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Proceedings of the IEEE

Semiclassical treatment of the optical maser

L. W. Davis

Published Jan 1, 1963• 33 citations
Publisher

Abstract

Using the semiclassical theory of radiation, the steady-state operation of the optical maser oscillator is studied in the case where a single "cavity" mode is excited. On introducing certain simplifying assumptions, a straightforward calculation leads to concise results for the frequency and amplitude of the field oscillations. These results are either well known or readily interpreted. For example, a frequency pulling effect is predicted which corresponds to the Bloch-Siegert shift, or alternatively is understandable as due to the Stark effect.

DOI
10.1109/proc.1963.1662

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Journal of Physics A Mathematical Nuclear and General•Oct 11, 1974•0 citations
Using the semiclassical theory of radiation, the steady-state operation of the optical maser oscillator is studied in the case where a single "cavity" mode is excited. On introducing certain simplifying assumptions, a straightforward calculation leads to concise results for the frequency and amplitude of the field oscillations. These results are either well known or readily interpreted. For example, a frequency pulling effect is predicted which corresponds to the Bloch-Siegert shift, or alternatively is understandable as due to the Stark effect.
This paper has two purposes: 1) to clarify the relationship between the quantum theory of radiation, where the electromagnetic field-expansion coefficients satisfy commutation relations, and the semiclassical theory, where the electromagnetic field is considered as a definite function of time rather than as an operator; and 2) to apply some of the results in a study of amplitude and frequency stability in a molecular beam maser. In 1), it is shown that the semiclassical theory, when extended te take into account both the effect of the field on the molecules and the effect of the molecules on the field, reproduces almost quantitatively the same laws of energy exchange and coherence properties as the quantized field theory, even in the limit of one or a few quanta in the field mode. In particular, the semiclassical theory is shown to lead to a prediction of spontaneous emission, with the same decay rate as given by quantum electrodynamics, described by the Einstein A coefficients. In 2), the semiclassical theory is applied to the molecular beam maser. Equilibrium amplitude and frequency of oscillation are obtained for an arbitrary velocity distribution of focused molecules, generalizing the results obtained previously by Gordon, Zeiger, and Townes for a singel-velocity beam, and by Lamb and Helmer for a Maxwellian beam. A somewhat surprising result is obtained; which is that the measurable properties of the maser, such as starting current, effective molecular Q, etc., depend mostly on the slowest 5 to 10 per cent of the molecules. Next we calculate the effect of amplitude and frequency of oscillation, of small systematic perturbations. We obtain a prediction that stability can be improved by adjusting the system so that the molecules emit all their energy h Ω to the field, then reabsorb part of it, before leaving the cavity. In general, the most stable operation is obtained when the molecules are in the process of absorbing energy from the radiation as they leave the cavity, most unstable when they are still emitting energy at that time. Finally, we consider the response of an oscillating maser to randomly time-varying perturbations. Graphs are given showing predicted response to a small superimposed signal of a frequency near the oscillation frequency. The existence of "noise enhancing" and "noise quieting" modes of operation found here is a general property of any oscillating system in which amplitude is limited by nonlinearity.
The interaction between an electromagnetic (em) pulse and a maser medium is described by a general set of five equations, under the assumption of a homogeneously broadened electric-dipole transition with two Bloch relaxation times T2and T1and of a linear broadband loss mechanism. When the equations are specialized at resonance, their solutions include the results of the previous treatments on the amplifier problem obtained under particular assumptions. The steady-state pulse (S. S. P.) introduced by Wittke and Warter forT_{2}/T_{1} = 0is here generalized forT_{2}/T_{1} \neq 0and it is shown to propagate at the same velocity of the light in the medium. In the caseT_{2}/T_{1} = 0the steady state is described by exact analytical relations. For times short in comparison to the relaxation times, a solution is given which generalizes the usual interaction formula between an em field and a two-level system by introducing propagation effects. In the general case out of resonance, it is shown that an S. S. P. exists, and that its frequency coincides with the frequency of the atomic transition, independent of the frequency of the input field.
A theoretical model for the behavior of an optical maser is presented in which the electromagnetic field is treated classically, and the active medium is made up of thermally moving atoms which acquire nonlinear electric dipole moments under the action of the field according to the laws of quantum mechanics. The corresponding macroscopic electric polarization of the medium acts as a source for an electromagnetic field. The self-consistency requirement that a quasistationary field should be sustained by the induced polarization leads to equations which determine the amplitudes and frequencies of multimode oscillation as functions of the various parameters characterizing the maser. Among the results obtained are: threshold conditions, single-mode output as a function of cavity tuning, frequency pulling and pushing, mode competition phenomena including frequency locking, production of combination tones, and population pulsations. A more approximate discussion of maser action using rate equations is also given in which the concept of "hole burning" plays a role.
A simple model of a maser or laser consisting of a single-mode field coupled to NNN identical two-level atoms is considered. The semiclassical approximation is equivalent to neglecting the statistical correlations between the atoms and the field. The accuracy of this approximation is investigated by writing equations of motion for the correlations. To obtain a complete, self-consistent set of equations, it is necessary to include correlations of the field with itself (related to the coherence of the field) and correlations between different atoms. Relaxations and an energy source are introduced phenomenologically into the equations of motion. They are then solved for the case of steady-state oscillation. It is found that the correlations are smaller than the terms kept in the semiclassical theory by the order of 1 over the number of photons present in the field, larger if thermal photons abound, but smaller if the field relaxation is dominant. Expressions are also found for the amplitude and phase fluctuations of the field. The latter yield a linewidth for the maser oscillator in agreement with earlier calculations, but obtained by a different method.
The spectrum of power radiated by a solid-state optical maser in steady-state operation is obtained by considering each atomic system to be a source of randomly fluctuating dipole moment which drives every mode of the cavity. The nonlinear behavior of the collection of atomic systems is treated in such a way that a detailed examination of the distribution of power in the various modes is possible. A number of examples are considered which show how critically dependent on the relative loss rates of the various modes are the characteristics of the output from a multimode oscillator. An interesting result of this calculation is the appearance in some cases of an abrupt transition as the pumping power is increased: above this point a large fraction of energy goes into the mode which is resonant with the atomic transition and which has the lowest loss rate. Another case is studied which does not have this feature, but which could be useful in analyzing the behavior of solid-state optical masers which have substantial scattering due to crystal imperfections.