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Nature Communications

Simultaneous Faraday filtering of the Mollow triplet sidebands with the Cs-D1 clock transition

Simone Luca Portalupi, Matthias Widmann, Cornelius Nawrath, Michael Jetter, Peter Michler, Jörg Wrachtrup, Ilja Gerhardt

Published Nov 25, 2016• 55 citations
Publisher

Abstract

Abstract Hybrid quantum systems integrating semiconductor quantum dots (QDs) and atomic vapours become important building blocks for scalable quantum networks due to the complementary strengths of individual parts. QDs provide on-demand single-photon emission with near-unity indistinguishability comprising unprecedented brightness—while atomic vapour systems provide ultra-precise frequency standards and promise long coherence times for the storage of qubits. Spectral filtering is one of the key components for the successful link between QD photons and atoms. Here we present a tailored Faraday anomalous dispersion optical filter based on the caesium-D1 transition for interfacing it with a resonantly pumped QD. The presented Faraday filter enables a narrow-bandwidth (Δω=2π × 1 GHz) simultaneous filtering of both Mollow triplet sidebands. This result opens the way to use QDs as sources of single as well as cascaded photons in photonic quantum networks aligned to the primary frequency standard of the caesium clock transition.

DOI
10.1038/ncomms13632

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Abstract Hybrid quantum systems integrating semiconductor quantum dots (QDs) and atomic vapours become important building blocks for scalable quantum networks due to the complementary strengths of individual parts. QDs provide on-demand single-photon emission with near-unity indistinguishability comprising unprecedented brightness—while atomic vapour systems provide ultra-precise frequency standards and promise long coherence times for the storage of qubits. Spectral filtering is one of the key components for the successful link between QD photons and atoms. Here we present a tailored Faraday anomalous dispersion optical filter based on the caesium-D1 transition for interfacing it with a resonantly pumped QD. The presented Faraday filter enables a narrow-bandwidth (Δω=2π × 1 GHz) simultaneous filtering of both Mollow triplet sidebands. This result opens the way to use QDs as sources of single as well as cascaded photons in photonic quantum networks aligned to the primary frequency standard of the caesium clock transition.
Hybrid quantum systems are based on the capability to interface elements from complementary fields: only the best properties from all components are utilized, overcoming the limitation of each field. Semiconductor quantum dots (QDs) are well established as sources of bright, pure and highly indistinguishable on-demand single photons. A crucial limitation is given by the relatively short coherence time. This can be overtaken by interfacing them to alkali atoms, which display a very long coherence time and will benefit from the superior properties of QD-based non-classical light sources. As one example of an efficient QD-to-atom interface, we recently demonstrated the filtering of two consecutive single photons generated from a resonantly excited QD by using a Cs-based Faraday anomalous dispersion optical filter (FADOF). The Mollow triplet sidebands were tuned on resonance with the Cs-D1transition and simultaneously filtered with more than 10 % transmission. All other spectral components were suppressed below the noise level. In the present study, a Cs vapor was used to realize a variable optical delay. A resonantly excited QD is used as a source of on-demand single photons, frequency tuned in between the aforementioned Cs-D1 transition. An extensive study on the effects of vapor temperature on the achievable delay has been conducted using single photons with several different linewidth. A record delay of 28 ns was achieved for almost 100% of the transmitted photons. Autocorrelation measurements revealed that an almost ideal g(2)(0) ≈ 0 is preserved after the interaction with the atomic vapor.
In forthcoming quantum networks various quantum systems might be involved to accomplish individual tasks, including storage of quantum states, quantum logic operations, error correction, or entanglement distillation. An interface between a single photon emitter and a potential photon storage could provide one fundamental building block of such a hybrid quantum system. Semiconductor quantum dots (QD) and atomic vapors have already been brought together by single photon spectroscopy of cesium and rubidium [1,2], narrow filtering of QD resonance fluorescence in cesium [3], slowing down QD photons by dispersion between the 6.8 GHz hyperfine-split rubidium D2transitions [4] and in the middle of the four cesium D1 transitions [5] (at around 5.0 GHz in Fig. 1 b).In our experiment the neutrally charged excitonic transition of a strain-tunable InGaAs QD is pumped either resonantly or non-resonantly by a pulsed laser. The QD emission is set between two cesium D1 transitions at 894 nm, which are hyperfine-split only by 1.2 GHz, with a very strong dispersion compared to preceding studies [4,5]. This allows for delay times of a few nanoseconds even at low optical densities, resulting in a propagation velocity at the order of 1/20 of the vacuum speed of light. Such a single photon - atom interface might lay the foundations for a low-loss quantum memory in a future hybrid quantum network.
Faraday Filtering on the Cs-D1_11​-Line for Quantum Hybrid Systems
Narrow-band filtering of light is widely used in optical spectroscopy. Atomic filters, which rely on the Faraday effect, allow for GHz-wide transmission spectra, which are intrinsically matched to an atomic transition. We present an experimental realization and a theoretical study of a Faraday anomalous dispersion optical filter (FADOF) based on cesium and its D1_11​-line-transition (62S1/2→62P1/26^2S_{1/2}\rightarrow6^2P_{1/2}62S1/2​→62P1/2​) around 894nm. We also present the prospects and visions for combining this filter with the single photon emission of a single quantum dot (QD), which matches with the atomic transition.
Future quantum networks will need flying qubits and stationary nodes. As for the generation of single photons which may act as flying qubits, resonantly excited single-semiconductor quantum dots are ideal in terms of their on-demand single-photon emission, indistinguishability, and brightness. Atomic systems can effectively act as mediators for photon–photon interactions, storage media, or building blocks for stationary qubits. Here, we hybridize these two systems and investigate the non-classical interference of spectral Lorentzian-shaped photons, fine-tuned between the cesium (Cs)-D1 hyperfine resonances. The temporal delay in the dispersive hot atomic cesium vapor amounts up to 50 times the photons’ initial width and reveals beats on the single quanta. The photons’ indistinguishability is preserved even after atomic-enabled delay. This proves that the interaction with the Cs vapor conserves the photons’ coherence. The role of spectral diffusion in the solid-state emitter is studied in single- and two-photon experiments in light of the strong frequency dependence of the atomic medium. Our results pave the way for efficient hybrid interfaces between quantum dots and hot atomic vapors as storage media in future quantum networks.
Narrow-band filtering of light is widely used in optical spectroscopy. Atomic filters, which rely on the Faraday effect, allow for GHz-wide transmission spectra, which are intrinsically matched to an atomic transition. We present an experimental realization and a theoretical study of a Faraday filter based on cesium and its D1-line-transition (62S1/2→ 62P1/2) around 894 nm. We also present the prospects and visions for combining this filter with the single photon emission of a single quantum dot, which matches with the atomic transition. The option to lock the spectral position of a quantum dot is discussed at the end of this letter.