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European Quantum Electronics Conference (EQEC)

Pulse-matching and correlation of phase fluctuations in Λ-systems with initially prepared coherence

Th. Richer, Michael Fleischhauer

Published Aug 24, 2005• 0 citations
Publisher
DOI
10.1109/eqec.1994.698234

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The interaction of a bichromatic quantized field with three-level \ensuremath{\Lambda}-type atoms is analyzed on the basis of c-number Langevin equations. In the presence of ground-state coherence one particular combination of field modes is selectively absorbed leading to a correlation of the output fields. This correlation manifests itself in a matching of Fourier components of the field modes and in a strong reduction of the diffusion of the difference phase. This correlation phenomenon is studied for the case of externally generated coherence as well as for coherence produced by population trapping in conjunction with a nonadiabatic atomic response.
We show that nonadiabatic, resonant amplitude- and phase-modulated pulses can be frequency converted with greater efficiency than adiabatic resonant pulses in a coherently prepared $\ensuremath{\Lambda}$ system. Indeed, conversion efficiencies close to unity, similar to those achieved using highly detuned pulses, can been obtained by using highly nonadiabatic resonant pulses. Moreover, by solving the Maxwell-Bloch equations using Fourier transforms, we derive analytical expressions for the probe and the generated four-wave mixing (FWM) pulses as a function of time and propagation distance. From these expressions, which are valid for either adiabatic or nonadiabatic pulses, we derive the result that starting from a nonadiabatic probe pulse, an asymptotically matched probe-FWM pulse pair with the same shape as the initial probe pulse is obtained. In addition, we show that, starting with a nonadiabatic matched pulse pair or a pair of matched pulse trains, we obtain propagation of these pulses without either deformation or losses.
Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.