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Quantum chaos in atom optics

M. B. d’Arcy

Published Jan 1, 2002• 2 citations
Publisher

Abstract

This thesis presents an account of experimental and numerical investigations of two quantum systems whose respective classical analogues are chaotic. These are the delta-kicked rotor, a paradigm in classical chaos theory, and the novel delta-kicked accelerator, created by application of a constant external acceleration or torque to the rotor. The experimental realisation of these systems has been achieved by the exposure of laser-cooled caesium atoms to approximate delta-kicks from a pulsed, high-intensity, vertical standing wave of laser light. Gravity’s effect on the atoms can be controlled by appropriate shifting of the profile of the standing wave. Numerical simulations of the systems are based on a diffractive model of the potential’s effect. Each system’s dynamics are characterised by the final form of the momentum distribution and the dependence of the atoms’ mean kinetic energy on the number and time period of the delta-kicks. The phenomena of dynamical localisation and quantum resonances in the delta-kicked rotor, which have no counterparts in the system’s classical analogue, are observed and investigated. Similar experiments on the delta-kicked accelerator reveal the striking phenomenon of the quantum accelerator mode, in which a large momentum is transferred to a substantial fraction of the atomic ensemble. This feature, absent in the system’s classical analogue, is characterised and an analytic explanation is presented. The effect on each quantum system of decoherence, introduced through spontaneous emission in the atoms, is examined and comparison is made with the results of classical simulations. While having little effect on the classical systems, the level of decoherence used is found to degrade quantum signatures of behaviour. Classical-like behaviour is, to some extent, restored, although significant quantum features remain. Possible applications of the quantum accelerator mode are discussed. These include use as a tool in atom optics and interferometry, a technique for measuring gravity, and a method of preparing atoms in a particular region of phase space. This may allow measurement of quantum phase space stability, and hence investigation of quantum chaos and quantum-classical correspondence.

DOI
10.5287/ora-j5e2q8pjp

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This thesis presents an account of experimental and numerical investigations of two quantum systems whose respective classical analogues are chaotic. These are the delta-kicked rotor, a paradigm in classical chaos theory, and the novel delta-kicked accelerator, created by application of a constant external acceleration or torque to the rotor. The experimental realisation of these systems has been achieved by the exposure of laser-cooled caesium atoms to approximate delta-kicks from a pulsed, high-intensity, vertical standing wave of laser light. Gravity’s effect on the atoms can be controlled by appropriate shifting of the profile of the standing wave. Numerical simulations of the systems are based on a diffractive model of the potential’s effect. Each system’s dynamics are characterised by the final form of the momentum distribution and the dependence of the atoms’ mean kinetic energy on the number and time period of the delta-kicks. The phenomena of dynamical localisation and quantum resonances in the delta-kicked rotor, which have no counterparts in the system’s classical analogue, are observed and investigated. Similar experiments on the delta-kicked accelerator reveal the striking phenomenon of the quantum accelerator mode, in which a large momentum is transferred to a substantial fraction of the atomic ensemble. This feature, absent in the system’s classical analogue, is characterised and an analytic explanation is presented. The effect on each quantum system of decoherence, introduced through spontaneous emission in the atoms, is examined and comparison is made with the results of classical simulations. While having little effect on the classical systems, the level of decoherence used is found to degrade quantum signatures of behaviour. Classical-like behaviour is, to some extent, restored, although significant quantum features remain. Possible applications of the quantum accelerator mode are discussed. These include use as a tool in atom optics and interferometry, a technique for measuring gravity, and a method of preparing atoms in a particular region of phase space. This may allow measurement of quantum phase space stability, and hence investigation of quantum chaos and quantum-classical correspondence.
In this thesis we investigate quantum resonant effects in the atom-optical ὁ-kicked accelerator. Using Floquet analysis, we theoretically study the time evolution of quantum systems which have a classical counterpart that exhibits chaotic dynamics. We introduce quantum resonance and quantum antiresonance features of the quantum ὁ -kicked rotor by setting the pulse period to an integer multiple of the half-Talbot time. The model is generalised to the atom-optical ὁ -kicked accelerator by considering thermal alkali atoms subject to a periodically pulsed standing wave potential formed from counter-propagating laser beams. The dynamics of the momentum distribution is analysed by evaluating the momentum moments and momentum cumulants. We derive analytic solutions for these observables for the ultracold and thermal limiting cases, and observe fractional quantum resonant phenomena. Simulations have been developed to examine the time evolution for individual momentum eigenstates, which we use to construct a non-interacting finite temperature gas, based upon a Monte Carlo method. We investigate the temperature dependence of the ὁ-kicked rotor, neglecting gravitational effects, and show that the atomic dynamics is highly sensitive to the initial momentum width of the gas. A generalisation of the model to quantify the transition between the ultracold and thermal temperature regimes of the atom-optical ὁ -kicked accelerator is examined using linear regression analysis. High order quantum resonance features are found to be sensitive to the relative acceleration between the atomic gas and the pulsed optical standing wave. We assess the dependence of the ὁ -kicked accelerator upon gravitational acceleration, quantifying the width of the high order quantum resonance features, which we use to assess the prospect for precision measurement using a finite temperature gas.
We describe measurements of the mean energy of an ensemble of laser-cooled atoms in an atom optical system in which the cold atoms, falling freely under gravity, receive approximate delta-kicks from a pulsed standing wave of laser light. We call this system a "delta-kicked accelerator." Additionally, we can counteract the effect of gravity by appropriate shifting of the position of the standing wave, which restores the dynamics of the standard delta-kicked rotor. The presence of gravity (delta-kicked accelerator) yields quantum phenomena, quantum accelerator modes, which are markedly different from those in the case for which gravity is absent (delta-kicked rotor). Quantum accelerator modes result in a much higher rate of increase in the mean energy of the system than is found in its classical analog. When gravity is counteracted, the system exhibits the suppression of the momentum diffusion characteristic of dynamical localization. The effect of noise is examined and a comparison is made with simulations of both quantum-mechanical and classical versions of the system. We find that the introduction of noise results in the restoration of several signatures of classical behavior, although significant quantum features remain.
This thesis deals with an investigation of the chaotic dynamics of an atom optics δ-kicked rotor (AOKR) system, a paradigm of classical and quantum chaos. The AOKR rotor is realized by subjecting a Bose-Einstein condensate (BEC) of ⁸⁷Rb atoms to a periodic potential. The potential in the form of a standing wave, obtained from a far detuned laser beam is turned on and off periodically in time, producing short pulses (kicks) of laser light. For certain values of the period between the kicks, resonant effects known as quantum resonances are observed that are purely quantum effects. Quantum resonances have been examined in the AOKR for a series of kicks. For large number of kicks, the width of these resonances have been shown to become narrow. Higher order resonances corresponding to fractional Talbot times have been observed in the system. These quantum resonant effects have been found to depend sensitively on the initial velocity of the atoms. The first three primary resonances have been studied in detail, by measuring the momentum distribution and the kinetic energy of the atoms, for two and four kicks. A sinusoidal dependence of the energy on the initial momentum has been observed for two kicks. By increasing the number of kicks, the system becomes extremely sensitive to the initial momentum of the atoms. For four kicks, a more complex behavior is observed in the system energy. A scheme for investigating Loschmidt time reversal of chaotic dynamics of the atomic deBroglie waves have been described in the AOKR system. It has been demonstrated that the initial wave function of an ensemble of ultracold atoms is restored, after a series of delta-kicks in what is essentially a multiple beam interferometry experiment. During the process, the evolution of the system for a fraction of the atoms with a very small initial momentum is reversed, which results in a narrowing of the momentum distribution. It is hoped that the research presented in this thesis will significantly contribute to the understanding of the connection between the classical and quantum worlds.
This thesis investigates quantum transport in the energy space of two paradigm systems of quantum chaos theory. These are highly excited hydrogen atoms subject to a microwave field, and kicked atoms which mimic the delta-kicked rotor model. Both of these systems show a complex dynamical evolution arising from the interaction with an external time-periodic driving force. In particular two quantum phenomena, which have no counterpart on the classical level, are studied: the suppression of classical diffusion, known as dynamical localisation, and quantum resonances as a regime of enhanced transport for the delta-kicked rotor. The first part of the thesis provides new support for the quantitative analogy between energy transport in strongly driven highly excited atoms and particle transport in Anderson-localised solids. A comprehensive numerical analysis of the atomic ionisation rates shows that they obey a universal power-law distribution, in agreement with Anderson localisation theory. This is demonstrated for a one-dimensional model as well as for the real three-dimensional atom. We also discuss the implications of the universal decay-rate distributions for the asymptotic time-decay of the survival probability of the atoms. The second part of the thesis clarifies the effect of decoherence, induced by spontaneous emission, on the quantum resonances which have been observed in a recent experiment with delta-kicked atoms. Scaling laws are derived, based on a quasi-classical approximation of the quantum evolution. These laws describe the shape of the resonance peaks in the mean energy of an experimental ensemble of kicked atoms. Our analytical results match perfectly numerical computations and explain the initially surprising experimental observations. Furthermore, they open the door to the study of the competing effects of decoherence and chaos on the stability of the time evolution of kicked atoms. This stability may be characterised by the overlap of two identical initial states which are subject to different time evolutions. This overlap, called fidelity, is investigated in an experimentally accessible situation.
We discuss recent experimental and theoretical investigations of quantum dynamics in periodically kicked chaotic systems. These investigations are centred on a modified version of the classic δ-kicked rotor, as realized using laser-cooled caesium atoms. Dramatic phenomena, principally quantum accelerator modes, have been observed and these have inspired novel theoretical approaches to quantum chaos. The latter work has, in turn, prompted further experiments and the combined experimental and theoretical effort continues to lead to exciting advances in this field.
Scope and Method of Study: The purpose of this research was to experimentally study quantum dynamics of systems whose classical dynamics are chaotic. Quantum delta-kicked systems such as kicked rotor and kicked accelerator were used. The cold non condensed atoms were kicked first to realize the kicked accelerator. Among the objectives were the realization of resonances of the kicked accelerator and associated phenomena of quantum accelerator modes using a Bose-Einstein Condensation (BEC). One of the major achievements of the work in this thesis was the creation of the quantum delta-kicked rotor and its associated resonances to realize a quantum ratchet. The properties of the ratchet were studied in detail.