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IEEE Journal of Quantum Electronics

Theory of optical maser amplifiers

F. T. Arecchi, R. Bonifacio

Published Jul 1, 1965• 268 citations
Publisher

Abstract

The interaction between an electromagnetic (em) pulse and a maser medium is described by a general set of five equations, under the assumption of a homogeneously broadened electric-dipole transition with two Bloch relaxation times T2and T1and of a linear broadband loss mechanism. When the equations are specialized at resonance, their solutions include the results of the previous treatments on the amplifier problem obtained under particular assumptions. The steady-state pulse (S. S. P.) introduced by Wittke and Warter forT_{2}/T_{1} = 0is here generalized forT_{2}/T_{1} \neq 0and it is shown to propagate at the same velocity of the light in the medium. In the caseT_{2}/T_{1} = 0the steady state is described by exact analytical relations. For times short in comparison to the relaxation times, a solution is given which generalizes the usual interaction formula between an em field and a two-level system by introducing propagation effects. In the general case out of resonance, it is shown that an S. S. P. exists, and that its frequency coincides with the frequency of the atomic transition, independent of the frequency of the input field.

DOI
10.1109/jqe.1965.1072212

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Physical Review•Mar 10, 1969•166 citations
The interaction between an electromagnetic (em) pulse and a maser medium is described by a general set of five equations, under the assumption of a homogeneously broadened electric-dipole transition with two Bloch relaxation times T2and T1and of a linear broadband loss mechanism. When the equations are specialized at resonance, their solutions include the results of the previous treatments on the amplifier problem obtained under particular assumptions. The steady-state pulse (S. S. P.) introduced by Wittke and Warter forT_{2}/T_{1} = 0is here generalized forT_{2}/T_{1} \neq 0and it is shown to propagate at the same velocity of the light in the medium. In the caseT_{2}/T_{1} = 0the steady state is described by exact analytical relations. For times short in comparison to the relaxation times, a solution is given which generalizes the usual interaction formula between an em field and a two-level system by introducing propagation effects. In the general case out of resonance, it is shown that an S. S. P. exists, and that its frequency coincides with the frequency of the atomic transition, independent of the frequency of the input field.
Pulse propagation in maser-type traveling-wave amplifiers with a homogeneously broadened transition is treated by a formalism analogous to the Bloch equations. Phenomenological dephasing (T2) and recovery (T1) times are defined, and a linear (nonsaturable) loss mechanism is included. In the numerical calculations, only the case of negligible excitation during the time it takes a pulse to pass is considered. When pulses are allowed to grow until the amplifier is ``saturated,'' steady-state pulses having a unique shape and intensity independent of the initial pulse are found. The parameters of these steady-state pulses depend only on the ratio of the linear loss and gain coefficients. Steady-state pulses have a peak intensity that decreases monotonically from infinity to zero as the linear loss coefficient varies from zero to the gain coefficient, while the pulse width correspondingly varies from zero to infinity, and the pulse energy varies from a finite value to zero. Steady-state pulses propogate at a velocity less than that of the small signal velocity in the medium.
The transient response of a three-level optical maser is calculated for a density of homogeneously broadened atoms coupled to one homogeneously broadened cavity mode. The atoms are treated in terms of the density matrix and the cavity mode is treated classically. Solutions are found analytically for the steady state and for the linearized form of two simplifications of the general equations. These special solutions have been previously obtained by Bloom and Statz and de Mars. Numerical solutions are found for a certain set of parameters. The response linewidth is found assuming one cavity mode coupled to a density of inhomogeneously broadened atoms.
The problem of a light pulse propagating in a nonlinear laser medium is investigated. The electromagnetic field is treated classically and the active medium consists of thermally moving atoms which have two electronic states with independent decay constants ${\ensuremath{\gamma}}_{a}$ and ${\ensuremath{\gamma}}_{b}$ in addition to the decay constant ${\ensuremath{\gamma}}_{\mathrm{ab}}$ describing the phase memory. The self-consistency requirement that the field sustained by the polarized medium be equal to the field inducing the polarization leads to coupled equations of motion for the density matrix, and equations of propagation for the electromagnetic field. Although the theory is developed for a Doppler-broadened gaseous medium, it may also be applied to a solid medium with inhomogeneous broadening. A unified treatment is given encompassing a wide range of pulse durations from cw signals to psec pulses. Continuous pumping is allowed, as well as any amount of detuning of the carrier frequency of the pulse from the atomic resonance frequency. The three independent decay constants ${\ensuremath{\gamma}}_{a}$, ${\ensuremath{\gamma}}_{b}$, and ${\ensuremath{\gamma}}_{\mathrm{ab}}$ provide greater flexibility than that obtained by using 1T1\frac{1}{{T}_{1}}T1​1​ and 1T2\frac{1}{{T}_{2}}T2​1​. The equations are solved analytically in a few specialized cases and numerically in the general case. Flow charts for accomplishing the numerical integration are given. Among the special problems considered is the apparent paradox of pulses propagating faster than the velocity of light under circumstances described by Basov et al. It is shown that this contradiction with relativity arises from the use of an unphysical initial condition.
A theoretical model is developed for the behavior of an optical maser medium in a static magnetic field of arbitrary strength in the ZZZ direction and an electromagnetic field which is composed of traveling waves with both states of polarization and with both +z+z+z and $\ensuremath{-}z$ directions. An integral formulation of a truncated phenomenological density matrix is introduced to treat the degeneracy of the atomic energy levels within the natural width. This integral is an exact solution of the phenomenological differential equation for the density matrix which was introduced by Wilcox and Lamb. The inherent degeneracy in the electromagnetic field is included by treating the field in a classical manner. The integral formulation is iterated to yield the first- and third-order contributions to the electric polarization vector P in a spatial element drd\mathrm{r}dr, and the electric field and the electric polarization are made self-consistent in this spatial element by using coefficients in Maxwell's equations which are slowly varying functions of position and time. Atomic motion, hyperfine, isotope, and other line-broadening effects are included in the polarization vector P. The general linear-amplifier, linear-oscillator, and closed-path-oscillator or photon-rate-gyroscope problems are formulated and in the simplest case require the analysis of eight nonlinear equations. These reduce to four equations for the linear oscillator with an axial magnetic field, and these examples are discussed in detail and compared with experiment. An anomalous situation arises for the ja=jb{j}_{a}={j}_{b}ja​=jb​ or Fa=Fb{F}_{a}={F}_{b}Fa​=Fb​ linear amplifiers or linear-oscillator masers, and the development indicates that these systems are stable near line center only for either right or left circular polarization in zero or weak magnetic fields. A magnetic field "dip" near line center is discussed. Special examples which require four or fewer nonlinear equations are discussed.
A simple maser model consisting of a single-mode field coupled to N identical two-level atoms is presented. The assumption of negligible statistical correlation between the atoms and the field, permits the Heisenberg equations of motion to be replaced by a self-consistent set of ordinary nonlinear differential equations. Relaxation terms and an energy source are introduced phenomenologically. The resulting equations exhibit a threshold, stable and unstable steady states, relaxation oscillations and, sometimes, spiking. The dynamic equations for the hydrogen maser and the rate equations of laser theory are derived as special cases. Also discussed are the maser amplifier, locking of a maser to an external signal, and the effects of cavity thermal noise.
Recent advances in laser technology have led to the production of ultrashort electromagnetic pulses of very high peak power. In this paper we develop a theory which describes the transient behavior of such pulses in a laser amplifier. The effects of atomic coherence and inhomogeneous broadening, necessary for a complete treatment of the problem, are included. In the present development, the degree of homogeneous and inhomogeneous broadening is variable. The two-level active atoms are characterized by a phase memory time T2{T}_{2}T2​ and an inhomogeneous frequency distribution (which leads to a reversible decay time T2∗T_{2}^{}{}_{}{}^{*}T2​​∗). The field (Maxwell) and atomic (Schr\"odinger) equations are coupled in a self-consistent manner as in Lamb's theory of an optical maser. The resulting equations are solved analytically in certain limits, while the general case is integrated numerically. The emphasis is placed on the situation in which T2∗T_{2}^{}{}_{}{}^{*}T2​​∗ and the pulse width are much shorter than T2{T}_{2}T2​. Thus our main effort is devoted to the physics of the inhomogeneously broadened system. The theory itself, however, contains the effects of both forms of broadening. The basic difference between inhomogeneous and homogeneous broadening is discussed. In the former case, the decay of radiation is caused by the dephasing of dipoles, and is reversible. The atomic memory is retained during the dephasing, and an internal reflection of the atomic coordinates, as is exemplified in the "photon echo" process, will cause the dipoles to rephase. The phonon interruptions or atomic collisions that bring about the homogeneous broadening are random processes which lead to an irreversible destruction of the atomic phase memory. The implications of the reversible versus irreversible decay processes are seen to have important consequences in the problem of pulse amplification.