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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Optical pulse probing of coherency gradient in Λ-medium

Igor V. Kazinets, I. E. Mazets, Boris G. Matisov

Published May 5, 1999• 0 citations
Publisher

Abstract

Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.

DOI
10.1117/12.347396

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Quantum coherence and interference in atomic systems can lead to interesting optical phenomena such as nonabsorbing resonances, lasing without inversion, generating an ultrahigh index of refraction without absorption, propagation of light pulses without losses. In the last-named is given the title transparency. Up to now it is known some types of transparency in multi-level resonant media. One of them is electromagnetically induced transparency (EIT). The phenomenon of EIT in the propagation of laser radiation through an absorbing medium has been recently investigated and explained in terms of quantum coherence and interference for multi-level atomic system. For instance in the (Lambda) -system, if the atomic medium is prepared in a quantum superposition of states, matched pulses, i.e., a pair of optical pulses whose amplitude and phase have a well defined relation, propagate without absorption. The mechanism of coherent population trapping is responsible for EIT in a (Lambda) -system. There is another, well known mechanism for creating transparency in a two-state atom: self-induced transparency, or SIT. Here, a single pulse whose area (the integral of its Rabi frequency over time) is 2(pi) is applied to the medium. Such a pulse causes the atoms to cycle smoothly from the ground to the excited state and then back again. In principle, such a pulse can propagate over long distances. SIT can be generalized to multi-level systems and multiple quasi-monochromatic fields. Generalization of SIT in a (Lambda) -system was obtained in reference 2. In this report we present a new type of transparency (combined transparency). This type describes propagation of laser pulse through a (Lambda) -type medium where the initial atomic state is prepared in the form of spatially varying coherent superposition of low-energetic states (initial coherency gradient). The common envelope behaves as usual 2(pi) hyperbolic secant pulse, but the ratio between the components of frequencies transitions 1> yields 3> and 2> yields 3> changes due to coherent Raman scattering so (phi) equals atan(E1/E2) equals (pi) /2-Gz, where z is the coordinate, G is the constant determined by both the incident pulse parameters and the initial coherence between the atomic states. Our solution demonstrates a direct connection of EIT in adiabatic regime to the SIT effects. This type of a transparency is given the title screw-type transparency, because for the given form of incident pulse (pitch of screw) medium is transparent, if medium's the initial coherence gradient is correspondingly prepared (thread on a engine nut). Besides a transparency, this phenomenon contains a transformation of the incident pulse frequency during the process of the propagation. This property of the phenomena can be result in a complete conversion of the frequency.
We study the propagation dynamics of a single pair of probe and coupling laser pulses in a three-level cascade atomic medium by numerical solving the Maxwell-Bloch equations for atoms and fields. Influences of the pulse durations, intensity and pulse area of the coupling laser on the probe laser propagation are investigated. We found the conditions that the undistorted probe pulse in such medium, i.e., the EIT effect is established. Under EIT conditions, the ground state population is trapped in a dark state. Full Text: PDF References A. Imamoglu, S.E. Harris, "Lasers without inversion: interference of dressed lifetime-broadened states", Opt. Lett. 14 (1989) 1344. CrossRef K.J. Boller, A. Imamoglu, S.E. Harris, "Observation of electromagnetically induced transparency", Phys. Rev. Lett. 66 (1991) 2593. CrossRef A.S. Zibrov, M.D. Lukin, D.E. Nikonov, L. Hollberg, M.O. Scully, V.L. Velichansky, and H.G. Robinson, "Experimental Demonstration of Laser Oscillation without Population Inversion via Quantum Interference in Rb", Phys. Rev. Lett. 75 (1995) 1499. CrossRef L.V. Hau, S. E. Harris, Z. Dutton, C.H. Bejroozi, "Light speed reduction to 17 metres per second in an ultracold atomic gas", Nature, 397 (1999) 594. CrossRef L.V. Doai, D.X. Khoa, and N.H. Bang, "EIT enhanced self-Kerr nonlinearity in the three-level lambda system under Doppler broadening", Phys. Scr. 90 (2015)045502. CrossRef D.X. Khoa, L.V. Doai, D.H. Son, and N.H. Bang, "Enhancement of self-Kerr nonlinearity via electromagnetically induced transparency in a five-level cascade system: an analytical approach", J. Opt. Soc. Am. B, 31, N6 (2014), pp. 1330. CrossRef F.T. Hioe and R. Grobe, "Matched Optical Solitary Waves for Three- and Five-Level Systems", Phys. Rev. Lett. 73, (1994) 2559. CrossRef S.E. Harris and Z.F. Luo, "Preparation energy for electromagnetically induced transparency", Phys. Rev. A. 52 (1995) R928. CrossRef V. G. Arkhipkin, I.V. Timofeev, "Adiabatic propagation of short pulses under conditions of electromagnetically induced transparency", Quantum Electronics, 30 (2000) 180. CrossRef M. Kiffner, T. N. Dey, "Dynamical control of pulse propagation in electromagnetically induced transparency", Phys. Rev. A. 79 (2009) 023829. CrossRef R. Yu, J. Li, P. Huang, A. Zheng, X. Yang, "Dynamic control of light propagation and optical switching through an RF-driven cascade-type atomic medium", Phys. Lett. A. 373 (2009) 2992. CrossRef E. Paspalakis,N. J. Kylstra and P. L. Knight, "Propagation and nonlinear generation dynamics in a coherently prepared four-level system", Phys. Rev. A 65 (2002) 053808. CrossRef E. Ignesti, R. Buffa, L. Fini, E. Sali, M. V. Tognetti, S. Cavalieri, "Controlling the propagation of broadband light pulses by Electromagnetically Induced Transparency", Opt. Commun, 285 (2012) 1185. CrossRef P. R. Bermanand C. H. Raymond Ooi, "Pulse propagation in a medium of ?-type atoms", Phys. Rev. A 86 (2012), 053812. CrossRef G. Buica, T. Nakajima, "Propagation of two short laser pulse trains in a ?-type three-level medium under conditions of electromagnetically induced transparency", Opt. Commun. 332 (2014) 59. CrossRef L. V. Doai, P. V. Trong, D. X. Khoa, and Ng. H. Bang, "Electromagnetically induced transparency in five-level cascade scheme of 85Rb atoms: An analytical approach", Optik, 125 (2014) 3666?3669. CrossRef J.H. Eberly, "Transmission of dressed fields in three-level media", Quantum Semiclass. Opt. 7 (1995) 373. CrossRef M.D. Crisp, "Propagation of Small-Area Pulses of Coherent Light through a Resonant Medium", Phys. Rev. A 1 (1970) 1604. CrossRef
We study the propagation dynamics of a single pair of probe and coupling laser pulses in a three-level cascade atomic medium by numerical solving the Maxwell-Bloch equations for atoms and fields. Influences of the pulse durations, intensity and pulse area of the coupling laser on the probe laser propagation are investigated. We found the conditions that the undistorted probe pulse in such i.e., the effect is established. Under conditions, the ground state population is trapped in a dark state. Full Text: PDF References A. Imamoglu, S.E. Harris, Lasers without inversion: interference of dressed lifetime-broadened states, Opt. Lett. 14 (1989) 1344. CrossRef K.J. Boller, A. Imamoglu, S.E. Harris, Observation of electromagnetically induced transparency, Phys. Rev. Lett. 66 (1991) 2593. CrossRef A.S. Zibrov, M.D. Lukin, D.E. Nikonov, L. Hollberg, M.O. Scully, V.L. Velichansky, and H.G. Robinson, Experimental Demonstration of Laser Oscillation without Population Inversion via Quantum Interference in Rb, Phys. Rev. Lett. 75 (1995) 1499. CrossRef L.V. Hau, S. E. Harris, Z. Dutton, C.H. Bejroozi, speed reduction to 17 metres per second in an ultracold atomic gas, Nature, 397 (1999) 594. CrossRef L.V. Doai, D.X. Khoa, and N.H. Bang, EIT enhanced self-Kerr nonlinearity in the three-level lambda system under Doppler broadening, Phys. Scr. 90 (2015)045502. CrossRef D.X. Khoa, L.V. Doai, D.H. Son, and N.H. Bang, Enhancement of self-Kerr nonlinearity via electromagnetically induced transparency in a five-level cascade system: an analytical approach, J. Opt. Soc. Am. B, 31, N6 (2014), pp. 1330. CrossRef F.T. Hioe and R. Grobe, Matched Optical Solitary Waves for Three- and Five-Level Systems, Phys. Rev. Lett. 73, (1994) 2559. CrossRef S.E. Harris and Z.F. Luo, Preparation energy for electromagnetically induced transparency, Phys. Rev. A. 52 (1995) R928. CrossRef V. G. Arkhipkin, I.V. Timofeev, Adiabatic propagation of short pulses under conditions of electromagnetically induced transparency, Quantum Electronics, 30 (2000) 180. CrossRef M. Kiffner, T. N. Dey, Dynamical control of pulse propagation in electromagnetically induced transparency, Phys. Rev. A. 79 (2009) 023829. CrossRef R. Yu, J. Li, P. Huang, A. Zheng, X. Yang, Dynamic control of light propagation and optical switching through an RF-driven cascade-type atomic medium, Phys. Lett. A. 373 (2009) 2992. CrossRef E. Paspalakis,N. J. Kylstra and P. L. Knight, Propagation and nonlinear generation dynamics in a coherently prepared four-level system, Phys. Rev. A 65 (2002) 053808. CrossRef E. Ignesti, R. Buffa, L. Fini, E. Sali, M. V. Tognetti, S. Cavalieri, Controlling the propagation of broadband light pulses by Induced Transparency, Opt. Commun, 285 (2012) 1185. CrossRef P. R. Bermanand C. H. Raymond Ooi, Pulse propagation in a medium of ?-type atoms, Phys. Rev. A 86 (2012), 053812. CrossRef G. Buica, T. Nakajima, Propagation of two short laser pulse trains in a ?-type three-level medium under conditions of electromagnetically induced transparency, Opt. Commun. 332 (2014) 59. CrossRef L. V. Doai, P. V. Trong, D. X. Khoa, and Ng. H. Bang, Electromagnetically induced transparency in five-level cascade scheme of 85Rb atoms: An analytical approach, Optik, 125 (2014) 3666?3669. CrossRef J.H. Eberly, Transmission of dressed fields in three-level media, Quantum Semiclass. Opt. 7 (1995) 373. CrossRef M.D. Crisp, Propagation of Small-Area Pulses of Coherent Light through a Resonant Medium, Phys. Rev. A 1 (1970) 1604. CrossRef
Propagation of single- and two-color hyperbolic secant femtosecond laser pulses in a three-level $\ensuremath{\Lambda}$-type quantum system is investigated by solving the Maxwell and density matrix equations with the finite-difference time-domain and Runge-Kutta methods. As a first study of our modeling, we simulate pulse self-induced transparency (SIT) in two-level systems and see how this phenomenon can be controlled by manipulating the initial relative phase between the SIT pulse and a second control pulse, provided the ratio between both pulse frequencies obeys the relation ${\ensuremath{\omega}}_{1}∕{\ensuremath{\omega}}_{2}=3$. We then examine frequency down-conversion processes that are observed with single- and two-color pulses the envelope area of which is equal to or a multiple of $2\ensuremath{\pi}$, for pulse frequencies close to resonance with the transitions of a three-level $\ensuremath{\Lambda}$ medium. Also, phase-sensitive phenomena are discussed in the case of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses propagating resonantly in the three-level system. In particular, possibilities for such coherent control are found for frequency down-conversion processes when the ratio of the frequencies of optical transitions is ${\ensuremath{\omega}}_{13}∕{\ensuremath{\omega}}_{12}=3$. The conditions for quantum control of four-wave mixing processes are also examined when the pulse frequencies of two-color $\ensuremath{\omega}\text{\ensuremath{-}}3\ensuremath{\omega}$ pulses are far from any resonance of the three-level system. We demonstrate the possibility to cancel the phase sensitivity of the four-wave coupling in a $\ensuremath{\Lambda}$-type system by competition effects between optical transitions.
The appearance of quantum interference in the microscopic world is one of the deepest mysteries at the very root of quantum mechanics. When light interacts with atoms, it can induce transitions by way of distinct but indistinguishable pathways and yield unexpected and often counter-intuitive results. Electromagnetically Induced Transparency (EIT), Coherent Population Trapping (CPT), and Lasing Without Inversion (LWI) are modern examples of phenomena where the traditional rules that govern absorption and dispersion undergo major revisions. Spectacular consequences of this new state of affairs include the ability of a light beam to propagate through a normally absorbing medium with little or no absorption, or to undergo amplification even if the active medium is not prepared in a state of population inversion. Light signals have been shown to travel with strongly subluminal group velocities of only a handful of meters per second and, even, to propagate at speed greater than the ordinary speed of light, but without violation of causality or of the established rules that control the transfer of optical information through space. Three-level atoms can interact with two coherent electromagnetic fields according to three different systems, known as Cascade, Lambda and Vee systems. The propagation of a weak probe field can be deeply affected by the presence of a second stronger beam, the so-called coupling field. Transparency windows, splitting of emission and absorption lines and enormously enhanced dispersion have been documented in numerous experiments. In this thesis we explore the physical origin of the transparency induced in these systems by the simultaneous interplay of the coupling and probe fields. We focus our attention on the Cascade system and study its two configurations, Cascade-EIT and Cascade-AT. We develop a variety of complementary approaches for the description of these two configurations, some semiclassical and others fully quantum mechanical. We prove the existence of quantum interference in Electromagnetically Induced Transparency and also the surprising absence of interference in a closely related phenomenon, known as the Autler-Townes effect. Finally we complement the traditional machinery of theoretical quantum optics with techniques borrowed from quantum scattering theory, and offer what we believe is the most convincing physical evidence for the appearance, or for the absence, of quantum interference effects.
Summary form only given. Electromagnetically induced transparency (EIT) refers to a phenomenon, whereby the optically resonant transition is rendered nearly transparent by applying a strong coupling laser field. The mechanism of EIT is usually explained in terms of quantum coherence or quantum interference. This EIT has attracted increasing interest because absorption associated with nonlinear optical processes can be removed. In the typical three-level /spl lambda/-system, which includes the ground state and the metastable state, when the atomic population is prepared in the superposition of the states by the coupling fields, the optical response of the media to the probe field is significantly modified. Since this is a coherent control of an electric field by another field via the atomic coherence, several schemes to control light coherently have been suggested. We propose an optical coherent control scheme of the polarization of optical pulses using the EIT quantum coherence, and numerically study its applicability to fast optical switching.
Coherent preparation by laser light of quantum states of atoms and molecules can lead to quantum interference in the amplitudes of optical transitions. In this way the optical properties of a medium can be dramatically modified, leading to electromagnetically induced transparency and related effects, which have placed gas-phase systems at the center of recent advances in the development of media with radically new optical properties. This article reviews these advances and the new possibilities they offer for nonlinear optics and quantum information science. As a basis for the theory of electromagnetically induced transparency the authors consider the atomic dynamics and the optical response of the medium to a continuous-wave laser. They then discuss pulse propagation and the adiabatic evolution of field-coupled states and show how coherently prepared media can be used to improve frequency conversion in nonlinear optical mixing experiments. The extension of these concepts to very weak optical fields in the few-photon limit is then examined. The review concludes with a discussion of future prospects and potential new applications.