Trapped gases of ultracold metastable helium atoms are a unique experimental sys- tem. The trapped cloud’s low temperatures, the ability to selectively trap and ma- nipulate individual atomic states and the isolation provided in a vacuum chamber are all conducive to the measurement of precision atomic parameters, such as atomic transition rates. Due to it’s atomic structure helium - the simplest multi-electron atom - is a favourite test-bed for precision QED theoretical calculations compared to experimentally determined parameters. This thesis reports on a number of tran- sition rates measured for the first time with high accuracy, including the first excited metastable state lifetime, found to be 7870(510)s, the longest of any neutral atomic species yet measured. Transition rates from the 23P level to the ground state were also measured for the first time and found to be in excellent agreement with theory. Further cooling of helium produces a Bose-Einstein condensate (BEC), where all atoms are in an identical quantum state, the analogue of an optical laser. One par- ticularly interesting property a BEC posesses is long-range coherence to all orders, meaning all component particles are described by a single wavefunction. While first order coherence is measured in an interference experiment like Young’s double slit, higher order coherence is the ability for correlations to exist between groups of two, three or more particles, quantified by the measurement of correlation functions. Prior to the work in this thesis correlation functions for atoms had only been measured for second order. Here we develop a new technique which we use to show that a BEC is coherent to second and third order to 0.1% accuracy, compared to a thermal cloud which we show is incoherent. At small inter-particle spacings, there is an enhanced probability of measuring double and triple events in the thermal cloud (termed bunching). A drawback of all previous atomic correlation measurements is that the small de-Broglie wavelengths compared to the detector resolution leads to a significant reduction in the measured bunching amplitudes compared to theory. By altering our trapping configuration and temperature we are able to measure a two-particle bunching amplitude which is 88% of the theoretical maximum. This system also allowed the measurement of correlations up to 5th order in thermal gases. The near ideal bunching allowed us to demonstrate perturbations to the correlation functions due to the 1D nature of the system. These advances should lead to correlation measurements being used as a probe to characterise more exotic system properties such as low dimensionality, engineered quantum states and paticle pairing. Finally, a waveguide was created using a dipole laser beam and used to guide atoms in analogy to an optical laser in a fibre. Guided ‘atom lasers’ are likely to be important components for practical devices such as precision sensors. We demonstrate that a guided atom laser has a gaussian profile matching the lowest transverse mode of the waveguide and is first and second order coherent. In contrast guided thermal atoms show matter-wave speckle and are incoherent.
Trapped gases of ultracold metastable helium atoms are a unique experimental sys- tem. The trapped cloud’s low temperatures, the ability to selectively trap and ma- nipulate individual atomic states and the isolation provided in a vacuum chamber are all conducive to the measurement of precision atomic parameters, such as atomic transition rates. Due to it’s atomic structure helium - the simplest multi-electron atom - is a favourite test-bed for precision QED theoretical calculations compared to experimentally determined parameters. This thesis reports on a number of tran- sition rates measured for the first time with high accuracy, including the first excited metastable state lifetime, found to be 7870(510)s, the longest of any neutral atomic species yet measured. Transition rates from the 23P level to the ground state were also measured for the first time and found to be in excellent agreement with theory. Further cooling of helium produces a Bose-Einstein condensate (BEC), where all atoms are in an identical quantum state, the analogue of an optical laser. One par- ticularly interesting property a BEC posesses is long-range coherence to all orders, meaning all component particles are described by a single wavefunction. While first order coherence is measured in an interference experiment like Young’s double slit, higher order coherence is the ability for correlations to exist between groups of two, three or more particles, quantified by the measurement of correlation functions. Prior to the work in this thesis correlation functions for atoms had only been measured for second order. Here we develop a new technique which we use to show that a BEC is coherent to second and third order to 0.1% accuracy, compared to a thermal cloud which we show is incoherent. At small inter-particle spacings, there is an enhanced probability of measuring double and triple events in the thermal cloud (termed bunching). A drawback of all previous atomic correlation measurements is that the small de-Broglie wavelengths compared to the detector resolution leads to a significant reduction in the measured bunching amplitudes compared to theory. By altering our trapping configuration and temperature we are able to measure a two-particle bunching amplitude which is 88% of the theoretical maximum. This system also allowed the measurement of correlations up to 5th order in thermal gases. The near ideal bunching allowed us to demonstrate perturbations to the correlation functions due to the 1D nature of the system. These advances should lead to correlation measurements being used as a probe to characterise more exotic system properties such as low dimensionality, engineered quantum states and paticle pairing. Finally, a waveguide was created using a dipole laser beam and used to guide atoms in analogy to an optical laser in a fibre. Guided ‘atom lasers’ are likely to be important components for practical devices such as precision sensors. We demonstrate that a guided atom laser has a gaussian profile matching the lowest transverse mode of the waveguide and is first and second order coherent. In contrast guided thermal atoms show matter-wave speckle and are incoherent.
Trapped ultracold gases of metastable helium atoms provide a unique experimental system. The high internal energy enables electronic detection of single atoms. This thesis presents a number of experimental studies using metastable helium. Ionization rates in a mixture of metastable helium and rubidium were measured. Spin polarisation of the system has been shown to result in suppression of Penning ionization of rubidium by metastable helium atoms, suppressed by at least a hundred fold. This demonstration is a promising step towards the first creation of a binary BEC comprising atoms in both ground and excited states. The other experiments presented are mainly concerned with Hanbury Brown-Twiss and Higher order correlations. Single atom detection for metastable helium empowers experimenters to acquire spatial and temporal information, and to obtain full 3D reconstruction for released atomic clouds. Measurements on incoherent boson sources show bunching of particles. This enhancement to probability of joint detection events for two or more particles within short separations is in contrast to the uniform distribution of a coherent state, as measured for a Bose-Einstein condensate or an atom laser. By manipulating correlation length at the detector we were able to demonstrate the first atomic measurement of spatial three-particle correlation, and the results show significant improvement over previously reported values. Furthermore, by using a different trap geometry, it was possible perform measurement of atomic correlation functions to the 6th order, and have observed near ideal correlation functions to the 5th order, demonstrating enhancement for multi-particle detection probability consistent with the prediction of Wick's theorem. Correlations are then exploited to monitor the evolution of coherence property during the formation of a Bose-Einstein condensate. The experimental results are consistent with the existence of a quasi-condensation stage during the system's evolution from an incoherent thermal cloud towards a condensate with long range order. Two cases of mixing processes leading to the production of paired atom beams were Studied. In one case, correlation measurement provided the first higher order test of coherence of amplified matter waves. Coherence properties of matter waves generated via Bose stimulation are critical for active atom optical devices. Previously, coherence properties of amplified matter waves have only been demonstrated to first order by interference fringes. In the second case, a novel mixing process previously unknown was observed. Single atom counting is used to show number difference squeezing between opposite modes. Both processes studied hold potential of providing simple and elegant ways of producing pairs of coherent, sub-Poissonian number difference, and even entangled modes of atomic beams. Finally, physics of lower dimensions was studied. Observation was made of the phenomenon of two-step condensation in a quasi-1D system, where the gas condenses in the tightly confining transverse directions, yet remain thermal in the longitudinal direction. The lack of long-rang coherence of the system is revealed with correlations. Furthermore, an attempt was made to identify the Berezinskii-Kosterlitz-Thouless (BKT) transition.
The field of atom optics has progressed rapidly over the past 20 years since the realisation of Bose-Einstein condensation, such that the wave behaviour of atomic gases is now routinely demonstrated. Furthermore, the study of quantum atom optics, which goes beyond a ‘mean-field’ description of quantum systems to consider the behaviour of single particles, has demonstrated both the similarities between photons and massive species, and their differences as a result of the internal structure and external interactions of atoms. An important class of observable quantities which allow such effects to be measured are nth order correlation functions, which can be interpreted as a result of either particle or wave behaviour. These functions provide a statistical description of fluctuations in n-tuples of particles in a source, which rigorously defines concepts such as coherence. The quantum statistics of a Bose-Einstein condensate should be the same as that for an optical laser, while an ideal thermal Bose gas matches the behaviour of incoherent light. However, correlation measurements can also be used to quantify the influence of interactions, dimensionality, confining potentials and waveguides, and the difference in quantum statistics between fermions and bosons, which illustrates the rich range of behaviour exhibited by atomic gases. In this thesis, several aspects of quantum atom optics are explored with experiments using ultracold metastable helium, a species with the unique advantage of facilitating simple single-atom detection with high resolution, while still allowing Bose-Einstein condensates to be formed. The coherence of atomic systems is shown to be maintained when outcoupled as pulsed atom lasers, and the long-range order characteristic of Bose-Einstein condensates is demonstrated to third order for the first time. Conversely, thermal bunching is observed for a variety of atomic systems, including the measurement of correlation functions up to sixth order with near-ideal interference contrast. These results clearly demonstrate the correspondence between the quantum statistics of photons and atoms as was formalised by Glauber, as well as confirming the validity of applying Wick’s theorem to simplify the statistics of atomic gases. Correlation functions are also shown to be an ideal tool to probe the quantum state of an ultracold gas, and were used to observe the phenomenon of transverse condensation in an elongated Bose gas, as well as characterise the mode occupancy of matter waves guided by an optical potential. Ultracold metastable helium is also suitable for exploring other fundamental topics in quantum optics such particle/wave duality. The notion of complementarity stimulated long running philosophical discussions about how apparently mutually exclusive behaviours can coexist, which culminated in Wheeler devising his famous ‘delayed choice’ gedankenexperiment. A proposed experimental method to realise Wheeler’s experiment with ultracold atoms is discussed, and preliminary measurements presented which indicate that the completion of this experiment could be achieved in the near future. Not only is this of interest in its own right, but the implementation of this experiment has also developed techniques which may enable further studies in quantum atom optics such as investigations of the Hong-Ou-Mandel effect and quantum entanglement with massive particles.
This thesis presents two experiments on ultracold gases of metastable Helium that constitute the extension, to matter waves, of experiments that have been fundamental for the development of quantum optics. Both experiments have been realized by using a single atom detector, that allows one to reconstruct the position of the atoms in three dimensions. In the first experiment we directly compared the two-body correlation function for a cold cloud of identical fermions and for a cold cloud of identical bosons at the same temperature issued from the same experimental apparatus. Since bosons and fermions obey different quantum statistics, the two-body correlation functions are different: identical bosons tend to be detected bunched in pairs, while identical fermions tend to antibunch because of the Pauli exclusion principle. In the second experiment we studied the correlation between pairs of bosonic atoms generated in the collision of two Bose-Einstein condensates. The measurement of the correlation function allows us to demonstrate that atoms flying back to back in the centre of mass frame are correlated in pairs. Furthermore the observation of a Hanbury Brown Twiss correlation between atoms with collinear velocity demonstrates that our system cannot be interpreted in terms of classical mechanics, but that the bosonic statistics plays a crucial role. A new version of the experiment will allow us to measure the angular dependence of the population of the scattering modes and the number difference squeezing between two correlated modes.
Here we utilize the single-atom detection capability of metastable helium to measure the second-order and third-order correlation functions for ensembles of ultracold atoms. We then extend these measurements to characterize the quantum statistics of atoms guided in a dipole potential. By appropriately loading atoms into the guide we are able to populate a selected number of guided modes, ranging from the majority of atoms in the lowest order mode (a BEC), to multi-mode guiding (equivalent to a thermal source). The guided BEC was characterised by a smooth gaussian transverse spatial profile, and a second-order correlation value of unity consistent with a coherent source. For multi-mode guiding, the matter-wave equivalent of speckle was observed. Furthermore, at short arrival times, the second-order correlation function was greater than unity, corresponding to atom bunching characteristic of an incoherent (thermal) source.
Since the achievement of Bose-Einstein condensation (BEC), the progress in matterwave \nphysics has been immense. Among the many recent achievements there is \nthe miniaturization of atom traps, demonstration of the superfluid-Mott insulator \nquantum-phase transition in optical lattices and the experimental demonstration of \nthe BEC-BCS crossover in ultra-cold gases. \nMiniaturization of atom traps using micro-structured wires on a chip is one important \nstep towards an on-chip cold-atom device. These so-called \\atom chips" provide \nhigh control and versatility for trapping and guiding the ultra-cold atomic clouds. \nParticularly interesting is the use of these microchips to build mesoscopic devices \nfor cold atomic clouds as, for instance, in the case of an atom-cloud interferometer. \nHowever, these mesoscopic devices require coherent transport of the atom cloud. A \ngeneral method to treat decoherence due to current fluctuations in multi-wire atomchip \ntraps is presented in the rst part of this thesis. The decoherence rate Γ shows a \nstrong dependence on the distance between the wire and the atom cloud, r0, scaling \nas Γ ~ r-4 0 for a single atom waveguide. Considering an interferometer device, a \nstrong dependence of the decoherence rate on the trap geometry is found. \n \nStudying many-body eects in ultra-cold quantum gases is another important \nresearch eld. Experiments using ultra-cold quantum gases in optical lattices have \ndemonstrated the superuid-Mott insulator quantum phase transition and manybody \nentanglement. Optical lattices are based on a periodic modulation of the light \nintensity, generated by retro-reected laser beams. Correlations of the atomic cloud \nbetween dierent lattice sites of the optical lattice play a central role in these manybody \nexperiments. The dierent phases of the superuid-Mott insulator system can \nbe characterized by the dierent behavior of the inter-lattice site correlations. There \nare several numerical methods such as Quantum Monte Carlo (QMC) simulations, \nDensity Matrix Renormalization Group (DMRG) simulations, exact-diagonalization, \nor the Gutzwiller ansatz, to investigate the dynamics of an ultra-cold gas in an optical \nlattice theoretically. The Gutzwiller method, corresponding to the mean-eld solution, \nallows for the treatment of large lattice sizes. Mean-eld approaches have proven \nto be very useful to describe many-body physics. However, diculties arise in the correct \ndescription of the behavior of the decay of inter-lattice site correlations. Based on \nthe Gutzwiller approach, we have developed a method which allows the successive inclusion \nof inter-lattice site correlations. Comparing the results for the particle-number \nuctuations and the correlation function obtained from pure Gutzwiller calculations, \nto calculations which perturbatively include short-range correlations and calculations \n \nusing \\quasi-exact methods", showed a considerable improvement relative to the pure \nGutzwiller results due to the inclusion of short-range correlations. \nMany-body eects do not only arise in periodic potentials, but become increasingly \nimportant at ultra-low temperatures. The formation of Bose-Einstein condensates \nrequires an overlap of the atom wavefunctions and, hence, the formation of \na single condensate wavefunction. Another example of a many-body state is the \nsuperuid-BCS state, commonly used as a description of superconductivity. Here, \nfermions in dierent hyperne states form Cooper pairs. Experiments with ultracold \nquantum gases enable a variation of the interparticle interaction, e.g. , by using \na Feshbach resonance. Using Feshbach resonances to tune the interaction strength \nhas enabled the experimental observation of the crossover from a superuid-BCS \nstate to a Bose-Einstein condensate of molecules. A useful way to characterize the \ndierent states of ultra-cold quantum gases is to investigate the particle-number uctuations. \nIn this thesis we suggest to divide the atomic cloud into bins and consider \nthe atom-number uctuations in these bins. We calculate the full counting statistics \nfor dierent physical systems of ultra-cold gases (e.g. bosonic gases, fermionic gases, \nand spin mixtures). In particular, we consider the BCS-state as a rst trial example \nto show that there is a strong variation in the particle-number statistics at the \ncrossover from a superuid-BCS state to a Bose-Einstein condensate of molecules.
Exited atoms may relax to the ground state by radiative decay, a process which is usually very fast (of order nanoseconds). However, quantum-mechanical selection rules can prevent such rapid decay, in which case these "metastable" states can have lifetimes of order seconds or longer. In this Letter, we determine experimentally the lifetime of the longest-lived neutral atomic state-the first excited state of helium (the 2(3)S1 metastable state)-to the highest accuracy yet measured. We use laser cooling and magnetic trapping to isolate a cloud of metastable helium (He*) atoms from their surrounding environment, and measure the decay rate to the ground 1(1)S0 state via extreme ultraviolet (XUV) photon emission. This is the first measurement using a virtually unperturbed ensemble of isolated helium atoms, and yields a value of 7870(510) seconds, in excellent agreement with the predictions of quantum electrodynamic theory.