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Journal of Applied Physics

Theory of Quantum Oscillators in a Multimode Cavity

W. G. Wagner, GEORGE L. BIRNBAUM

Published Jul 1, 1961• 56 citations
Publisher

Abstract

The spectrum of power radiated by a solid-state optical maser in steady-state operation is obtained by considering each atomic system to be a source of randomly fluctuating dipole moment which drives every mode of the cavity. The nonlinear behavior of the collection of atomic systems is treated in such a way that a detailed examination of the distribution of power in the various modes is possible. A number of examples are considered which show how critically dependent on the relative loss rates of the various modes are the characteristics of the output from a multimode oscillator. An interesting result of this calculation is the appearance in some cases of an abrupt transition as the pumping power is increased: above this point a large fraction of energy goes into the mode which is resonant with the atomic transition and which has the lowest loss rate. Another case is studied which does not have this feature, but which could be useful in analyzing the behavior of solid-state optical masers which have substantial scattering due to crystal imperfections.

DOI
10.1063/1.1736202

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The spectrum of power radiated by a solid-state optical maser in steady-state operation is obtained by considering each atomic system to be a source of randomly fluctuating dipole moment which drives every mode of the cavity. The nonlinear behavior of the collection of atomic systems is treated in such a way that a detailed examination of the distribution of power in the various modes is possible. A number of examples are considered which show how critically dependent on the relative loss rates of the various modes are the characteristics of the output from a multimode oscillator. An interesting result of this calculation is the appearance in some cases of an abrupt transition as the pumping power is increased: above this point a large fraction of energy goes into the mode which is resonant with the atomic transition and which has the lowest loss rate. Another case is studied which does not have this feature, but which could be useful in analyzing the behavior of solid-state optical masers which have substantial scattering due to crystal imperfections.
A theoretical model for the behavior of an optical maser is presented in which the electromagnetic field is treated classically, and the active medium is made up of thermally moving atoms which acquire nonlinear electric dipole moments under the action of the field according to the laws of quantum mechanics. The corresponding macroscopic electric polarization of the medium acts as a source for an electromagnetic field. The self-consistency requirement that a quasistationary field should be sustained by the induced polarization leads to equations which determine the amplitudes and frequencies of multimode oscillation as functions of the various parameters characterizing the maser. Among the results obtained are: threshold conditions, single-mode output as a function of cavity tuning, frequency pulling and pushing, mode competition phenomena including frequency locking, production of combination tones, and population pulsations. A more approximate discussion of maser action using rate equations is also given in which the concept of "hole burning" plays a role.
Schwinger has applied his generalized quantum action principle and the method of thermodynamic Green's functions to an harmonic oscillator. He has shown how this technique describes the buildup of cavity oscillations in a simple model of the maser. This paper applies Schwinger's technique to multimode cavities. The energy, autocorrelation (or coherence), and spectral distribution of individual cavity modes in the steady state, their rate of buildup and their response to external signals have been calculated. Conditions for the buildup and for the steady state of laser action are stated. It has been shown that the steady-state laser radiation in each cavity mode can be described in terms of spontaneous and induced emissions, the latter one containing a coherent and an incoherent part.
The simplest open, nonlinear optical system consists of a single bosonic mode with nonlinear self-interactions coupled to driving fields and reservoirs. In this chapter, we will examine a number of systems of this type using the methods that have been developed in the preceding chapters. Systems of this type can exhibit a variety of interesting physical effects. For example, in the case of a driven nonlinear oscillator, there can be more than one steady state (bistability), and quantum statistical effects can manifest themselves by affecting the stability of these states. Other quantum statistical effects have also been predicted in a variety of related systems – such as photon anti-bunching, squeezing and changes to spectra. In general, the size of these effects scales inversely with the size of the system. This ‘system size’ refers to a threshold photon number, a number of atoms, or some similar quantity. The nature of the steady states themselves can become less than straightforward. Nonequilibrium dissipative systems, of which the systems considered in this chapter are examples, have parameters that describe the energy input to the system, and their steady states depend on these parameters. When driven far from equilibrium, such systems can exhibit bifurcations in their steady states. In more complex cases, this eventually leads to periodic oscillations and chaos. Devices like this can be realized with multiple types of nonlinearity, ranging from nonlinear dielectrics through to cavity QED (with near-resonant atoms), cavity optomechanics (with nanomechanical oscillators) and circuit QED (with superconducting Josephson junctions). We will start with cases where all the interactions are with the reservoirs, which may be linear or nonlinear, while the cavity itself is harmonic in its response.
We present the theory of a truly microscopic maser consisting of a single-mode high-Q resonator in which a monoenergetic beam of excited two-level atoms is injected at such a low flux that at most one atom at a time is present inside the cavity. Both a microscopic theory and a heuristic Fokker-Planck approach are presented. We show that the micromaser exhibits a number of novel features that are averaged out in usual masers and lasers. First, the field is in general sub-Poissonian, which reflects the quantization of both the field and its sources. Second, the onset of maser oscillations may be followed by a succession of abrupt transitions in the state of the field. Finally, as the atomic flux through the resonator is increased, the maser threshold acquires characteristics of a continuous phase transition, whereas the subsequent changes in the field distribution become analogous to first-order phase transitions.
The equations are generalized governing coherent emission from quantum mechanical amplifiers (microwave, infrared, and optical masers) using either electric or magnetic dipole transitions. Earlier analyses by Gordon, Zeiger and Townes, Feynman, Vernon and Hellworth, and Wang and Singer, are incorporated in this generalization. The principal new result of this analysis is that an amplitude modulation of the output is to be expected from all maser oscillators excepting those in which excited atoms are supplied at a notably greater rate than the depopulation rate due to coherent induced emission. This analysis also suggests that an energy population inversion of electric dipole moments can be performed using coherent light sources in the same manner as with magnetic dipole moments. It appears therefore that modulation of an optical or infrared maser (e.g., for communication purposes) may be easily accomplished by varying the population of excited states through control of the pumping energy. This modulation may be both by absorption and amplification. (Author)
Using the semiclassical theory of radiation, the steady-state operation of the optical maser oscillator is studied in the case where a single "cavity" mode is excited. On introducing certain simplifying assumptions, a straightforward calculation leads to concise results for the frequency and amplitude of the field oscillations. These results are either well known or readily interpreted. For example, a frequency pulling effect is predicted which corresponds to the Bloch-Siegert shift, or alternatively is understandable as due to the Stark effect.