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Physical Review

Infrared and Optical Masers

ARTHUR L. SCHAWLOW, Charles Hard Townes

Published Dec 15, 1958• 2,354 citations
Publisher

Abstract

The extension of maser techniques to the infrared and optical region is considered. It is shown that by using a resonant cavity of centimeter dimensions, having many resonant modes, maser oscillation at these wavelengths can be achieved by pumping with reasonable amounts of incoherent light. For wavelengths much shorter than those of the ultraviolet region, maser-type amplification appears to be quite impractical. Although use of a multimode cavity is suggested, a single mode may be selected by making only the end walls highly reflecting, and defining a suitably small angular aperture. Then extremely monochromatic and coherent light is produced. The design principles are illustrated by reference to a system using potassium vapor.

DOI
10.1103/physrev.112.1940

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The extension of maser techniques to the infrared and optical region is considered. It is shown that by using a resonant cavity of centimeter dimensions, having many resonant modes, maser oscillation at these wavelengths can be achieved by pumping with reasonable amounts of incoherent light. For wavelengths much shorter than those of the ultraviolet region, maser-type amplification appears to be quite impractical. Although use of a multimode cavity is suggested, a single mode may be selected by making only the end walls highly reflecting, and defining a suitably small angular aperture. Then extremely monochromatic and coherent light is produced. The design principles are illustrated by reference to a system using potassium vapor.
Introduction The idea of making use of the phenomenon of stimulated emission from an atom or molecule for amplification of the electromagnetic field, and then combining the amplifier with a resonator to make an oscillator, is due to Townes and his co-workers (Gordon, Zeiger and Townes, 1954, 1955) and independently to Basov and Prokhorov (1954, 1955). The former constructed the first MASER, or microwave amplifier by stimulated emission of radiation . In 1958 Schawlow and Townes proposed an application of the same principle to the optical domain (Schawlow and Townes, 1958), in which a two-mirror Fabry–Perot interferometer serves as the optical resonator and an excited group of atoms as the gain medium. The first LASER, or light amplifier by stimulated emission of radiation , was constructed by Maiman (1960). The gain medium was ruby, which was excited by a bright flash of light from a gas discharge tube, whereupon the laser delivered a short optical pulse. The first continuously operating – or CW – laser was developed by Javan and his co-workers (Javan, Bennett and Herriott, 1961); it made use of a He:Ne gas mixture, that was continuously excited by a discharge, as the gain medium. This type of laser is still widely used today. Since that time many different kinds of laser have been developed, ranging in wavelength from the infrared to the ultraviolet. Some produce light at several different frequencies at once, and some are tunable over a wide range.
The subject of masers is introduced by giving an historical account of events which led to the amplification of microwave radiation by an inverted population in a system of weakly interacting ammonia molecules. The introduction also outlines the development of masers up to the present. Sections 2 and 3 are concerned with maser fundamentals. Methods for obtaining inverted populations are discussed in § 2. Section 3 is devoted to the theory of maser gain and noise. This is followed by a discussion of microwave solid state masers. Microwave maser materials and the development of unidirectional travelling wave maser amplifiers are emphasized. Optical masers are treated in § 5. In this section the theory of optical amplifiers and oscillators is outlined. Also included in the theoretical discussion is a rather lengthy consideration of pump power requirements in optically pumped masers. This is followed by a survey of solid state, semiconductor and gaseous optical masers. The review ends with some comments on the extension of masers to new wavelength regions.
The extension of optical maser techniques to the γ-ray region is considered. It is shown that under certain conditions induced γ rays can be produced. The condition of criticality rather than that of oscillation is used because a γ-ray maser does not have a resonant structure. The main observable effects are the shortening of lifetimes of some γ excitations and the appearance of two or more coherent γ quanta. It appears to be difficult to prepare samples that will become critical. The principles are applied to a specific example.
The extension of optical maser techniques to the γ-ray region is considered. It is shown that under certain conditions induced γ rays can be produced. The condition of criticality rather than that of oscillation is used because a γ-ray maser does not have a resonant structure. The main observable effects are the shortening of lifetimes of some γ excitations and the appearance of two or more coherent γ quanta. It appears to be difficult to prepare samples that will become critical. The principles are applied to a specific example.
The one-atom maser or micromaser is, in contrary to ordinary masers and lasers, a pure quantum device operating with only a few photons and less than one pump atom on the average in the maser cavity. It is thus an ideal device to study quantum phenomena such as the generation of nonclassical light. The cavity is a superconducting niobium microwave resonator with a high quality factor (up to 3 × 1010). Using a single trapped ion related experiments can now also be performed in the infrared spectral region.
The equations are generalized governing coherent emission from quantum mechanical amplifiers (microwave, infrared, and optical masers) using either electric or magnetic dipole transitions. Earlier analyses by Gordon, Zeiger and Townes, Feynman, Vernon and Hellworth, and Wang and Singer, are incorporated in this generalization. The principal new result of this analysis is that an amplitude modulation of the output is to be expected from all maser oscillators excepting those in which excited atoms are supplied at a notably greater rate than the depopulation rate due to coherent induced emission. This analysis also suggests that an energy population inversion of electric dipole moments can be performed using coherent light sources in the same manner as with magnetic dipole moments. It appears therefore that modulation of an optical or infrared maser (e.g., for communication purposes) may be easily accomplished by varying the population of excited states through control of the pumping energy. This modulation may be both by absorption and amplification. (Author)