This thesis investigates quantum transport in the energy space of two paradigm systems of quantum chaos theory. These are highly excited hydrogen atoms subject to a microwave field, and kicked atoms which mimic the delta-kicked rotor model. Both of these systems show a complex dynamical evolution arising from the interaction with an external time-periodic driving force. In particular two quantum phenomena, which have no counterpart on the classical level, are studied: the suppression of classical diffusion, known as dynamical localisation, and quantum resonances as a regime of enhanced transport for the delta-kicked rotor. The first part of the thesis provides new support for the quantitative analogy between energy transport in strongly driven highly excited atoms and particle transport in Anderson-localised solids. A comprehensive numerical analysis of the atomic ionisation rates shows that they obey a universal power-law distribution, in agreement with Anderson localisation theory. This is demonstrated for a one-dimensional model as well as for the real three-dimensional atom. We also discuss the implications of the universal decay-rate distributions for the asymptotic time-decay of the survival probability of the atoms. The second part of the thesis clarifies the effect of decoherence, induced by spontaneous emission, on the quantum resonances which have been observed in a recent experiment with delta-kicked atoms. Scaling laws are derived, based on a quasi-classical approximation of the quantum evolution. These laws describe the shape of the resonance peaks in the mean energy of an experimental ensemble of kicked atoms. Our analytical results match perfectly numerical computations and explain the initially surprising experimental observations. Furthermore, they open the door to the study of the competing effects of decoherence and chaos on the stability of the time evolution of kicked atoms. This stability may be characterised by the overlap of two identical initial states which are subject to different time evolutions. This overlap, called fidelity, is investigated in an experimentally accessible situation.
This thesis investigates quantum transport in the energy space of two paradigm systems of quantum chaos theory. These are highly excited hydrogen atoms subject to a microwave field, and kicked atoms which mimic the delta-kicked rotor model. Both of these systems show a complex dynamical evolution arising from the interaction with an external time-periodic driving force. In particular two quantum phenomena, which have no counterpart on the classical level, are studied: the suppression of classical diffusion, known as dynamical localisation, and quantum resonances as a regime of enhanced transport for the delta-kicked rotor. The first part of the thesis provides new support for the quantitative analogy between energy transport in strongly driven highly excited atoms and particle transport in Anderson-localised solids. A comprehensive numerical analysis of the atomic ionisation rates shows that they obey a universal power-law distribution, in agreement with Anderson localisation theory. This is demonstrated for a one-dimensional model as well as for the real three-dimensional atom. We also discuss the implications of the universal decay-rate distributions for the asymptotic time-decay of the survival probability of the atoms. The second part of the thesis clarifies the effect of decoherence, induced by spontaneous emission, on the quantum resonances which have been observed in a recent experiment with delta-kicked atoms. Scaling laws are derived, based on a quasi-classical approximation of the quantum evolution. These laws describe the shape of the resonance peaks in the mean energy of an experimental ensemble of kicked atoms. Our analytical results match perfectly numerical computations and explain the initially surprising experimental observations. Furthermore, they open the door to the study of the competing effects of decoherence and chaos on the stability of the time evolution of kicked atoms. This stability may be characterised by the overlap of two identical initial states which are subject to different time evolutions. This overlap, called fidelity, is investigated in an experimentally accessible situation.
This thesis presents an account of experimental and numerical investigations of two quantum systems whose respective classical analogues are chaotic. These are the delta-kicked rotor, a paradigm in classical chaos theory, and the novel delta-kicked accelerator, created by application of a constant external acceleration or torque to the rotor. The experimental realisation of these systems has been achieved by the exposure of laser-cooled caesium atoms to approximate delta-kicks from a pulsed, high-intensity, vertical standing wave of laser light. Gravity’s effect on the atoms can be controlled by appropriate shifting of the profile of the standing wave. Numerical simulations of the systems are based on a diffractive model of the potential’s effect. Each system’s dynamics are characterised by the final form of the momentum distribution and the dependence of the atoms’ mean kinetic energy on the number and time period of the delta-kicks. The phenomena of dynamical localisation and quantum resonances in the delta-kicked rotor, which have no counterparts in the system’s classical analogue, are observed and investigated. Similar experiments on the delta-kicked accelerator reveal the striking phenomenon of the quantum accelerator mode, in which a large momentum is transferred to a substantial fraction of the atomic ensemble. This feature, absent in the system’s classical analogue, is characterised and an analytic explanation is presented. The effect on each quantum system of decoherence, introduced through spontaneous emission in the atoms, is examined and comparison is made with the results of classical simulations. While having little effect on the classical systems, the level of decoherence used is found to degrade quantum signatures of behaviour. Classical-like behaviour is, to some extent, restored, although significant quantum features remain. Possible applications of the quantum accelerator mode are discussed. These include use as a tool in atom optics and interferometry, a technique for measuring gravity, and a method of preparing atoms in a particular region of phase space. This may allow measurement of quantum phase space stability, and hence investigation of quantum chaos and quantum-classical correspondence.
New experimental results are presented for short-pulse microwave ionization of highly excited hydrogen atoms. A comparison of these results with quantum numerical computations and analytical predictions provides for the first time experimentally grounded evidence of the localization phenomenon that leads to the suppression of the quantum version of the chaotic diffusion in action space occurring in the classical limit. The onset of chaotic motion in externally driven classical systems is a key problem in nonlinear dynamics that is now well understood in its essential aspects. In many physically interesting cases, as the perturbation strength increases beyond some critical value, the system starts absorbing energy in a diffusive way. The question whether “diffusive” excitation processes can take place also in externally driven quantum systems is then a very interesting one for the physics of atoms and molecules in external electromagnetic fields. This is a deep question involving the nature and the validity of the quasiclassical approximation when the underlying classical dynamics is chaotic. The question of “quantum diffusion” was first addressed in a simple model system, the kicked rotator. It was chosen because the features of classical chaos in it were relatively clean and well understood. Besides that, the numerical simulation of its quantum dynamics could be easily accomplished. The major indication of this model was that quantum mechanics suppresses the classical chaotic diffusion in action via a destructive interference effect similar to that responsible for the Anderson localization well known in condensed matter physics.
The kicked rotor provides a simple yet powerful model for introducing many of the central concepts of classical and quantum chaos. Despite its apparent simplicity, it exhibits rich dynamical behavior and has found applications across a wide range of fields, including atomic and optical physics, condensed matter physics, and emerging quantum technologies. This chapter begins by exploring foundational ideas using the kicked rotor as a unifying framework. We first discuss the transition from regular to chaotic motion in the classical system, and then introduce key quantum phenomena such as dynamical localization and quantum resonances. Special attention is devoted to the emergence of characteristic time scales and their role in the quantum-classical correspondence. To make these ideas more concrete, we also provide a brief overview of experimental realizations of the kicked rotor and its variants, illustrating how theoretical concepts are implemented in practice. In the second part of the chapter, we guide the reader toward more recent and advanced developments. Topics include near-resonant dynamics, topological features of kicked systems, the emergence of quantum dynamical phases inferred from classical transport properties, and extensions to non-Hermitian physics. We conclude with a discussion of open problems and future perspectives, outlining directions in which the kicked rotor continues to offer valuable insights.
The central theme of this thesis is the directed transport of cold atoms in optical lattices. Several methods for producing such an outcome are proposed, experimentally realised and characterised, in both dissipative and non-dissipative regimes. Accordingly, this thesis may be thought to be composed of two parts. The first section reports results of directed transport in non-dissipative optical lattices, where we used the atom optics realisation of the delta-kicked rotor (DKR) as a model system. Initial experiments performed on this system showed evidence of dynamical localisation, the signature of quantum chaos, and we exploited the presence of the momentum boundary (a barrier to diffusion arising from the approximation of delta-kicks with finite width impulses) to produce asymmetric momentum diffusion. Breaking the DKR system symmetries produced directed diffusion due to chaotic dynamics alone. We observed directed transport in a spatially symmetric system whenever temporal symmetry was broken, and also when the spatial and temporal symmetry of the DKR were simultaneously broken. We also report the first experimental evidence for a 'double-DKR', where experiments performed using a kick sequence composed of closely spaced pairs of kicks instead of single kicks caused significant alterations in the observed behaviour of the kicked rotor system. The origin of this new behaviour was explained in the framework of kick-to-kick correlations and our results were found to be in excellent agreement with numerical simulations. The second part of this thesis describes the realisation of a Brownian ratchet in a 3D dissipative lattice, where fluctuations between different potential surfaces acted as the source of noise. These fluctuations were rectified by the application of a periodic, bi-harmonic driving force, which broke the temporal symmetry of the system. Both current reversal and stochastic resonance behaviour characteristic of a Brownian ratchet were observed.
Quantum simulation is one of the most active trends in ultracold-atom physics. A quantum simulator is a system that mimics the dynamics of another system; the advantage being that the quantum simulator is simpler than the original, either from the experimental or the theoretical point of view (or both).The Anderson model is a paradigm for quantum disorder, originally introduced in the helm of solid-state physics; however, quantum solid-state disordered systems are very difficult to study experimentally, and even numerically (except in the one-dimensional case). The kicked rotor is a paradigm for classical and quantum Hamiltonian chaos, essentially because it is very easy to simulate it in a computer. Its quantum realization with ultracold atoms is also relatively simple, and is a “clean” (e.g. from decoherence) and controllable system. Amazingly, the quantum kicked rotor can be mathematically mapped onto the Anderson model. It is thus a quite subtle quantum simulator of the physics of disordered systems. In this talk I will describe a series of experiments we have performed in Lille taking advantage of the correspondence between disordered condensed matter systems and the atomic kicked rotor to investigate experimentally in great detail the Anderson metal-insulator transition. I will discuss the new possibilities opened by evolutions of this system, in particular by introducing nonlinearity via atom-atom interactions.
In this thesis we investigate quantum resonant effects in the atom-optical ὁ-kicked accelerator. Using Floquet analysis, we theoretically study the time evolution of quantum systems which have a classical counterpart that exhibits chaotic dynamics. We introduce quantum resonance and quantum antiresonance features of the quantum ὁ -kicked rotor by setting the pulse period to an integer multiple of the half-Talbot time. The model is generalised to the atom-optical ὁ -kicked accelerator by considering thermal alkali atoms subject to a periodically pulsed standing wave potential formed from counter-propagating laser beams. The dynamics of the momentum distribution is analysed by evaluating the momentum moments and momentum cumulants. We derive analytic solutions for these observables for the ultracold and thermal limiting cases, and observe fractional quantum resonant phenomena. Simulations have been developed to examine the time evolution for individual momentum eigenstates, which we use to construct a non-interacting finite temperature gas, based upon a Monte Carlo method. We investigate the temperature dependence of the ὁ-kicked rotor, neglecting gravitational effects, and show that the atomic dynamics is highly sensitive to the initial momentum width of the gas. A generalisation of the model to quantify the transition between the ultracold and thermal temperature regimes of the atom-optical ὁ -kicked accelerator is examined using linear regression analysis. High order quantum resonance features are found to be sensitive to the relative acceleration between the atomic gas and the pulsed optical standing wave. We assess the dependence of the ὁ -kicked accelerator upon gravitational acceleration, quantifying the width of the high order quantum resonance features, which we use to assess the prospect for precision measurement using a finite temperature gas.