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Optics Express

On-site monitoring of atomic density number for an all-optical atomic magnetometer based on atomic spin exchange relaxation

Hong Zhang, Sheng Zou, Xiyuan Chen, Ming Ding, Guangcun Shan, Zhaohui Hu, Wei Quan

Published Jul 21, 2016• 21 citations
Publisher

Abstract

We present a method for monitoring the atomic density number on site based on atomic spin exchange relaxation. When the spin polarization P ≪ 1, the atomic density numbers could be estimated by measuring magnetic resonance linewidth in an applied DC magnetic field by using an all-optical atomic magnetometer. The density measurement results showed that the experimental results the theoretical predictions had a good consistency in the investigated temperature range from 413 K to 463 K, while, the experimental results were approximately 1.5 ∼ 2 times less than the theoretical predictions estimated from the saturated vapor pressure curve. These deviations were mainly induced by the radiative heat transfer efficiency, which inevitably leaded to a lower temperature in cell than the setting temperature.

DOI
10.1364/oe.24.017234

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We present a method for monitoring the atomic density number on site based on atomic spin exchange relaxation. When the spin polarization P ≪ 1, the atomic density numbers could be estimated by measuring magnetic resonance linewidth in an applied DC magnetic field by using an all-optical atomic magnetometer. The density measurement results showed that the experimental results the theoretical predictions had a good consistency in the investigated temperature range from 413 K to 463 K, while, the experimental results were approximately 1.5 ∼ 2 times less than the theoretical predictions estimated from the saturated vapor pressure curve. These deviations were mainly induced by the radiative heat transfer efficiency, which inevitably leaded to a lower temperature in cell than the setting temperature.
Abstract The alkali number density inside the sealed vapor cell restricts the fundamental sensitivity of the atomic magnetometer and may decrease in the long term, thus motivating the investigation of an in situ density determination method on atomic magnetometers. This paper presents a method to measure the alkali number density, which is proportional to the spin-exchange relaxation rate, through phase-frequency analysis. The magnetic resonance response of the atomic magnetometer was actively strengthened at low polarization by increasing the oscillating field amplitude. To downplay the side effect of the transverse field broadening, phase-frequency analysis was applied to extract the transverse relaxation time limited by spin-exchange collisions. The experimental results coincided well with the saturated vapor pressure curve ranging from 413 K to 463 K. Calculated densities were approximately 0.779–0.992 times those of predictions. The density measurement accuracy was improved compared to traditional methods.
The number density of alkali atoms in vaper cell is an important parameter for atomic magnetometer. The vapor cell is usually heated to a high temperature for the number density exceed to 1018m−3to achieve the spin-exchange-relaxation-free (SERF) process. The optical rotation of multichannel atomic magnetometers is affected by the number density distribution. We present an effective method for monitoring and analyzing the spatial distribution homogeneity of the atomic number density in the alkali metal cell within the SERF magnetometer. The numerical results from researching the model of electric heating films and ovens show that the temperature gradient increases with an increase in the cell temperature. This causes an nonuniform number density distribution based on the saturated vapor pressure curve. We present a laser absorption spectroscopy method by using the high-resolution beam profiling camera to record the power of the beam before and after the cell. An optimized optical system of the atomic magnetometer has been established by measuring the the number density variation in the spatial distribution in mm scale. The number density variation coefficient, which is introduced to evaluate the distribution homogeneity, increases from 0.0257 to 0.0333 when the temperature of the oven wall rises from 140°C to 190 °C, showing the same trend as the simulation results. The optical rotation distribution is calculated according to the magnetometer output signal formula. This study is of great interest for optimizing the oven structure and improving the stability of atomic spin polarization and sensitivity of the multichannel magnetometer.
Abstract A single-beam spin-exchange relaxation-free (SERF) atomic magnetometer can extract vector magnetic field information by detecting the transmission intensity of a resonant circularly polarized pumping beam, which depends sensitively on the atomic density of the alkali metal. We present a novel scheme to determine atomic density based on zero-field magnetic resonance. The resonance linewidth under different transverse DC magnetic fields is fitted by means of a quadratic function. The atomic density can be extracted from the quadratic coefficients of the fitted function. The experimental results indicate that the deviation of measured density is less than two times compared with the theoretical values between 378 K and 403 K. Furthermore, the influence of modulation field on resonance linewidth is investigated experimentally and theoretically. A miniature single-beam SERF atomic magnetometer with a sensor head volume of only 16.2 cm 3 and the measuring sensitivity of 40 fT/ Hz 1/2 has been achieved. These results should be beneficial for guiding the development of a chip-scale atomic magnetometer with high sensitivity and spatial resolution for bio-magnetic field imaging applications.
This study proposes an in situ method for measuring the equilibrium spin polarization and its longitudinal spatial distribution in a spin-exchange relaxation-free (SERF) atomic magnetometer. The total relaxation rate was determined by analyzing the steady-state response of the magnetometer to the triaxial magnetic field. The transfer coefficient between spin polarization along the probe beam axis and the steady-state response was derived from the optical depth of the probe light and the incident/transmitted power through the vapor cell. By applying a DC magnetic field along the sensitive axis and combining the total relaxation rate with the transfer coefficient, the equilibrium spin polarization value under zero-field conditions was obtained. The equilibrium spin polarization distribution along the pump beam propagation direction was measured, showing consistent trends with simulation results, with a maximum relative error of less than 5%. The expanded uncertainty of the proposed equilibrium spin polarization measurement method ranges from 0.8% to 9.7%. The advantages of this method include no requirement for additional optical field or magnetic field modulation, immunity to temperature and temperature gradients, and the capability to directly determine the equilibrium spin polarization value.
The electronic spin polarization of alkali-metal-vapor atoms is a pivotal parameter for atomic magnetometers. Herein, a novel method is presented for determining the spin polarization with a miniaturized single-beam spin-exchange-relaxation-free (SERF) magnetometer on the basis of zero-field cross-over resonance. Two separate laser beams are utilized to heat the cell and interrogate the vapor atoms, respectively. Spin polarization can be extracted by measuring the resonance response signal of the magnetometer to the transverse magnetic field under different irradiances. Results of these experiments are consistent well with the theoretical predictions with the maximum deviation less than 4%. The proposed method has the integrated advantages of possessing a simple configuration and in-situ measurement. Furthermore, combined with a homemade optical differential detection system with a factor of approximately three of the power noise suppression, the developed single-beam SERF atomic magnetometer with a measuring sensitivity of 32 fT/Hz 1/2 has been achieved. This demonstrated approach can help guide the development of chip-scale atomic magnetometers for bio-magnetic field imaging applications.
Atomic spin relaxation in a vapor cell, which can be characterized by the magnetic resonance linewidth (MRL), is an important parameter that eventually determines the sensitivity of an atomic magnetometer. In this paper, we have extensively studied how the pump intensity affects the spin relaxation. The experiment is performed with a cesium vapor cell, and the influence of the pump intensity on MRL is measured at room temperature at zero-field resonance. A simple model with five atomic levels of a Λ-like configuration is discussed theoretically, which can be used to represent the experimental process approximately, and the experimental results can be explained to some extent. Both the experimental and the theoretical results show a nonlinear broadening of the MRL when the pump intensity is increasing. The work helps to understand the mechanism of pump induced atomic spin relaxation in the atomic magnetometers.