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上海交通大学学报：英文版

Excitonic Doppler-Rabi Oscillations in a Moving Organic Slab

Yao Ming

Published Jan 1, 2005• 0 citations
OpenAlex

Abstract

It is theoretically shown that excitonic Doppler-Rabi oscillations can occur in an organic slab moving along the axis of a high-Q cavity. Due to the N enhancement of the vacuum Rabi frequency, this effect can be more eas ily observed than that in a moving two-level atom.

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The dynamics of energy exchange between an atom moving in a high-Q cavity and the cavity field is analyzed by taking into account the Roentgen interaction. A two-level atom coupled to a Fock or coherent state of an optical or microwave cavity is considered. The mean cavity photon number required for high-frequency Doppler-Rabi oscillations to occur is relatively high for both Fock-and coherent-state cavity fields and increases with the atomic transition frequency. Conditions are found when the Roentgen interaction plays a key role in the Doppler-Rabi oscillations and must be taken into account, in addition to the conventional electric field-dipole interaction.
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Recently, cavity quantum electrodynamic (QED) effects in semiconductor microcavities have been of considerable interest since, in the weak-coupling regime they play an important role in selectively increasing spontaneous emission into the lasing mode of vertical-cavity surface-emitting lasers (VCSEL’s) [1,2], enabling low-threshold, high speed, and high efficiency. In a strong-coupling regime, the normal modes of the coupled system are superpositions of the exciton and cavity modes. Hence the impulsively excited system will evolve in time with the energy oscillating between the exciton and cavity modes. This is known as a vacuum-Rabi oscillation (VRO), with a frequency of Ω=d¯⋅E¯/@@h, where d¯ is the transition dipole moment of atoms and E¯ the vacuum-field strength. Of course, VRO are observable only when the cavity lifetime and exciton dephasing time are long enough compared to VRO period. Recently, Weisbuch et al. [3] have reported an observation of the normal-mode vacuum Rabi splitting in 2-D-exciton/planar-DBR microcavities. The observed splittings were as large as 6 meV in reflection and transmission spectra, implying 690-fs vacuum Rabi oscillations.
We study analytically and numerically vacuum Rabi oscillations of N identical two-level atoms moving through a single-mode lossless cavity. Equations of motion which take into account the atomic quantum correlations are obtained for the quantum mechanical expectation values in the strong-coupling, rotating-wave, pointlike, and Raman-Nath approximations. It is shown that moving atoms may demonstrate an unusual type of spontaneous emission, the chaotic vacuum Rabi oscillations. This manifestation of quantum dynamical chaos in the matter-vacuum interaction is caused by a spatial inhomogeneity of the cavity mode that modulates the vacuum Rabi frequency of moving atoms. For small values of the depth of this modulation we use the Melnikov method and show analytically the presence of homoclinic chaos in this interaction. Transition to global chaos and global phase space stochasticity under conditions of the strong modulation are studied numerically by computing the maximal Lyapunov exponent lambda of the atom-field dynamical system as a function of the number and velocity of atoms and detuning. We find a curious structure of the lambda(N) dependence reflecting an intermittent route to global chaos. The strength of chaos depends strongly on the initial state preparation of atoms just before injecting into a cavity. It is shown that initially fully inverted atoms, which are in a superfluorescent Dicke state, demonstrate much stronger chaos (under other equal conditions) than the atoms prepared initially in a superradiant state with macroscopic polarization. A maser operating with two-level Rydberg atoms to be injected into a high-Q superconducting microwave cavity seems to be a realistic device for observing some manifestations of the chaotic vacuum Rabi oscillations.