In this thesis I theoretically study quantum states of ultracold atoms. The majority of the Chapters focus on engineering specific quantum states of single atoms with high fidelity in experimentally realistic systems. In the sixth Chapter, I investigate the stability and dynamics of new multidimensional solitonic states that can be created in inhomogeneous atomic Bose-Einstein condensates. In Chapter three I present two papers in which I demonstrate how the coherent tunnelling by adiabatic passage (CTAP) process can be implemented in an experimentally realistic atom chip system, to coherently transfer the centre-of-mass of a single atom between two spatially distinct magnetic waveguides. In these works I also utilise GPU (Graphics Processing Unit) computing which offers a significant performance increase in the numerical simulation of the Schrödinger equation. In Chapter four I investigate the CTAP process for a linear arrangement of radio frequency traps where the centre-of-mass of both, single atoms and clouds of interacting atoms, can be coherently controlled. In Chapter five I present a theoretical study of adiabatic radio frequency potentials where I use Floquet theory to more accurately model situations where frequencies are close and/or field amplitudes are large. I also show how one can create highly versatile 2D adiabatic radio frequency potentials using multiple radio frequency fields with arbitrary field orientation and demonstrate their utility by simulating the creation of ring vortex solitons. In the sixth Chapter I discuss the stability and dynamics of a family of multidimensional solitonic states created in harmonically confined Bose-Einstein condensates. I demonstrate that these solitonic states have interesting dynamical instabilities, where a continuous collapse and revival of the initial state occurs. Through Bogoliubov analysis, I determine the modes responsible for the observed instabilities of each solitonic state and also extract information related to the time at which instability can be observed.
In this thesis I theoretically study quantum states of ultracold atoms. The majority of the Chapters focus on engineering specific quantum states of single atoms with high fidelity in experimentally realistic systems. In the sixth Chapter, I investigate the stability and dynamics of new multidimensional solitonic states that can be created in inhomogeneous atomic Bose-Einstein condensates. In Chapter three I present two papers in which I demonstrate how the coherent tunnelling by adiabatic passage (CTAP) process can be implemented in an experimentally realistic atom chip system, to coherently transfer the centre-of-mass of a single atom between two spatially distinct magnetic waveguides. In these works I also utilise GPU (Graphics Processing Unit) computing which offers a significant performance increase in the numerical simulation of the Schrödinger equation. In Chapter four I investigate the CTAP process for a linear arrangement of radio frequency traps where the centre-of-mass of both, single atoms and clouds of interacting atoms, can be coherently controlled. In Chapter five I present a theoretical study of adiabatic radio frequency potentials where I use Floquet theory to more accurately model situations where frequencies are close and/or field amplitudes are large. I also show how one can create highly versatile 2D adiabatic radio frequency potentials using multiple radio frequency fields with arbitrary field orientation and demonstrate their utility by simulating the creation of ring vortex solitons. In the sixth Chapter I discuss the stability and dynamics of a family of multidimensional solitonic states created in harmonically confined Bose-Einstein condensates. I demonstrate that these solitonic states have interesting dynamical instabilities, where a continuous collapse and revival of the initial state occurs. Through Bogoliubov analysis, I determine the modes responsible for the observed instabilities of each solitonic state and also extract information related to the time at which instability can be observed.
Bose-Einstein condensates (BECs), a quantum state of matter formed when bosonic atoms are cooled close to absolute zero, have become the premier platform for investigating fundamental physics with atomic vapours. Experiments on Bose-Einstein condensates now achieve exquisite control over many aspects of the system, including interactions, trapping potential, and dynamics. This has precipitated a new wave of research into many-body quantum phenomena and, in particular, solitons. These structures are fundamental excitations of an interacting non-linear medium, of interest to a multitude of scientific disciplines from non-linear optics to financial markets. The highly controllable environment of BECs form an attractive playground for the study of solitons allowing the non-linearity to be dynamically tuned, facilitating deeper investigations into these structures. Consistently generating and analysing solitons in BEC experiments continues to be problematic. In particular, the non-linear dynamics of BECs, though required for the generation of solitons, produce particularly challenging control and optimization problems. These control problems must be solved before further investigations into the fundamental physics of soliton dynamics can be answered. This thesis makes three important advances in the control and measurement of BECs that will lead to better generation and observation of solitons. (1) a theoretical model for a control scheme capable of highly precise wavefunction engineering, (2) the experimental implementation of a machine learning algorithm for online optimisation, and (3) a continuous non-destructive imaging system capable of directly observing soliton dynamics in real-time. Together, these advances provide a suite of tools for manipulating and exploiting solitons in Bose-Einstein condensates. A novel technique was developed theoretically, offering control of the macroscopic wavefunction of a Bose-Einstein condensate with unprecedented spatial resolution and speed. The ability to control the atomic wavefunction at the fundamental length scale is key to the advancement of many quantum technologies such as quantum simulators. The magnetic resonance control scheme is demonstrated through simulation of a 87Rb condensate with the exemplar model generating a single dark soliton with corresponding π phase kink. The soliton represents a structure at the fundamental length scale of the system, and demonstrates the potential of the scheme for precision state engineering. The scheme is extended to generate higher-order soliton modes which are yet to be experimentally realised. A machine learning algorithm based on Gaussian processes was developed and implemented on the evaporative cooling stage of the production of a 87Rb Bose-Einstein condensate, successfully demonstrating fast optimisation to condensation. The Gaussian process develops a statistical model based on the data that enables the characterisation of the relationship between the experimental controls and resultant quality of the BEC. This relationship is often obfuscated through technical details of the apparatus, frustrating the use of theoretical models to design optimal evaporation ramps. These models often only consider ergodic dynamics with two-body s-wave interactions and no other loss rates with better ramps likely exploiting more complex interactions. The internal model generated from the Gaussian process utilised uncertainty in measured data, making the optimisation more robust to experimental noise than alternate methods. The algorithm is shown to produce high quality Bose-Einstein condensates in 10 times fewer experimental iterations than previously used online optimisation techniques. By exploiting information on the sensitivity of each control, the model can be used to aid experimental design. The convergence of the optimisation is further improved by eliminating a superfluous parameter identified by the model. The general usefulness of machine learning compared with bespoke optimisation algorithms has seen machine learning approach ubiquity. Finally, an experimentally straightforward technique for continuous non-destructive imaging of matter-wave solitons was developed and implemented, facilitating measurements of stochastic phenomena. The technique is readily practicable on any ultracold atom experiment with an existing absorption imaging system, simply requiring the probe laser be far-detuned from resonance. With a signal-to-noise of ∼ 33 at 1.25 GHz detuning, the technique is capable of producing 100 images with no observable heating or atom loss. Coupled with a fast optical phase locked loop, the technique can be used in conjunction with absorption imaging to generate a series of non-destructive images followed by a final high signal-to-noise absorption image solely through moving the laser on resonance for the final image. The high performance and utility of this imaging setup make it a powerful tool for ultra-cold atom experiments.
This thesis includes theoretical studies regarding stability and manipulation of Bose-Einstein condensates (BECs) of ultra-cold atoms in 2D trapping geometry, as well as formation of steady states of exciton-polariton Bose-Einstein condensates created in solid states. We analyze and numerically model the dynamics and localization of the condensates using mean-field model. Chapter 1 contains an introduction to the physics of ultra-cold atom BEC and excitonpolariton BEC which provides a framework for the work presented in later chapters. In Chapter 2, we consider a method for achieving dynamically controllable transport of highly mobile matter-wave solitons in an ultra-cold atom BEC with attractive interparticle interaction loaded into a driven two-dimensional optical lattice. Our numerical analysis based on the mean-field model and the theory based on the effective particle approach demonstrate that fast, time-periodic rocking of the two-dimensional optical lattice enables efficient stabilization and manipulation of spatially localized matter wave packets via induced reconfigurable mobility channels. Chapter 3 consists of an investigation of the instability - collapse of a BEC with attractive interactions. In this chapter we explore the influence of an orbital angular momentum on the collapse of vortex-free elliptic clouds of Bose-Einstein condensates trapped in a radially symmetric harmonic potential or a rotating elliptic potential. The results of our analysis show that the number of trapped ultracold atoms corresponding to the collapse threshold can be radically increased for such rotating nonlinear matter waves in a radially harmonic trap. The results corresponding to a BEC cloud confined in a rotating elliptic trap show that the elongated stationary states can be parallel or perpendicular to the long axis of the trap and display bistable nature. In Chapter 4, we examine spatial localization and dynamical stability of Bose-Einstein condensates of exciton-polaritons in microcavities under the condition of off-resonant spatially inhomogeneous optical pumping both with and without a harmonic trapping potential. We employ the open-dissipative Gross-Pitaevskii model for describing an incoherently pumped polariton condensate coupled to an exciton reservoir. We reveal that spatial localization of the steady-state condensate occurs due to effective self-trapping created by the polariton flows, regardless of the presence of the external potential. A ground state of the polariton condensate with repulsive interactions between the quasiparticles represents a dynamically stable bright dissipative soliton. We also investigate the conditions for sustaining spatially localized structures, with nonzero angular momentum, in the form of single-charge vortices. Chapter 5 consider the existence of novel spatially localized states of exciton-polariton Bose-Einstein condensates in semiconductor microcavities with fabricated periodic inplane potentials. Our theory shows that, under the conditions of continuous nonresonant pumping, localization is observed for a wide range of optical pump parameters due to effective potentials self-induced by the polariton flows in the spatially periodic system. We show that the self-localization of exciton-polaritons in the lattice may occur both in the gaps and bands of the single-particle linear spectrum, and is dominated by the effects of gain and dissipation rather than the structured potential, in sharp contrast to the conservative condensates of ultra-cold alkali atoms.
This thesis describes the formation of a 85Rb Bose-Einstein condensate and the subsequent creation of a bright solitary matter-wave in a quasi-one-dimensional optical waveguide, with experiments investigating the dynamics of a solitary wave in comparison with a repulsive Bose-Einstein condensate. In the final chapters of this thesis, progress towards the interaction of a solitary wave with a narrow barrier and an attractive atom-surface potential is presented. Beyond the above, a review of recent soliton and solitary wave theory is presented from the perspective of an experimentalist, culminating in the numerical analysis of a variety of key areas, namely, quantum reflection, solitary wave size and solitary wave profile. The modelling and experimental results relating to the merging of ultracold gases of 85Rb and 87Rb, in order to create isotopic mixtures, is also described within this thesis. Such a scheme could be used as an initial step in the process of forming molecules or undertaking sympathetic cooling. Finally, the creation of a complex LabVIEW based experimental control system is also described within.
Coherent transport by adiabatic passage has recently been suggested as a high-fidelity technique to engineer the center-of-mass state of single atoms in inhomogeneous environments. While the basic theory behind this process is well understood, several conceptual challenges for its experimental observation have still to be addressed. One of these is the difficulty that currently available optical or magnetic micro-trap systems have in adjusting the tunneling rate time dependently while keeping resonance between the asymptotic trapping states at all times. Here we suggest that both requirements can be fulfilled to a very high degree in an experimentally realistic setup based on radio-frequency traps on atom chips. We show that operations with close to 100 fidelity can be achieved and that these systems also allow significant improvements for performing adiabatic passage with interacting atomic clouds.
Experiments on attractive Bose-Einstein condensates (BECs) have unlocked many intriguing out-of-equilibrium dynamics through the interplay between matter-wave dispersion and nonlinear attractive interaction. Competition between these effects leads to fascinating phenomena such as wave collapse, modulational instability, and formation of multidimensional bright solitons. This chapter reviews experimental studies on attractive condensates, with a primary focus on alkali atoms featuring two-body contact interactions. We review recent experimental advances in optical trapping and interaction control techniques, which have enabled new studies on attractive condensates in three and also in lower dimensions. Specifically, we discuss pioneering and recent experimental observations on the dynamics and stability of attractive BECs, including the formation of bright solitons, their collisions, and excitations in quasi-one-dimensional traps. Recent observations of the elusive two-dimensional Townes solitons and vortex solitons are also discussed in this Chapter. We then highlight an experimental technique revealing the nonclassical signatures of modulational instability in an attractive condensate.