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Physical Review A

Pump-probe spectroscopy of cold rubidium atoms in an integrating sphere

Wenli Wang, Richang Dong, Jianliao Deng, Yuzhu Wang

Published May 5, 2016• 0 citations
Publisher

Abstract

Absorption spectra of cold rubidium atoms in an integrating sphere under the influence of a diffuse laser field have been systematically investigated. A pronounced dispersionlike structure centered at the light-shifted pump frequency is observed with a subnatural linewidth. In particular, two clearly resolved absorption resonances on the $5{S}_{1/2}(F=2)\ensuremath{\rightarrow}5{P}_{3/2}({F}^{\ensuremath{'}}=3)$ transitions occur with variable probe beam intensity, which is consistent with our proposed theoretical model. Based on the two absorption resonances,we measure the dependence of light shifts, from which we can directly extract the effective Rabi frequency in a diffuse laser field, on the probe laser intensity, pump laser intensity, and pump laser detuning. Our work helps to identify the physical mechanisms behind these spectral features and is beneficial for studying the corresponding effect in a cold sample.

DOI
10.1103/physreva.93.052503

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Absorption spectra of cold rubidium atoms in an integrating sphere under the influence of a diffuse laser field have been systematically investigated. A pronounced dispersionlike structure centered at the light-shifted pump frequency is observed with a subnatural linewidth. In particular, two clearly resolved absorption resonances on the 5S1/2(F=2)\ensuremath→5P3/2(F\ensuremath′=3)5{S}_{1/2}(F=2)\ensuremath{\rightarrow}5{P}_{3/2}({F}^{\ensuremath{'}}=3)5S1/2​(F=2)\ensuremath→5P3/2​(F\ensuremath′=3) transitions occur with variable probe beam intensity, which is consistent with our proposed theoretical model. Based on the two absorption resonances,we measure the dependence of light shifts, from which we can directly extract the effective Rabi frequency in a diffuse laser field, on the probe laser intensity, pump laser intensity, and pump laser detuning. Our work helps to identify the physical mechanisms behind these spectral features and is beneficial for studying the corresponding effect in a cold sample.
We propose and demonstrate pump-probe spectroscopy of rubidium absorption that reveals the sub-Doppler hyperfine structure of the ${}^{5}{\mathrm{S}}_{1/2}\ensuremath{\leftrightarrow}{}^{5}{\mathrm{P}}_{3/2}$ (D2{\mathrm{D}}_{2}D2​) transitions. The counterpropagating pump and probe lasers are independently tunable in frequency, with the probe operating at the single-photon level. The two-dimensional spectrum measured as the laser frequencies are scanned shows fluorescence, Doppler-broadened absorption dips, and sub-Doppler features. The detuning between the pump and probe lasers allows compensation of the Doppler shift for all atomic velocities in the room-temperature vapor, meaning we observe sub-Doppler features for all atoms in the beam. We detail a theoretical model of the system that incorporates fluorescence, saturation effects, and optical pumping and compare this with the measured spectrum, finding a mean absolute percentage error of 3.11%. This high level of agreement allows us to extract the number density and temperature of the Rb\mathrm{Rb}Rb vapor from the two-dimensional spectrum. In the future this technique could be used as an atomic frequency standard for calibrating and characterising a single-photon or low-light-level source.
Absorption spectra of cold Cs atoms in a magneto-optical trap under the influence of a strong external pump laser field with arbitrary detuning and intensity have been systematically investigated. The spectra featured the Rabi sidebands of each transition, and their behavior was nicely fitted by the dressed-atom theory. A pronounced dispersion-type profile with sub-natural linewidth at the pump frequency may be attributable to the stimulated Raman process by sublevels that are lightshifted and optically pumped by the pump laser.
Abstract We demonstrate an integrating sphere to cool 87Rb atoms and measure the recoil-induced resonance and electromagnetically induced absorption spectrum. We measure the relationship between their linewidth and light shift with variation of the detuning and power of the cooling laser and study the performance of the diffuse laser cooling mechanism by the absorption linewidth radio Δν E/Δν R and light shift |Δ R–Δ E| using nonlinear spectroscopy. Specifically, when Δν E/Δν R reaches a value of 1.57, the temperature and number of cold atoms achieve the optimal cooling effect. This characterization of absorption linewidth and light shift will provide a method to estimate whether diffuse light cooling achieves the best cooling effect, contributing to the future development of isotropic laser cooling for application in quantum sensing.
We investigate systematically pump-probe spectroscopy of cold 87Rb{}^{87}\mathrm{Rb}87Rb atoms produced by a magneto-optical trap. The pump-probe spectra are measured without the presence of the trapping beams or any optical molasses. Various polarization configurations of the probe and pump fields result in very different spectra of probe absorption. The observed spectra exhibit a dispersive profile, a dispersionlike profile, a Lorentzian profile, or a dispersive profile plus a Lorentzian profile. The widths of all the spectral profiles are narrower than the natural linewidth of the excited state. Our work clarifies the mechanisms behind these different spectral profiles and provides essential information for the pump-probe spectroscopy of cold atoms.
In this paper the saturation spectra of rubidium vapour at room temperature, obtained with overlapped co-propagating laser beams, were examined. Unlike the standard saturation spectroscopy, here the transmission of the pump laser beam was detected. The pump laser was locked to an atomic transition of the D2 line, while the probe laser frequency was scanned in a wide frequency range. The pump and probe beams had approximately the same intensities; thus the probe laser can saturate transitions and contribute to optical pumping. This, together with Doppler broadening, leads to rich pump transmission spectra, with many lines appearing due to the interaction of lasers with atoms in different velocity groups. The advantages of this method are well-resolved structures and appearance of spectral lines on a flat, Doppler-free background. Agreement between experimental and theoretical results shows the usefulness of this simple model, based on the rate equations, for identification of lines and determination of relative contribution to the observed line intensity from atoms with different velocities. Theoretical spectra are a useful tool for the calibration of experimental spectra obtained by a nonlinear dependence of the laser frequency on the voltage applied to the piezo used for the laser diode frequency scanning.
The nonlinear spectroscopy of cold atoms in the diffuse laser cooling system is studied in this paper. We present the theoretical models of the recoil-induced resonances (RIR) and the electromagnetically-induced absorption (EIA) of cold atoms in diffuse laser light, and show their signals in an experiment of cooling (87)Rb atomic vapor in an integrating sphere. The theoretical results are in good agreement with the experimental ones when the light intensity distribution in the integrating sphere is considered. The differences between nonlinear spectra of cold atoms in the diffuse laser light and in the optical molasses are also discussed.