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Optics Express

Lifetime assessment of RbN_3-filled MEMS atomic vapor cells with Al_2O_3 coating

Sylvain Karlen, J. Gobet, Thomas Overstolz, Jacques Haesler, Steve Lecomte

Published Jan 26, 2017• 67 citations
Publisher

Abstract

coated cells is a very promising approach for low-cost wafer-level fabrication. Here we present a detailed lifetime study of such cells. The rubidium consumption being the main identified cell failure mode, it is monitored with an novel image analysis technique and with high temperature long term aging tests.
DOI
10.1364/oe.25.002187

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The microfabricated alkali atomic vapor cells are essential for the chip scale quantum sensing instruments which provide a robust, simple platform for precision measurement for a quantum system. In order to solve the problems of difficult quantitative filling of alkali atoms and poor hermeticity in the fabricated process of the cells, the preparation of microfabricated alkali atomic vapor cells with good hermeticity is studied. The cells are fabricated by the microelectromechanical system (MEMS) technology. Rubidium (Rb) atomic vapor cells with nitrogen (N 2 ) as buffer gas are successfully obtained by photolysis of rubidium azide (RbN 3 ), which is confirmed by the presence of Rb vapor in the cells through absorption spectroscopy for the 5S 1/2 → 5P 3/2 and 5S 1/2 → 5P 1/2 transitions in Rb atoms at 780 nm and 795 nm. The influences of filling amount and baking temperature of RbN 3 solution on the hermeticity of the microfabricated atomic vapor cells are demonstrated. Also, the influences of filling amount of Rb atoms and temperature on the absorption spectrum intensities of Rb vapor in the cells are studied through a theoretical analysis. This research provides a reference for the design and preparation of high quality microfabricated alkali atomic vapor cells.
Compared with superconducting quantum interference devices, chip-scale atomic magnetometers using the wafer-level micro alkali vapor cells can be used more conveniently in the applications of geophysical mapping, health care and remote monitoring. Drastic wall collisions and decreased polarization lifetime are the main barriers for the performance of the chip-scale atomic magnetometers. In this study, OTS organic films coated on the inner surface of the micro vapor cells were used to suppress wall collisions and improve polarization lifetime of the alkali atoms in the micro cells. First of all, the fabrication process of wafer-level micro OTS coated vapor cells is introduced, the process is based on anodic bonding technology. Then the prepared wafer-level micro OTS coated vapor cells have been characterized by the water-contact angle test and measured in the micro-machined spin-exchange relaxation free(SERF) atomic magnetometers. Results show that the OTS coating is effective after anodic bonding from the water contact angle test. Results also indicate that the spin exchange relaxation free atomic magnetometer using the micro OTS-coated vapor cell can operate successfully.
We report on an experiment in which the fluorescence decay time of 5P levels of Rb atoms in a coated vapor cell exceeds several of milliseconds, many orders of magnitude longer than normal decay time of excited of rubidium atoms. We found that this peculiarly long - term decay is not exponential and can only be observed in a high quality coated cell with a long lifetime of optical pumped atoms on atomic ground-state sublevels. A numerical simulation based on a complete density matrix is presented. It supports the population pumping process through the ground-state sublevels of Rb atoms as the most plausible mechanism for the observed phenomenon and it consistently demonstrates all the relevant features of the experiment. The investigation can be used, for example, to explore the quality of a various anti-relaxation coatings used for the resonant cells.