interference contrast. These results clearly demonstrate the correspondence between the quantum statistics of photons and atoms as was formalised by Glauber, as well as confirming the validity of applying Wick’s theorem to simplify the statistics of atomic gases. Correlation functions are also shown to be an ideal tool to probe the quantum state of an ultracold gas, and were used to observe the phenomenon of transverse condensation in an elongated Bose gas, as well as characterise the mode occupancy of matter waves guided by an optical potential. Ultracold metastable helium is also suitable for exploring other fundamental topics in quantum optics such particle/wave duality. The notion of complementarity stimulated long running philosophical discussions about how apparently mutually exclusive behaviours can coexist, which culminated in Wheeler devising his famous ‘delayed choice’ gedankenexperiment. A proposed experimental method to realise Wheeler’s experiment with ultracold atoms is discussed, and preliminary measurements presented which indicate that the completion of this experiment could be achieved in the near future. Not only is this of interest in its own right, but the implementation of this experiment has also developed techniques which may enable further studies in quantum atom optics such as investigations of the Hong-Ou-Mandel effect and quantum entanglement with massive particles.
This thesis deals with an investigation of the chaotic dynamics of an atom optics δ-kicked rotor (AOKR) system, a paradigm of classical and quantum chaos. The AOKR rotor is realized by subjecting a Bose-Einstein condensate (BEC) of ⁸⁷Rb atoms to a periodic potential. The potential in the form of a standing wave, obtained from a far detuned laser beam is turned on and off periodically in time, producing short pulses (kicks) of laser light. For certain values of the period between the kicks, resonant effects known as quantum resonances are observed that are purely quantum effects. Quantum resonances have been examined in the AOKR for a series of kicks. For large number of kicks, the width of these resonances have been shown to become narrow. Higher order resonances corresponding to fractional Talbot times have been observed in the system. These quantum resonant effects have been found to depend sensitively on the initial velocity of the atoms. The first three primary resonances have been studied in detail, by measuring the momentum distribution and the kinetic energy of the atoms, for two and four kicks. A sinusoidal dependence of the energy on the initial momentum has been observed for two kicks. By increasing the number of kicks, the system becomes extremely sensitive to the initial momentum of the atoms. For four kicks, a more complex behavior is observed in the system energy. A scheme for investigating Loschmidt time reversal of chaotic dynamics of the atomic deBroglie waves have been described in the AOKR system. It has been demonstrated that the initial wave function of an ensemble of ultracold atoms is restored, after a series of delta-kicks in what is essentially a multiple beam interferometry experiment. During the process, the evolution of the system for a fraction of the atoms with a very small initial momentum is reversed, which results in a narrowing of the momentum distribution. It is hoped that the research presented in this thesis will significantly contribute to the understanding of the connection between the classical and quantum worlds.
Research in the field of ultra-cold quantum gases provides a testbed to examine Hamiltonians from other areas of physics such as the Bose-Hubbard Hamiltonian, as well as interesting phenomena such as superconductivity and superfluidity. Of emerging interest in the field is the analysis of non-equilibrium behaviour. This thesis focuses on the non-equilibrium dynamics of Bose gases in two different elongated systems: a continuously-pumped atom laser, and the formation of solitons as a result of a rapid quench through the Bose-Einstein condensation phase transition. We begin by introducing the theoretical tools required to model these systems, including the Stochastic Projected Gross-Pitaevskii formalism that describes the dynamics of a condensate in contact with a thermal cloud. We apply the Stochastic Projected Gross-Pitaevskii formalism to model a Raman-outcoupled atom laser continuously outcoupled from a replenished condensate reservoir at finite temperature. We investigate the first and second order coherence of the output as a function of the temperature of the condensate reservoir. For large momentum kicks given to outcoupled atoms, we show for the first time that the coherence of the atom laser beam is linked to that of the condensate reservoir. We observe a decrease in first order coherence of the condensate reservoir as its temperature is increased, and show that this decrease is caused by the dephasing of thermal fluctuations. We also investigate the effects of varying the outcoupling rate and the momentum kick on the first order coherence of the beam. We demonstrate that the first order coherence of the atom laser beam deviates from that of the condensate reservoir for small momentum kicks which we identify as due to interactions between the condensate and atom laser beam. Thermal density fluctuations in the condensate cause the atom laser beam to experience a stochastic force and the temporal coherence of the atom laser beam is reduced. We find that the condensate reservoir is significantly depleted for large outcoupling rates, resulting in a reduction in the steady state condensate fraction and in the first order coherence of the atom laser beam. In a second study, the momentum linewidth of a guided atom laser outcoupled using a radio-frequency transition is investigated at zero and finite temperature. We examine the momentum distribution of the beam by measuring the transmission of atoms over a potential barrier following the experimental scheme of the group of Professor Alain Aspect at Institut d'Optique. We observe a noisy momentum distribution for outcoupling rates in the weak-outcoupling limit at zero temperature. We show that the noise is caused by bulk excitations within the condensate reservoir as a result of a density depression caused by the non-adiabatic switch-on of outcoupling. We show that these excitations can be prevented by increasing the outcoupling rate to its final value linearly over time. In addition, we demonstrate that a thermally-broadened linewidth could potentially be measured using this experimental technique, and discuss challenges associated with the measurement scheme. Finally, we focus on the non-equilibrium dynamics of condensate growth in elongated geometries. Following a rapid quench through the Bose-Einstein condensation phase transition, we observe the spontaneous appearance of density dips which we identify as solitons. We develop an algorithm for counting these solitons in order to observe the temporal dependence of the soliton number as a function of the quench rate. To compare with the predictions of the Kibble-Zurek mechanism describing topological defect formation as a result of the dynamics of phase transitions in homogeneous systems, we calculated the scaling exponent of the soliton number with respect to the quench rate. Our results were qualitatively consistent with the Kibble-Zurek predictions, but quantitative comparisons were inconclusive. In trapped systems the phase transition proceeds inhomogeneously, with a phase front that propagates in space with a velocity. If this is lower than a critical value it has been predicted that this can inhibit defect formation. However, our results do not show conclusive evidence of this in the parameter regime that we study. We find that the number of solitons reduces as the condensate reaches equilibrium as a result of the damping included in the Stochastic Projected Gross-Pitaevskii formalism.
This thesis presents an account of experimental and numerical investigations of two quantum systems whose respective classical analogues are chaotic. These are the delta-kicked rotor, a paradigm in classical chaos theory, and the novel delta-kicked accelerator, created by application of a constant external acceleration or torque to the rotor. The experimental realisation of these systems has been achieved by the exposure of laser-cooled caesium atoms to approximate delta-kicks from a pulsed, high-intensity, vertical standing wave of laser light. Gravity’s effect on the atoms can be controlled by appropriate shifting of the profile of the standing wave. Numerical simulations of the systems are based on a diffractive model of the potential’s effect. Each system’s dynamics are characterised by the final form of the momentum distribution and the dependence of the atoms’ mean kinetic energy on the number and time period of the delta-kicks. The phenomena of dynamical localisation and quantum resonances in the delta-kicked rotor, which have no counterparts in the system’s classical analogue, are observed and investigated. Similar experiments on the delta-kicked accelerator reveal the striking phenomenon of the quantum accelerator mode, in which a large momentum is transferred to a substantial fraction of the atomic ensemble. This feature, absent in the system’s classical analogue, is characterised and an analytic explanation is presented. The effect on each quantum system of decoherence, introduced through spontaneous emission in the atoms, is examined and comparison is made with the results of classical simulations. While having little effect on the classical systems, the level of decoherence used is found to degrade quantum signatures of behaviour. Classical-like behaviour is, to some extent, restored, although significant quantum features remain. Possible applications of the quantum accelerator mode are discussed. These include use as a tool in atom optics and interferometry, a technique for measuring gravity, and a method of preparing atoms in a particular region of phase space. This may allow measurement of quantum phase space stability, and hence investigation of quantum chaos and quantum-classical correspondence.
In this thesis a number of aspects on possible manipulation of Bose-Einstein condensate in trapped atomic gases is investigated. First, a model for atom optical experiments involving Bose condensates is proposed and numerical simulations are presented to illustrate its characteristics. We demonstrate ways of focusing and splitting the condensate by modifying experimentally adjustable parameters. We show that there are at least two ways of implementing atom optical elements: one may modulate the interatomic scattering length in space, or alternatively, use a sinusoidal, externally applied potential. The temporal evolution of quasiparticle excitations is studied via the Gross-Pitaevskii Equation. Nonlinear mode mixing of quasiparticles is introduced, and is observed using a quasiparticle projection method. This is used as a basis of time-dependent finite temperature simulations, which we argue to be valid under regimes of high occupation number. An illustration via a closely related evaporative cooling simulation is provided. A phenomenological damping formalism for superfluidity near the λ point is adopted to describe the damping of excitations in a Bose-Einstein condensate. An estimate for the damping parameter is found. The damping formalism as a numerical tool to calculate the ground eigenstate of the condensate is explored. A novel, experimentally realisable interferometry for Bose-Einstein condensates using near-field diffraction is proposed. The scheme is based on the phenomenon of intermode traces or quantum carpets; we demonstrate the structured spatio-temporal pattern for the dilute, atomic Bose-Einstein condensate. The pattern is found to change with temperature, which allows us to perform interferometric temperature measurements. Finally, an output coupler for Bose-Einstein Condensates based on stimulated Raman transition is investigated. The spectrum and coherence are calculated for an atomic beam slowly coupled out of a trap containing a partially condensed Bose gas at finite temperatures. A number conserving Hartree-Fock-Bogliubov formalism has been used to incorporate finite temperature effects. Various different processes are found to become dominant for a suitable choice of the coupling parameters.