Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Foundation experiments in quantum atom optics with ultracold metastable helium

Andrew Manning

Published Jan 1, 2014• 1 citation
Publisher

Abstract

The field of atom optics has progressed rapidly over the past 20 years since the realisation of Bose-Einstein condensation, such that the wave behaviour of atomic gases is now routinely demonstrated. Furthermore, the study of quantum atom optics, which goes beyond a ‘mean-field’ description of quantum systems to consider the behaviour of single particles, has demonstrated both the similarities between photons and massive species, and their differences as a result of the internal structure and external interactions of atoms. An important class of observable quantities which allow such effects to be measured are nth order correlation functions, which can be interpreted as a result of either particle or wave behaviour. These functions provide a statistical description of fluctuations in n-tuples of particles in a source, which rigorously defines concepts such as coherence. The quantum statistics of a Bose-Einstein condensate should be the same as that for an optical laser, while an ideal thermal Bose gas matches the behaviour of incoherent light. However, correlation measurements can also be used to quantify the influence of interactions, dimensionality, confining potentials and waveguides, and the difference in quantum statistics between fermions and bosons, which illustrates the rich range of behaviour exhibited by atomic gases. In this thesis, several aspects of quantum atom optics are explored with experiments using ultracold metastable helium, a species with the unique advantage of facilitating simple single-atom detection with high resolution, while still allowing Bose-Einstein condensates to be formed. The coherence of atomic systems is shown to be maintained when outcoupled as pulsed atom lasers, and the long-range order characteristic of Bose-Einstein condensates is demonstrated to third order for the first time. Conversely, thermal bunching is observed for a variety of atomic systems, including the measurement of correlation functions up to sixth order with near-ideal interference contrast. These results clearly demonstrate the correspondence between the quantum statistics of photons and atoms as was formalised by Glauber, as well as confirming the validity of applying Wick’s theorem to simplify the statistics of atomic gases. Correlation functions are also shown to be an ideal tool to probe the quantum state of an ultracold gas, and were used to observe the phenomenon of transverse condensation in an elongated Bose gas, as well as characterise the mode occupancy of matter waves guided by an optical potential. Ultracold metastable helium is also suitable for exploring other fundamental topics in quantum optics such particle/wave duality. The notion of complementarity stimulated long running philosophical discussions about how apparently mutually exclusive behaviours can coexist, which culminated in Wheeler devising his famous ‘delayed choice’ gedankenexperiment. A proposed experimental method to realise Wheeler’s experiment with ultracold atoms is discussed, and preliminary measurements presented which indicate that the completion of this experiment could be achieved in the near future. Not only is this of interest in its own right, but the implementation of this experiment has also developed techniques which may enable further studies in quantum atom optics such as investigations of the Hong-Ou-Mandel effect and quantum entanglement with massive particles.

DOI
10.25911/5d73903cb71ea

Related papers

Transition lifetime measurements and correlation experiments with ultra-cold metastable helium

Sean S. Hodgman

Trapped gases of ultracold metastable helium atoms are a unique experimental sys- tem. The trapped cloud’s low temperatures, the ability to selectively trap and ma- nipulate individual atomic states and the isolation provided in a vacuum chamber are all conducive to the measurement of precision atomic parameters, such as atomic transition rates. Due to it’s atomic structure helium - the simplest multi-electron atom - is a favourite test-bed for precision QED theoretical calculations compared to experimentally determined parameters. This thesis reports on a number of tran- sition rates measured for the first time with high accuracy, including the first excited metastable state lifetime, found to be 7870(510)s, the longest of any neutral atomic species yet measured. Transition rates from the 23P level to the ground state were also measured for the first time and found to be in excellent agreement with theory. Further cooling of helium produces a Bose-Einstein condensate (BEC), where all atoms are in an identical quantum state, the analogue of an optical laser. One par- ticularly interesting property a BEC posesses is long-range coherence to all orders, meaning all component particles are described by a single wavefunction. While first order coherence is measured in an interference experiment like Young’s double slit, higher order coherence is the ability for correlations to exist between groups of two, three or more particles, quantified by the measurement of correlation functions. Prior to the work in this thesis correlation functions for atoms had only been measured for second order. Here we develop a new technique which we use to show that a BEC is coherent to second and third order to 0.1% accuracy, compared to a thermal cloud which we show is incoherent. At small inter-particle spacings, there is an enhanced probability of measuring double and triple events in the thermal cloud (termed bunching). A drawback of all previous atomic correlation measurements is that the small de-Broglie wavelengths compared to the detector resolution leads to a significant reduction in the measured bunching amplitudes compared to theory. By altering our trapping configuration and temperature we are able to measure a two-particle bunching amplitude which is 88% of the theoretical maximum. This system also allowed the measurement of correlations up to 5th order in thermal gases. The near ideal bunching allowed us to demonstrate perturbations to the correlation functions due to the 1D nature of the system. These advances should lead to correlation measurements being used as a probe to characterise more exotic system properties such as low dimensionality, engineered quantum states and paticle pairing. Finally, a waveguide was created using a dipole laser beam and used to guide atoms in analogy to an optical laser in a fibre. Guided ‘atom lasers’ are likely to be important components for practical devices such as precision sensors. We demonstrate that a guided atom laser has a gaussian profile matching the lowest transverse mode of the waveguide and is first and second order coherent. In contrast guided thermal atoms show matter-wave speckle and are incoherent.

•Jan 1, 2011•0 citations

Hanbury Brown-Twiss and higher order correlations in ultracold atomic clouds of metastable Helium

RuGway Wu

Trapped ultracold gases of metastable helium atoms provide a unique experimental system. The high internal energy enables electronic detection of single atoms. This thesis presents a number of experimental studies using metastable helium. Ionization rates in a mixture of metastable helium and rubidium were measured. Spin polarisation of the system has been shown to result in suppression of Penning ionization of rubidium by metastable helium atoms, suppressed by at least a hundred fold. This demonstration is a promising step towards the first creation of a binary BEC comprising atoms in both ground and excited states. The other experiments presented are mainly concerned with Hanbury Brown-Twiss and Higher order correlations. Single atom detection for metastable helium empowers experimenters to acquire spatial and temporal information, and to obtain full 3D reconstruction for released atomic clouds. Measurements on incoherent boson sources show bunching of particles. This enhancement to probability of joint detection events for two or more particles within short separations is in contrast to the uniform distribution of a coherent state, as measured for a Bose-Einstein condensate or an atom laser. By manipulating correlation length at the detector we were able to demonstrate the first atomic measurement of spatial three-particle correlation, and the results show significant improvement over previously reported values. Furthermore, by using a different trap geometry, it was possible perform measurement of atomic correlation functions to the 6th order, and have observed near ideal correlation functions to the 5th order, demonstrating enhancement for multi-particle detection probability consistent with the prediction of Wick's theorem. Correlations are then exploited to monitor the evolution of coherence property during the formation of a Bose-Einstein condensate. The experimental results are consistent with the existence of a quasi-condensation stage during the system's evolution from an incoherent thermal cloud towards a condensate with long range order. Two cases of mixing processes leading to the production of paired atom beams were Studied. In one case, correlation measurement provided the first higher order test of coherence of amplified matter waves. Coherence properties of matter waves generated via Bose stimulation are critical for active atom optical devices. Previously, coherence properties of amplified matter waves have only been demonstrated to first order by interference fringes. In the second case, a novel mixing process previously unknown was observed. Single atom counting is used to show number difference squeezing between opposite modes. Both processes studied hold potential of providing simple and elegant ways of producing pairs of coherent, sub-Poissonian number difference, and even entangled modes of atomic beams. Finally, physics of lower dimensions was studied. Observation was made of the phenomenon of two-step condensation in a quasi-1D system, where the gas condenses in the tightly confining transverse directions, yet remain thermal in the longitudinal direction. The lack of long-rang coherence of the system is revealed with correlations. Furthermore, an attempt was made to identify the Berezinskii-Kosterlitz-Thouless (BKT) transition.

•Jan 1, 2013•0 citations

Two experiments on quantum correlations in gases of metastable helium: fermion antibunching and a study of boson pair correlations in the collision of two condensates

Valentina Krachmalnicoff

This thesis presents two experiments on ultracold gases of metastable Helium that constitute the extension, to matter waves, of experiments that have been fundamental for the development of quantum optics. Both experiments have been realized by using a single atom detector, that allows one to reconstruct the position of the atoms in three dimensions. In the first experiment we directly compared the two-body correlation function for a cold cloud of identical fermions and for a cold cloud of identical bosons at the same temperature issued from the same experimental apparatus. Since bosons and fermions obey different quantum statistics, the two-body correlation functions are different: identical bosons tend to be detected bunched in pairs, while identical fermions tend to antibunch because of the Pauli exclusion principle. In the second experiment we studied the correlation between pairs of bosonic atoms generated in the collision of two Bose-Einstein condensates. The measurement of the correlation function allows us to demonstrate that atoms flying back to back in the centre of mass frame are correlated in pairs. Furthermore the observation of a Hanbury Brown Twiss correlation between atoms with collinear velocity demonstrates that our system cannot be interpreted in terms of classical mechanics, but that the bosonic statistics plays a crucial role. A new version of the experiment will allow us to measure the angular dependence of the population of the scattering modes and the number difference squeezing between two correlated modes.

•Jun 22, 2009•1 citation

Quantum correlations and atomic speckle

Sean S. Hodgman, R. G. Dall, Andrew Manning +3 more

Here we utilize the single-atom detection capability of metastable helium to measure the second-order and third-order correlation functions for ensembles of ultracold atoms. We then extend these measurements to characterize the quantum statistics of atoms guided in a dipole potential. By appropriately loading atoms into the guide we are able to populate a selected number of guided modes, ranging from the majority of atoms in the lowest order mode (a BEC), to multi-mode guiding (equivalent to a thermal source). The guided BEC was characterised by a smooth gaussian transverse spatial profile, and a second-order correlation value of unity consistent with a coherent source. For multi-mode guiding, the matter-wave equivalent of speckle was observed. Furthermore, at short arrival times, the second-order correlation function was greater than unity, corresponding to atom bunching characteristic of an incoherent (thermal) source.

•Jan 1, 2011•0 citations

Quantum-Atom Optics and Dynamical Simulations of Fermionic Many-Body Systems

Magnus Ögren, Karen V. Kheruntsyan, Joel Frederick Corney +1 more

Abstract The measurement and characterisation of correlation functions has recently become one of the central themes in the studies of ultracold quantum gases. By probing complex many-body states of these interacting systems, correlation functions facilitate the most in-depth understanding of the underlying physics, not accessible through simple density profile measurements. In this thesis, we study the dynamics of second-order correlation functions for atoms created in pair-production processes such as molecular dissociation and atomic four-wave mixing. More specifically, in Chapter 3 we analyse the dynamics of correlated atom pairs created via controlled dissociation of a Bose-Einstein condensate of diatomic molecules. The atomic constituents can be either a pair of bosonic or fermionic atoms. The process provides a matter-wave analog of parametric down-conversion with photons, which was pivotal in the advancement of quantum optics by enabling experimental demonstrations of the famous Einstein-Podolsky-Rosen paradox and violations of a classical Bell inequality. The atom-optics analogues of parametric down-conversion make it possible to envisage similar demonstrations using ensembles of massive particles in quantum gas regimes. In the case of fermionic constituents, molecular dissociation offers the possibility of a new paradigm in fermionic quantum-atom optics. By aiming at experimentally realistic modelling, we examine the role of spatial inhomogeneity of harmonically trapped molecular condensates on the strength and the shape of atom-atom correlations. Using the undepleted molecular-field approximation, we obtain explicit analytic results for the short-time asymptotic behaviour of the second-order correlation functions and for relative number squeezing between the dissociated atoms in one, two, and three spatial dimensions. Comparisons with the numerical results, which incorporate the molecular depletion and s-wave scattering interactions, show that the analytic approaches employed here capture the main underlying physics and provide useful insights into the dynamics of dissociation for conversion efficiencies up to 10%. The results show explicitly how the strength of atom-atom correlations and relative number squeezing degrade with the reduction of the size of the molecular condensate. In Chapter 4, we study highly anisotropic molecular condensates in order to quantify the effects of bosonic stimulation and fermionic Pauli blocking on the dissociation dynamics. We show that the difference in quantum statistics of the atomic constituent is manifest as complementary geometric structures in the density profiles of the dissociated atoms. Atomic bosons are preferentially emitted along the long axis of the molecular condensate due to bosonic stimulation, while atomic fermions are preferentially emitted along the short axis due to Pauli blocking. This anisotropy potentially simplifies the measurement of correlations between the atoms through relative number squeezing. In Chapter 5 we apply our analytic approaches to a related problem of atomic four-wave mixing and analyze atom-atom correlations in the s-wave scattering halo of two colliding condensates. The results in the short-time limit are in agreement with the first-principles simulations using the positive-P representation and provide analytic insights into the experimental observations of Perrin et al. [Phys. Rev. Lett. 99, 150405 2007]. The final chapter of the thesis, Chapter 6, is devoted to the first application of the Gaussian fermionic phase-space method to a dynamical simulation of a multimode fermion-boson system. As a first-principles approach, the method provides benchmarking of approximate approaches and can be used to validate dynamical probes for characterizing strongly correlated phases of fermionic systems. We have applied the Gaussian phase-space method to the problem of molecular dissociation in the simplest uniform case and demonstrated a successful treatment of large molecular condensates containing up to 10^4 molecules and 10^3 distinct atomic modes. Simulating a system in such a large Hilbert space would be impossible using a more traditional exact numerical method based on the number-state representation. Our simulations reveal, in the long-time limit, significant deviations of atom-molecule and molecule-molecule correlations from the predictions of approximate pairing mean-field theories, as well as significant departures of atom-atom correlations from Wick's factorisation scheme. We have examined the accuracy and limitations of the fermionic phase-space results by comparison with the number-state calculations for small-size systems and via the analysis of conserved quantities. Future extensions of this work will have to incorporate spatial inhomogeneity and s-wave scattering interactions in order to enable first-principles dynamical simulations of a broader class of fermionic systems of current experimental interest. To this end, we have implemented a phase-space treatment of the Fermi-Hubbard model and present some exploratory simulations of Hubbard dynamics.

•Jun 1, 2011•0 citations

Higher Order Correlations in Ultracold Quantum Gases

Andrew G. Truscott, R. G. Dall, Sean S. Hodgman +5 more

One of the seminal advances in quantum optics was the understanding that a quantised description of ensembles of photons is best characterised by correlation functions. Correlations are also a fundamental property of matter waves, and the single wavefunction that describes a Bose-Einstein condensate (BEC) is in principle characterised by long range coherence to all orders (i.e. a universal correlation value of unity). Here we measure the higher order correlation properties of ultra-cold matter waves and use them to probe the coherence of the gas.

•Jan 1, 2011•0 citations
The field of atom optics has progressed rapidly over the past 20 years since the realisation of Bose-Einstein condensation, such that the wave behaviour of atomic gases is now routinely demonstrated. Furthermore, the study of quantum atom optics, which goes beyond a ‘mean-field’ description of quantum systems to consider the behaviour of single particles, has demonstrated both the similarities between photons and massive species, and their differences as a result of the internal structure and external interactions of atoms. An important class of observable quantities which allow such effects to be measured are nth order correlation functions, which can be interpreted as a result of either particle or wave behaviour. These functions provide a statistical description of fluctuations in n-tuples of particles in a source, which rigorously defines concepts such as coherence. The quantum statistics of a Bose-Einstein condensate should be the same as that for an optical laser, while an ideal thermal Bose gas matches the behaviour of incoherent light. However, correlation measurements can also be used to quantify the influence of interactions, dimensionality, confining potentials and waveguides, and the difference in quantum statistics between fermions and bosons, which illustrates the rich range of behaviour exhibited by atomic gases. In this thesis, several aspects of quantum atom optics are explored with experiments using ultracold metastable helium, a species with the unique advantage of facilitating simple single-atom detection with high resolution, while still allowing Bose-Einstein condensates to be formed. The coherence of atomic systems is shown to be maintained when outcoupled as pulsed atom lasers, and the long-range order characteristic of Bose-Einstein condensates is demonstrated to third order for the first time. Conversely, thermal bunching is observed for a variety of atomic systems, including the measurement of correlation functions up to sixth order with near-ideal interference contrast. These results clearly demonstrate the correspondence between the quantum statistics of photons and atoms as was formalised by Glauber, as well as confirming the validity of applying Wick’s theorem to simplify the statistics of atomic gases. Correlation functions are also shown to be an ideal tool to probe the quantum state of an ultracold gas, and were used to observe the phenomenon of transverse condensation in an elongated Bose gas, as well as characterise the mode occupancy of matter waves guided by an optical potential. Ultracold metastable helium is also suitable for exploring other fundamental topics in quantum optics such particle/wave duality. The notion of complementarity stimulated long running philosophical discussions about how apparently mutually exclusive behaviours can coexist, which culminated in Wheeler devising his famous ‘delayed choice’ gedankenexperiment. A proposed experimental method to realise Wheeler’s experiment with ultracold atoms is discussed, and preliminary measurements presented which indicate that the completion of this experiment could be achieved in the near future. Not only is this of interest in its own right, but the implementation of this experiment has also developed techniques which may enable further studies in quantum atom optics such as investigations of the Hong-Ou-Mandel effect and quantum entanglement with massive particles.
Trapped gases of ultracold metastable helium atoms are a unique experimental sys- tem. The trapped cloud’s low temperatures, the ability to selectively trap and ma- nipulate individual atomic states and the isolation provided in a vacuum chamber are all conducive to the measurement of precision atomic parameters, such as atomic transition rates. Due to it’s atomic structure helium - the simplest multi-electron atom - is a favourite test-bed for precision QED theoretical calculations compared to experimentally determined parameters. This thesis reports on a number of tran- sition rates measured for the first time with high accuracy, including the first excited metastable state lifetime, found to be 7870(510)s, the longest of any neutral atomic species yet measured. Transition rates from the 23P level to the ground state were also measured for the first time and found to be in excellent agreement with theory. Further cooling of helium produces a Bose-Einstein condensate (BEC), where all atoms are in an identical quantum state, the analogue of an optical laser. One par- ticularly interesting property a BEC posesses is long-range coherence to all orders, meaning all component particles are described by a single wavefunction. While first order coherence is measured in an interference experiment like Young’s double slit, higher order coherence is the ability for correlations to exist between groups of two, three or more particles, quantified by the measurement of correlation functions. Prior to the work in this thesis correlation functions for atoms had only been measured for second order. Here we develop a new technique which we use to show that a BEC is coherent to second and third order to 0.1% accuracy, compared to a thermal cloud which we show is incoherent. At small inter-particle spacings, there is an enhanced probability of measuring double and triple events in the thermal cloud (termed bunching). A drawback of all previous atomic correlation measurements is that the small de-Broglie wavelengths compared to the detector resolution leads to a significant reduction in the measured bunching amplitudes compared to theory. By altering our trapping configuration and temperature we are able to measure a two-particle bunching amplitude which is 88% of the theoretical maximum. This system also allowed the measurement of correlations up to 5th order in thermal gases. The near ideal bunching allowed us to demonstrate perturbations to the correlation functions due to the 1D nature of the system. These advances should lead to correlation measurements being used as a probe to characterise more exotic system properties such as low dimensionality, engineered quantum states and paticle pairing. Finally, a waveguide was created using a dipole laser beam and used to guide atoms in analogy to an optical laser in a fibre. Guided ‘atom lasers’ are likely to be important components for practical devices such as precision sensors. We demonstrate that a guided atom laser has a gaussian profile matching the lowest transverse mode of the waveguide and is first and second order coherent. In contrast guided thermal atoms show matter-wave speckle and are incoherent.
Trapped ultracold gases of metastable helium atoms provide a unique experimental system. The high internal energy enables electronic detection of single atoms. This thesis presents a number of experimental studies using metastable helium. Ionization rates in a mixture of metastable helium and rubidium were measured. Spin polarisation of the system has been shown to result in suppression of Penning ionization of rubidium by metastable helium atoms, suppressed by at least a hundred fold. This demonstration is a promising step towards the first creation of a binary BEC comprising atoms in both ground and excited states. The other experiments presented are mainly concerned with Hanbury Brown-Twiss and Higher order correlations. Single atom detection for metastable helium empowers experimenters to acquire spatial and temporal information, and to obtain full 3D reconstruction for released atomic clouds. Measurements on incoherent boson sources show bunching of particles. This enhancement to probability of joint detection events for two or more particles within short separations is in contrast to the uniform distribution of a coherent state, as measured for a Bose-Einstein condensate or an atom laser. By manipulating correlation length at the detector we were able to demonstrate the first atomic measurement of spatial three-particle correlation, and the results show significant improvement over previously reported values. Furthermore, by using a different trap geometry, it was possible perform measurement of atomic correlation functions to the 6th order, and have observed near ideal correlation functions to the 5th order, demonstrating enhancement for multi-particle detection probability consistent with the prediction of Wick's theorem. Correlations are then exploited to monitor the evolution of coherence property during the formation of a Bose-Einstein condensate. The experimental results are consistent with the existence of a quasi-condensation stage during the system's evolution from an incoherent thermal cloud towards a condensate with long range order. Two cases of mixing processes leading to the production of paired atom beams were Studied. In one case, correlation measurement provided the first higher order test of coherence of amplified matter waves. Coherence properties of matter waves generated via Bose stimulation are critical for active atom optical devices. Previously, coherence properties of amplified matter waves have only been demonstrated to first order by interference fringes. In the second case, a novel mixing process previously unknown was observed. Single atom counting is used to show number difference squeezing between opposite modes. Both processes studied hold potential of providing simple and elegant ways of producing pairs of coherent, sub-Poissonian number difference, and even entangled modes of atomic beams. Finally, physics of lower dimensions was studied. Observation was made of the phenomenon of two-step condensation in a quasi-1D system, where the gas condenses in the tightly confining transverse directions, yet remain thermal in the longitudinal direction. The lack of long-rang coherence of the system is revealed with correlations. Furthermore, an attempt was made to identify the Berezinskii-Kosterlitz-Thouless (BKT) transition.
This thesis presents two experiments on ultracold gases of metastable Helium that constitute the extension, to matter waves, of experiments that have been fundamental for the development of quantum optics. Both experiments have been realized by using a single atom detector, that allows one to reconstruct the position of the atoms in three dimensions. In the first experiment we directly compared the two-body correlation function for a cold cloud of identical fermions and for a cold cloud of identical bosons at the same temperature issued from the same experimental apparatus. Since bosons and fermions obey different quantum statistics, the two-body correlation functions are different: identical bosons tend to be detected bunched in pairs, while identical fermions tend to antibunch because of the Pauli exclusion principle. In the second experiment we studied the correlation between pairs of bosonic atoms generated in the collision of two Bose-Einstein condensates. The measurement of the correlation function allows us to demonstrate that atoms flying back to back in the centre of mass frame are correlated in pairs. Furthermore the observation of a Hanbury Brown Twiss correlation between atoms with collinear velocity demonstrates that our system cannot be interpreted in terms of classical mechanics, but that the bosonic statistics plays a crucial role. A new version of the experiment will allow us to measure the angular dependence of the population of the scattering modes and the number difference squeezing between two correlated modes.
Here we utilize the single-atom detection capability of metastable helium to measure the second-order and third-order correlation functions for ensembles of ultracold atoms. We then extend these measurements to characterize the quantum statistics of atoms guided in a dipole potential. By appropriately loading atoms into the guide we are able to populate a selected number of guided modes, ranging from the majority of atoms in the lowest order mode (a BEC), to multi-mode guiding (equivalent to a thermal source). The guided BEC was characterised by a smooth gaussian transverse spatial profile, and a second-order correlation value of unity consistent with a coherent source. For multi-mode guiding, the matter-wave equivalent of speckle was observed. Furthermore, at short arrival times, the second-order correlation function was greater than unity, corresponding to atom bunching characteristic of an incoherent (thermal) source.
Abstract The measurement and characterisation of correlation functions has recently become one of the central themes in the studies of ultracold quantum gases. By probing complex many-body states of these interacting systems, correlation functions facilitate the most in-depth understanding of the underlying physics, not accessible through simple density profile measurements. In this thesis, we study the dynamics of second-order correlation functions for atoms created in pair-production processes such as molecular dissociation and atomic four-wave mixing. More specifically, in Chapter 3 we analyse the dynamics of correlated atom pairs created via controlled dissociation of a Bose-Einstein condensate of diatomic molecules. The atomic constituents can be either a pair of bosonic or fermionic atoms. The process provides a matter-wave analog of parametric down-conversion with photons, which was pivotal in the advancement of quantum optics by enabling experimental demonstrations of the famous Einstein-Podolsky-Rosen paradox and violations of a classical Bell inequality. The atom-optics analogues of parametric down-conversion make it possible to envisage similar demonstrations using ensembles of massive particles in quantum gas regimes. In the case of fermionic constituents, molecular dissociation offers the possibility of a new paradigm in fermionic quantum-atom optics. By aiming at experimentally realistic modelling, we examine the role of spatial inhomogeneity of harmonically trapped molecular condensates on the strength and the shape of atom-atom correlations. Using the undepleted molecular-field approximation, we obtain explicit analytic results for the short-time asymptotic behaviour of the second-order correlation functions and for relative number squeezing between the dissociated atoms in one, two, and three spatial dimensions. Comparisons with the numerical results, which incorporate the molecular depletion and s-wave scattering interactions, show that the analytic approaches employed here capture the main underlying physics and provide useful insights into the dynamics of dissociation for conversion efficiencies up to 10%. The results show explicitly how the strength of atom-atom correlations and relative number squeezing degrade with the reduction of the size of the molecular condensate. In Chapter 4, we study highly anisotropic molecular condensates in order to quantify the effects of bosonic stimulation and fermionic Pauli blocking on the dissociation dynamics. We show that the difference in quantum statistics of the atomic constituent is manifest as complementary geometric structures in the density profiles of the dissociated atoms. Atomic bosons are preferentially emitted along the long axis of the molecular condensate due to bosonic stimulation, while atomic fermions are preferentially emitted along the short axis due to Pauli blocking. This anisotropy potentially simplifies the measurement of correlations between the atoms through relative number squeezing. In Chapter 5 we apply our analytic approaches to a related problem of atomic four-wave mixing and analyze atom-atom correlations in the s-wave scattering halo of two colliding condensates. The results in the short-time limit are in agreement with the first-principles simulations using the positive-P representation and provide analytic insights into the experimental observations of Perrin et al. [Phys. Rev. Lett. 99, 150405 2007]. The final chapter of the thesis, Chapter 6, is devoted to the first application of the Gaussian fermionic phase-space method to a dynamical simulation of a multimode fermion-boson system. As a first-principles approach, the method provides benchmarking of approximate approaches and can be used to validate dynamical probes for characterizing strongly correlated phases of fermionic systems. We have applied the Gaussian phase-space method to the problem of molecular dissociation in the simplest uniform case and demonstrated a successful treatment of large molecular condensates containing up to 10^4 molecules and 10^3 distinct atomic modes. Simulating a system in such a large Hilbert space would be impossible using a more traditional exact numerical method based on the number-state representation. Our simulations reveal, in the long-time limit, significant deviations of atom-molecule and molecule-molecule correlations from the predictions of approximate pairing mean-field theories, as well as significant departures of atom-atom correlations from Wick's factorisation scheme. We have examined the accuracy and limitations of the fermionic phase-space results by comparison with the number-state calculations for small-size systems and via the analysis of conserved quantities. Future extensions of this work will have to incorporate spatial inhomogeneity and s-wave scattering interactions in order to enable first-principles dynamical simulations of a broader class of fermionic systems of current experimental interest. To this end, we have implemented a phase-space treatment of the Fermi-Hubbard model and present some exploratory simulations of Hubbard dynamics.
One of the seminal advances in quantum optics was the understanding that a quantised description of ensembles of photons is best characterised by correlation functions. Correlations are also a fundamental property of matter waves, and the single wavefunction that describes a Bose-Einstein condensate (BEC) is in principle characterised by long range coherence to all orders (i.e. a universal correlation value of unity). Here we measure the higher order correlation properties of ultra-cold matter waves and use them to probe the coherence of the gas.