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Physical Review Letters

General Analysis of Optical, Infrared, and Microwave Maser Oscillator Emission

J. R. Singer, S. Wang

Published Apr 1, 1961• 21 citations
Publisher

Abstract

The equations are generalized governing coherent emission from quantum mechanical amplifiers (microwave, infrared, and optical masers) using either electric or magnetic dipole transitions. Earlier analyses by Gordon, Zeiger and Townes, Feynman, Vernon and Hellworth, and Wang and Singer, are incorporated in this generalization. The principal new result of this analysis is that an amplitude modulation of the output is to be expected from all maser oscillators excepting those in which excited atoms are supplied at a notably greater rate than the depopulation rate due to coherent induced emission. This analysis also suggests that an energy population inversion of electric dipole moments can be performed using coherent light sources in the same manner as with magnetic dipole moments. It appears therefore that modulation of an optical or infrared maser (e.g., for communication purposes) may be easily accomplished by varying the population of excited states through control of the pumping energy. This modulation may be both by absorption and amplification. (Author)

DOI
10.1103/physrevlett.6.351

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The equations are generalized governing coherent emission from quantum mechanical amplifiers (microwave, infrared, and optical masers) using either electric or magnetic dipole transitions. Earlier analyses by Gordon, Zeiger and Townes, Feynman, Vernon and Hellworth, and Wang and Singer, are incorporated in this generalization. The principal new result of this analysis is that an amplitude modulation of the output is to be expected from all maser oscillators excepting those in which excited atoms are supplied at a notably greater rate than the depopulation rate due to coherent induced emission. This analysis also suggests that an energy population inversion of electric dipole moments can be performed using coherent light sources in the same manner as with magnetic dipole moments. It appears therefore that modulation of an optical or infrared maser (e.g., for communication purposes) may be easily accomplished by varying the population of excited states through control of the pumping energy. This modulation may be both by absorption and amplification. (Author)
A theoretical model for the behavior of an optical maser is presented in which the electromagnetic field is treated classically, and the active medium is made up of thermally moving atoms which acquire nonlinear electric dipole moments under the action of the field according to the laws of quantum mechanics. The corresponding macroscopic electric polarization of the medium acts as a source for an electromagnetic field. The self-consistency requirement that a quasistationary field should be sustained by the induced polarization leads to equations which determine the amplitudes and frequencies of multimode oscillation as functions of the various parameters characterizing the maser. Among the results obtained are: threshold conditions, single-mode output as a function of cavity tuning, frequency pulling and pushing, mode competition phenomena including frequency locking, production of combination tones, and population pulsations. A more approximate discussion of maser action using rate equations is also given in which the concept of "hole burning" plays a role.
Abstract : The time variation of amplitude of a maser oscillator is derived from a study of the rate equations connecting the population inversion and the electromagnetic energy stored in the maser resonator. The methods of nonlinear mechanics are used to derive a qualitative description of the amplitude variation in the absence of a complete solution of the rate equations. Modifications of the simple rate equations necessary to account for the existence of undamped relaxation oscillations are introduced for both microwave and optical masers, and their physical significance is discussed. The production of 'giant pulses' of radiation is also treated. (Author)
The spectrum of power radiated by a solid-state optical maser in steady-state operation is obtained by considering each atomic system to be a source of randomly fluctuating dipole moment which drives every mode of the cavity. The nonlinear behavior of the collection of atomic systems is treated in such a way that a detailed examination of the distribution of power in the various modes is possible. A number of examples are considered which show how critically dependent on the relative loss rates of the various modes are the characteristics of the output from a multimode oscillator. An interesting result of this calculation is the appearance in some cases of an abrupt transition as the pumping power is increased: above this point a large fraction of energy goes into the mode which is resonant with the atomic transition and which has the lowest loss rate. Another case is studied which does not have this feature, but which could be useful in analyzing the behavior of solid-state optical masers which have substantial scattering due to crystal imperfections.
Maser action due to a mixing between unperturbed spin states, which is produced by a strong coherent pumping field at an angular frequency ω, is investigated by using rate equations of a spin density matrix referred to a rotating coordinate system. The relaxation of each state, which was introduced usually by phenomenological considerations, is obtained from an interaction Hamiltonian of the spin moments with local fields. The induced oscillating fields at 2ω±ω s and ω s , which are proportional to a small signal field at a frequency ω s , have the possibility of power emission (or absorption) by choosing suitably the pumping field. The components at 2ω±ω s are responsible for a frequency mixing between ω and ω±ω s occuring in the rotating coordinates. The emitted (or absorbed) line shape is not a simple Lorentzian in the case of the spin moment 1×ℏ1{\times}\hbar1×ℏ and considered to be a quantum affect in the three level scheme. The frequencies of the emitted (or absorbed) fields are expected to be shifted by varying the magnitude, or the frequency of the pumping field, or the static magnetic field.
This paper has two purposes: 1) to clarify the relationship between the quantum theory of radiation, where the electromagnetic field-expansion coefficients satisfy commutation relations, and the semiclassical theory, where the electromagnetic field is considered as a definite function of time rather than as an operator; and 2) to apply some of the results in a study of amplitude and frequency stability in a molecular beam maser. In 1), it is shown that the semiclassical theory, when extended te take into account both the effect of the field on the molecules and the effect of the molecules on the field, reproduces almost quantitatively the same laws of energy exchange and coherence properties as the quantized field theory, even in the limit of one or a few quanta in the field mode. In particular, the semiclassical theory is shown to lead to a prediction of spontaneous emission, with the same decay rate as given by quantum electrodynamics, described by the Einstein A coefficients. In 2), the semiclassical theory is applied to the molecular beam maser. Equilibrium amplitude and frequency of oscillation are obtained for an arbitrary velocity distribution of focused molecules, generalizing the results obtained previously by Gordon, Zeiger, and Townes for a singel-velocity beam, and by Lamb and Helmer for a Maxwellian beam. A somewhat surprising result is obtained; which is that the measurable properties of the maser, such as starting current, effective molecular Q, etc., depend mostly on the slowest 5 to 10 per cent of the molecules. Next we calculate the effect of amplitude and frequency of oscillation, of small systematic perturbations. We obtain a prediction that stability can be improved by adjusting the system so that the molecules emit all their energy h Ω to the field, then reabsorb part of it, before leaving the cavity. In general, the most stable operation is obtained when the molecules are in the process of absorbing energy from the radiation as they leave the cavity, most unstable when they are still emitting energy at that time. Finally, we consider the response of an oscillating maser to randomly time-varying perturbations. Graphs are given showing predicted response to a small superimposed signal of a frequency near the oscillation frequency. The existence of "noise enhancing" and "noise quieting" modes of operation found here is a general property of any oscillating system in which amplitude is limited by nonlinearity.
An analysis of a three-level system using time-dependent perturbation theory shows that two distinct photon-emission processes take place within such a system when stimulated optical emission occurs: one-and two-photon transitions. The two-photon transition consists of the emission of a stimulated photon followed by the absorption of a coherent pump photon. In three-level systems which possess a narrow pump level, two-photon transitions are dominant at high pump powers while the maser line is split into two lines due to the modulation of the wave function at an angular frequency determined by the rate of pumping. This might lead to the possibility of frequency-modulating the maser line. These results are extended qualitatively to include optical masers which possess broad pump-bands.