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European Quantum Electronics Conference (EQEC)

Two-component superradiance at the self-terminating transitions of Ca and Tl of 535 nm

A.V. Andreev, Sergei I. Derzhavin, D A Mashkovskii

Published Aug 24, 2005• 0 citations
Publisher
DOI
10.1109/eqec.1994.698265

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We present the results of an experimental study of a Tl vapour/Ar mixture as an active medium. Under optical excitation of thallium to the 6d 2 D 3/2 state, we have achieved lasing at λ = 1.3 μm (7p 2 P 0 1/2 — 7s 2 S 1/2 transition) and 535 nm (7s 2 S 1/2 — 6p 2 P 0 3/2 ) through cascade transitions from the 6d 2 D 3/2 state to the upper laser levels. The electron deexcitation rate of the 6p 2 P 0 3/2 metastable state is no slower than 1.5×10 -8 cm 3 s -1 , meaning that this process cannot prevent self-terminating laser action at the 7s 2 S 1/2 — 6p 2 P 0 3/2 transition under electron-beam pumping at pulse repetition rates up to 100 kHz.
Stimulated emission of the 535 nm line of thallium was observed when a Tl-He mixture was pumped optically in the violet wing of a pressure-broadened resonance line of thallium at 377.6 nm by a recombination He–Ca laser emitting at λ = 373.7 nm. Pumping resulted from the absorption transitions between repulsive terms of the Tl-He quasimolecule. The average stimulated radiation power reached 5 mW when the pulse repetition frequency was 6 kHz. The efficiency of conversion of the useful part of the pump pulse was 45%.