Abstract A scanning optical quantum magnetometer with submicron spatial resolution is proposed that is based on the phenomenon of hole burning in the signal of optically detected magnetic resonance (ODMR) on atomic-sized color centers in silicon carbide crystals under conditions of spin level saturation by means of additional high-frequency resonance pumping. An increase in the sensitivity is achieved due to narrowing of the ODMR line and increasing slope of the dependence of signal frequency on the magnetic field.
The response of a spin exchange relaxation free atomic magnetometer to a repetitive short-pulsed pump was investigated. Quantum sub-resonances at a repetition rate of 1/n of the Larmor frequency of the magnetic field inside the shield are experimentally observed and theoretically explained. This is a type of synchronization phenomenon. Investigations in single alkali atom cells and mixed alkali atoms of K and Rb are presented. In the latter, one species is pumped while the probe is on the other species polarized by spin exchange. The effect of spin destruction, spin exchange, and collisions is studied in order to account for the width of the resonances. Quantum calculations of a three-level Λ model for this phenomenon exhibit a dip at the resonance frequency in the absorption spectrum for both cases of pulsed and cw pump modes and an evidence for electromagnetically induced transparency.
Quantum sensing aims to detect signals with unparalleled sensitivity, potentially surpassing classical limitations. Solid-state spin defects, particularly nitrogen-vacancy centers in diamond, have emerged as promising platforms due to their long coherence time, optical addressability, high field sensitivity, and spatial and spectral resolution, making them ideal for sensing and imaging applications. Their compact size and robust performance under room temperature and ambient conditions further enhance their suitability for real-world applications. We provide an overview of quantum sensing principles and explore efforts to improve sensor functionality, including advanced sensing protocols, spatial imaging techniques, and integration with optical systems to enhance detection efficiency. We also highlight recent progress in the applications of these sensors across various use cases, including biomedical diagnostics, semiconductor device inspection, and industrial and military applications.
The silicon vacancy center in Silicon Carbide (SiC) provides an optically addressable qubit at room temperature in its spin-
23 electronic state. However, optical spin initialization and readout are less efficient compared to those of spin-1 systems, such as nitrogen-vacancy centers in diamond, under non-resonant optical excitation. Spin-dependent fluorescence exhibits contrast only between
∣m=±3/2⟩ and
∣m=±1/2⟩ states, and optical pumping does not create a population difference between
∣+1/2⟩ and
∣−1/2⟩ states. Thus, operating one qubit (e.g.,
{∣+3/2⟩,∣+1/2⟩} states) leaves the population in the remaining state (
∣−1/2⟩ ) unaffected, contributing to background in optical readout. To mitigate this problem, we propose a sensing scheme based on duplex qubit operation in the quartet, using microwave pulses with two resonant frequencies to simultaneously operate
{∣+3/2⟩,∣+1/2⟩} and
{∣−1/2⟩,∣−3/2⟩} . Experimental results demonstrate that this approach doubles signal contrast in optical readout and improves sensitivity in AC magnetometry compared to simplex operation.
The detection of environmental magnetic fields is well established by optically pumped atomic magnetometers. Another focus of magnetometry can be the research on magnetic or spin-active solid-state samples. Here we introduce a simple and compact design of a rubidium-based Mx magnetometer, which allows for hosting solid-state samples. The optical, mechanical, and electrical design is reported, as well as simple measurements which introduce the ground-state spin-relaxation time, the signal-to-noise ratio of a measurement, and subsequently the overall sensitivity of the magnetometer. The magnetometer is optimized for the most sensitive operation with respect to laser power and magnetic field excitation at the Larmor frequency.
An optical magnetometer based on atomic coherence effects is analyzed using a quantum Langevin approach. The large dispersion of a phase-coherent atomic medium (``phaseonium'') at a point of vanishing absorption is used to detect magnetic level shifts via optical phase measurements in a Mach-Zehnder interferometer with sensitivities potentially superior to state-of-the-art devices. Effects of Doppler broadening and fluctuations of the driving field are discussed and a comparison to standard optical-pumping magnetometers is made.