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Quantum Electronics and Laser Science Conference

Measurement of laser-induced dispersion in a neon three-level system

Peter Jungner, Birger Stahlberg, Tomas Fellman, K.-A. Suomien, Stig Stenholm

Published May 12, 1991• 0 citations
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Abstract

The polarization state of laser light is affected by the nonlinear processes in the matter it passes through. Wieman and Hancsh’ used this effect to investigate the spectra of molecular systems. Another example is the laser-based investigations of parity-breaking weak interactions,2 In this contribution we investigate polarization changes induced by a three-level cascade system when laser light is used to break the left-right symmetry of the atom. By causing the asymmetry externally we can manipulate the effect and observe its magnitude and signal shape. Works related to ours are those by Liao and Bjorklund.3,4

Related papers

Laser-induced dispersion in a three-level system

Kalle‐Antti Suominen, Birger Stahlberg, Stig Stenholm

A theoretical calculation of the polarization changes of a weak probe laser beam as it traverses a strongly pumped gaseous atomic medium is presented. The medium is chosen to be a three-level cascade (J = 0–J = 1–J = 0) system. The polarization of the probe changes from linear to elliptical owing to the asymmetrical population transfer induced by a strong, circularly polarized pumping laser beam. We study this phenomenon as a function of laser intensities, laser detunings, and the relaxation parameters of the medium. We compare the predictions of the theory with results obtained from experimental studies of the neon 1s4(J = 1)–2p4(J = 2)–3s2(J = 1) system.

Journal of the Optical Society of America B•Sep 1, 1991•14 citations

Polarization dependence of Electromagnetic Induced Transparency in multilevel cascade system

Vineet Bharti, Ajay Wasan

A theoretical model using density matrix approach has been presented to show the polarization dependence of Electromagnetically Induced Transparency (EIT) in cascade multilevel atomic system. EIT has already been investigated both theoretically and experimentally by using three-level system in lambda (Λ), vee (V), and cascade (Ξ) configurations. However there is asymmetry in absorption measurement. To understand this asymmetry we introduce hyperfine levels in EIT cascade system. We present a five-level atomic system, which is a simple case of87Rb. This study has been extended to investigate the polarization dependence of probe and control lasers on EIT. It has been observed that there is significant change in transparency window for different laser polarizations.

International Conference on Optical Engineering (ICOE)•Jul 1, 2012•1 citation

Laser-induced dichroism and birefringence in two- and three-level systems of neon

Christian Delsart, J. Keller

We have observed the Doppler-free dichroism and birefringence induced by a linearly polarized laser beam (pump beam) by monitoring the polarization and amplitude changes of a weak probe beam through an analyzer. The effects have been observed in two-level systems and also in three-level systems of Ne I. At rather low pump power, a typical refractive-index anisotropy of 10−8 has been measured. We have shown that, when the normal resonance curve exhibits a broad background due to collisions, our method allows the elimination of this background. In addition, using a rotating analyzer, we have obtained simultaneously the dichroism and birefringence curves, i.e., the imaginary and real part of the anisotropic-induced susceptibility.

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Magneto-Optic Spectroscopy on Neon Using Laser-Induced Forward Scattering

Åsa Marie Lindberg

The forward-scattered light observed when a single-mode dye laser interacts with the three neon transitions 1 s 5 ( J = 2)-2 p s ( J = 2), 1s 3 ( J = 0)-2 p 5 ( J = 1), and 1 s 4 ( J = 1)-2 p 7 ( J = 1) has been investigated as an applied longitudinal magnetic field is varied. The 1 s 5 and the 1 s 3 states are metastable. This condition allows a comparison of the spectra for the cases 1 s 5 ( J = 2)-2 p 8 ( J = 2) and 1 s 3 ( J = 0)-2 p 5 ( J = 1) in order to discuss whether the complex line shapes obtained for the J = 2 to J = 2 atomic system are due to higher-order coherences or whether they originate from coherences between m = ±1 states. Experimental and calculated line shapes are presented. The calculations have been performed with the use of a semiclassical model for the light/matter interaction. A J = 0 to J = 1 (or a J = 1 to J = 1) model reproduces the overall shapes of the recorded spectra for all three transitions. The results show that, even when laser beam spatial effects and the sample isotopic effects are taken into account, interpretations of forward-scattering spectra in order to determine atomic parameters can reliably be done for simple J = 0 to J = 1 systems only.

Applied Spectroscopy•Dec 1, 1994•1 citation

Autler-Townes splitting of ultracold cesium Rydberg atoms

Xue Yong-Mei, Hao Li-Ping, Jiao Yue-Chun +4 more

Autler-Townes (A-T) splitting, known as an AC Stark effect, shows a change of an absorption/emission spectral line of a probe beam when an oscillating field is tuned in resonance with the atomic or molecular transition. The A-T splitting is observed in different three-level atoms and widely investigated in a vapor cell and in a magneto-optical trap (MOT). The A-T splitting plays an important role in the atom-based microwave electric-field measurements where a cascade three-level system involving Rydberg state is adopted. In this work, an A-T splitting is observed in an ultracold cesium Rydberg gas, which is cooled down to about 100 pK and center density is about 1010 cm-3 in a conventional MOT by using the laser cooling technology. We present the A-T spectrum in a ladder three-level atomic system involving a 34D5/2 Rydberg state. The cesium ground state (6S1/2), excited state (6P3/2) and Rydberg state (34D5/2) constitute a Rydberg three-level system. A coupling laser, locked to the Rydberg transition by using a Rydberg electromagnetically induced transparency signal that is obtained from a cesium room-temperature vapor cell, couples 6P3/2 (F'=5) 34D5/2 Rydberg transition. A weak probe laser, stabilized to a ground-state transition by using a polarization spectroscopy, is swept, covering the transition 6S1/2 (F=4) 6P3/2 (F'=5) with a double-passed acousto-optic modulator. The probe and coupling lasers are counter-propagated through the MOT center. The power of probe light is 200 pW, corresponding Rabi frequency p=21.05 MHz. During the experiment, 50 s after turning off the trapping laser, both the coupling and probe beams are switched on and last 100 s. The A-T spectrum as a function of the probe detuning is detected with a single-photon counter module detector. We use Gaussian multiple peak fitting to obtain the positions of the A-T peaks and the A-T splitting. The measured A-T splitting is proportional to the Rabi frequency of the coupling light. We numerically solve the density matrix equations to obtain the A-T spectrum, and the calculations reproduce A-T spectra well. The measured A-T splitting shows good agreement with the theoretical calculation for Rabi frequency of the coupling light c29 MHz. The A-T splitting is less than the calculation for the case of c29 MHz, the deviation is mainly attributed to the increased dephasing rate induced by the strong interaction between Rydberg atoms, whose number increases with the coupling laser Rabi frequency. In this work, the adopted method for the cascade three-level system involving Rydberg state is also suitable for -and V-type cases.

Acta Physica Sinica•Jan 1, 2017•3 citations

Laser induced polarization properties of a neon three-level system

Birger Stahlberg, Peter Jungner, Tomas Fellman +2 more

Optics Communications•Jun 1, 1990•6 citations
The polarization state of laser light is affected by the nonlinear processes in the matter it passes through. Wieman and Hancsh’ used this effect to investigate the spectra of molecular systems. Another example is the laser-based investigations of parity-breaking weak interactions,2 In this contribution we investigate polarization changes induced by a three-level cascade system when laser light is used to break the left-right symmetry of the atom. By causing the asymmetry externally we can manipulate the effect and observe its magnitude and signal shape. Works related to ours are those by Liao and Bjorklund.3,4
A theoretical calculation of the polarization changes of a weak probe laser beam as it traverses a strongly pumped gaseous atomic medium is presented. The medium is chosen to be a three-level cascade (J = 0–J = 1–J = 0) system. The polarization of the probe changes from linear to elliptical owing to the asymmetrical population transfer induced by a strong, circularly polarized pumping laser beam. We study this phenomenon as a function of laser intensities, laser detunings, and the relaxation parameters of the medium. We compare the predictions of the theory with results obtained from experimental studies of the neon 1s4(J = 1)–2p4(J = 2)–3s2(J = 1) system.
A theoretical model using density matrix approach has been presented to show the polarization dependence of Electromagnetically Induced Transparency (EIT) in cascade multilevel atomic system. EIT has already been investigated both theoretically and experimentally by using three-level system in lambda (Λ), vee (V), and cascade (Ξ) configurations. However there is asymmetry in absorption measurement. To understand this asymmetry we introduce hyperfine levels in EIT cascade system. We present a five-level atomic system, which is a simple case of87Rb. This study has been extended to investigate the polarization dependence of probe and control lasers on EIT. It has been observed that there is significant change in transparency window for different laser polarizations.
We have observed the Doppler-free dichroism and birefringence induced by a linearly polarized laser beam (pump beam) by monitoring the polarization and amplitude changes of a weak probe beam through an analyzer. The effects have been observed in two-level systems and also in three-level systems of Ne I. At rather low pump power, a typical refractive-index anisotropy of 10−8 has been measured. We have shown that, when the normal resonance curve exhibits a broad background due to collisions, our method allows the elimination of this background. In addition, using a rotating analyzer, we have obtained simultaneously the dichroism and birefringence curves, i.e., the imaginary and real part of the anisotropic-induced susceptibility.
The forward-scattered light observed when a single-mode dye laser interacts with the three neon transitions 1 s 5 ( J = 2)-2 p s ( J = 2), 1s 3 ( J = 0)-2 p 5 ( J = 1), and 1 s 4 ( J = 1)-2 p 7 ( J = 1) has been investigated as an applied longitudinal magnetic field is varied. The 1 s 5 and the 1 s 3 states are metastable. This condition allows a comparison of the spectra for the cases 1 s 5 ( J = 2)-2 p 8 ( J = 2) and 1 s 3 ( J = 0)-2 p 5 ( J = 1) in order to discuss whether the complex line shapes obtained for the J = 2 to J = 2 atomic system are due to higher-order coherences or whether they originate from coherences between m = ±1 states. Experimental and calculated line shapes are presented. The calculations have been performed with the use of a semiclassical model for the light/matter interaction. A J = 0 to J = 1 (or a J = 1 to J = 1) model reproduces the overall shapes of the recorded spectra for all three transitions. The results show that, even when laser beam spatial effects and the sample isotopic effects are taken into account, interpretations of forward-scattering spectra in order to determine atomic parameters can reliably be done for simple J = 0 to J = 1 systems only.
Autler-Townes (A-T) splitting, known as an AC Stark effect, shows a change of an absorption/emission spectral line of a probe beam when an oscillating field is tuned in resonance with the atomic or molecular transition. The A-T splitting is observed in different three-level atoms and widely investigated in a vapor cell and in a magneto-optical trap (MOT). The A-T splitting plays an important role in the atom-based microwave electric-field measurements where a cascade three-level system involving Rydberg state is adopted. In this work, an A-T splitting is observed in an ultracold cesium Rydberg gas, which is cooled down to about 100 pK and center density is about 1010 cm-3 in a conventional MOT by using the laser cooling technology. We present the A-T spectrum in a ladder three-level atomic system involving a 34D5/2 Rydberg state. The cesium ground state (6S1/2), excited state (6P3/2) and Rydberg state (34D5/2) constitute a Rydberg three-level system. A coupling laser, locked to the Rydberg transition by using a Rydberg electromagnetically induced transparency signal that is obtained from a cesium room-temperature vapor cell, couples 6P3/2 (F'=5) 34D5/2 Rydberg transition. A weak probe laser, stabilized to a ground-state transition by using a polarization spectroscopy, is swept, covering the transition 6S1/2 (F=4) 6P3/2 (F'=5) with a double-passed acousto-optic modulator. The probe and coupling lasers are counter-propagated through the MOT center. The power of probe light is 200 pW, corresponding Rabi frequency p=21.05 MHz. During the experiment, 50 s after turning off the trapping laser, both the coupling and probe beams are switched on and last 100 s. The A-T spectrum as a function of the probe detuning is detected with a single-photon counter module detector. We use Gaussian multiple peak fitting to obtain the positions of the A-T peaks and the A-T splitting. The measured A-T splitting is proportional to the Rabi frequency of the coupling light. We numerically solve the density matrix equations to obtain the A-T spectrum, and the calculations reproduce A-T spectra well. The measured A-T splitting shows good agreement with the theoretical calculation for Rabi frequency of the coupling light c29 MHz. The A-T splitting is less than the calculation for the case of c29 MHz, the deviation is mainly attributed to the increased dephasing rate induced by the strong interaction between Rydberg atoms, whose number increases with the coupling laser Rabi frequency. In this work, the adopted method for the cascade three-level system involving Rydberg state is also suitable for -and V-type cases.