Bose-Einstein condensates (BECs), a quantum state of matter formed when bosonic atoms are cooled close to absolute zero, have become the premier platform for investigating fundamental physics with atomic vapours. Experiments on Bose-Einstein condensates now achieve exquisite control over many aspects of the system, including interactions, trapping potential, and dynamics. This has precipitated a new wave of research into many-body quantum phenomena and, in particular, solitons. These structures are fundamental excitations of an interacting non-linear medium, of interest to a multitude of scientific disciplines from non-linear optics to financial markets. The highly controllable environment of BECs form an attractive playground for the study of solitons allowing the non-linearity to be dynamically tuned, facilitating deeper investigations into these structures. Consistently generating and analysing solitons in BEC experiments continues to be problematic. In particular, the non-linear dynamics of BECs, though required for the generation of solitons, produce particularly challenging control and optimization problems. These control problems must be solved before further investigations into the fundamental physics of soliton dynamics can be answered. This thesis makes three important advances in the control and measurement of BECs that will lead to better generation and observation of solitons. (1) a theoretical model for a control scheme capable of highly precise wavefunction engineering, (2) the experimental implementation of a machine learning algorithm for online optimisation, and (3) a continuous non-destructive imaging system capable of directly observing soliton dynamics in real-time. Together, these advances provide a suite of tools for manipulating and exploiting solitons in Bose-Einstein condensates. A novel technique was developed theoretically, offering control of the macroscopic wavefunction of a Bose-Einstein condensate with unprecedented spatial resolution and speed. The ability to control the atomic wavefunction at the fundamental length scale is key to the advancement of many quantum technologies such as quantum simulators. The magnetic resonance control scheme is demonstrated through simulation of a 87Rb condensate with the exemplar model generating a single dark soliton with corresponding π phase kink. The soliton represents a structure at the fundamental length scale of the system, and demonstrates the potential of the scheme for precision state engineering. The scheme is extended to generate higher-order soliton modes which are yet to be experimentally realised. A machine learning algorithm based on Gaussian processes was developed and implemented on the evaporative cooling stage of the production of a 87Rb Bose-Einstein condensate, successfully demonstrating fast optimisation to condensation. The Gaussian process develops a statistical model based on the data that enables the characterisation of the relationship between the experimental controls and resultant quality of the BEC. This relationship is often obfuscated through technical details of the apparatus, frustrating the use of theoretical models to design optimal evaporation ramps. These models often only consider ergodic dynamics with two-body s-wave interactions and no other loss rates with better ramps likely exploiting more complex interactions. The internal model generated from the Gaussian process utilised uncertainty in measured data, making the optimisation more robust to experimental noise than alternate methods. The algorithm is shown to produce high quality Bose-Einstein condensates in 10 times fewer experimental iterations than previously used online optimisation techniques. By exploiting information on the sensitivity of each control, the model can be used to aid experimental design. The convergence of the optimisation is further improved by eliminating a superfluous parameter identified by the model. The general usefulness of machine learning compared with bespoke optimisation algorithms has seen machine learning approach ubiquity. Finally, an experimentally straightforward technique for continuous non-destructive imaging of matter-wave solitons was developed and implemented, facilitating measurements of stochastic phenomena. The technique is readily practicable on any ultracold atom experiment with an existing absorption imaging system, simply requiring the probe laser be far-detuned from resonance. With a signal-to-noise of ∼ 33 at 1.25 GHz detuning, the technique is capable of producing 100 images with no observable heating or atom loss. Coupled with a fast optical phase locked loop, the technique can be used in conjunction with absorption imaging to generate a series of non-destructive images followed by a final high signal-to-noise absorption image solely through moving the laser on resonance for the final image. The high performance and utility of this imaging setup make it a powerful tool for ultra-cold atom experiments.
Bose-Einstein condensates (BECs), a quantum state of matter formed when bosonic atoms are cooled close to absolute zero, have become the premier platform for investigating fundamental physics with atomic vapours. Experiments on Bose-Einstein condensates now achieve exquisite control over many aspects of the system, including interactions, trapping potential, and dynamics. This has precipitated a new wave of research into many-body quantum phenomena and, in particular, solitons. These structures are fundamental excitations of an interacting non-linear medium, of interest to a multitude of scientific disciplines from non-linear optics to financial markets. The highly controllable environment of BECs form an attractive playground for the study of solitons allowing the non-linearity to be dynamically tuned, facilitating deeper investigations into these structures. Consistently generating and analysing solitons in BEC experiments continues to be problematic. In particular, the non-linear dynamics of BECs, though required for the generation of solitons, produce particularly challenging control and optimization problems. These control problems must be solved before further investigations into the fundamental physics of soliton dynamics can be answered. This thesis makes three important advances in the control and measurement of BECs that will lead to better generation and observation of solitons. (1) a theoretical model for a control scheme capable of highly precise wavefunction engineering, (2) the experimental implementation of a machine learning algorithm for online optimisation, and (3) a continuous non-destructive imaging system capable of directly observing soliton dynamics in real-time. Together, these advances provide a suite of tools for manipulating and exploiting solitons in Bose-Einstein condensates. A novel technique was developed theoretically, offering control of the macroscopic wavefunction of a Bose-Einstein condensate with unprecedented spatial resolution and speed. The ability to control the atomic wavefunction at the fundamental length scale is key to the advancement of many quantum technologies such as quantum simulators. The magnetic resonance control scheme is demonstrated through simulation of a 87Rb condensate with the exemplar model generating a single dark soliton with corresponding π phase kink. The soliton represents a structure at the fundamental length scale of the system, and demonstrates the potential of the scheme for precision state engineering. The scheme is extended to generate higher-order soliton modes which are yet to be experimentally realised. A machine learning algorithm based on Gaussian processes was developed and implemented on the evaporative cooling stage of the production of a 87Rb Bose-Einstein condensate, successfully demonstrating fast optimisation to condensation. The Gaussian process develops a statistical model based on the data that enables the characterisation of the relationship between the experimental controls and resultant quality of the BEC. This relationship is often obfuscated through technical details of the apparatus, frustrating the use of theoretical models to design optimal evaporation ramps. These models often only consider ergodic dynamics with two-body s-wave interactions and no other loss rates with better ramps likely exploiting more complex interactions. The internal model generated from the Gaussian process utilised uncertainty in measured data, making the optimisation more robust to experimental noise than alternate methods. The algorithm is shown to produce high quality Bose-Einstein condensates in 10 times fewer experimental iterations than previously used online optimisation techniques. By exploiting information on the sensitivity of each control, the model can be used to aid experimental design. The convergence of the optimisation is further improved by eliminating a superfluous parameter identified by the model. The general usefulness of machine learning compared with bespoke optimisation algorithms has seen machine learning approach ubiquity. Finally, an experimentally straightforward technique for continuous non-destructive imaging of matter-wave solitons was developed and implemented, facilitating measurements of stochastic phenomena. The technique is readily practicable on any ultracold atom experiment with an existing absorption imaging system, simply requiring the probe laser be far-detuned from resonance. With a signal-to-noise of ∼ 33 at 1.25 GHz detuning, the technique is capable of producing 100 images with no observable heating or atom loss. Coupled with a fast optical phase locked loop, the technique can be used in conjunction with absorption imaging to generate a series of non-destructive images followed by a final high signal-to-noise absorption image solely through moving the laser on resonance for the final image. The high performance and utility of this imaging setup make it a powerful tool for ultra-cold atom experiments.
To engineer the wavefunction of a Bose–Einstein condensate is to exert control over both the density and phase of the Bose–Einstein condensate order parameter. Having the ability to engineer the condensate order parameter down to the smallest length scale relevant to condensate dynamics—the healing length scale—would enable the study of new combinations of topological defects and may pave the way to using Bose–Einstein condensates as versatile, precise quantum simulators. In this thesis, we present a new wavefunction engineering technique which reaches the sub-optical healing length scale. Influenced by magnetic resonance imaging, we name this technique magnetic resonance control. This technique uses time-varying coupling between internal spin states of a spinor Bose–Einstein condensate within a magnetic field gradient to address spatial regions of the condensate, enabling control over both the phase and the density of the condensate order parameter down to the healing length scale. Techniques already exist to engineer condensate wavefunctions, but not with such a fine degree of control. These techniques primarily rely on either the intensity variation of a laser beam, which limits the resolution to the diffraction limit (larger than the typically sub-optical healing length scale), or the adiabatic inversion of a magnetic trapping potential, which can not be easily changed to produce a variety of structures in the condensate wavefunction. To develop our magnetic resonance control technique, we simulate a spinor condensate in one dimension with time-dependent coupling between spin states and time-dependent external magnetic field gradients using the Gross–Pitaevskii equation. We show that magnetic resonance control can engineer a single black soliton using experimentally feasible parameters. A black soliton is an ideal target state to select for this demonstration because engineering such a state requires control over both the phase and density of the condensate with healing-length resolution. We demonstrate that magnetic resonance control can be extended to engineer more complicated target states by simulating the creation of multiple solitons in a condensate, with control over the initial positions and trajectories of the solitons. When magnetic resonance control is applied to Bose–Einstein condensates in the laboratory, it will be necessary to have an imaging system capable of resolving the fine structures created. As an alternative to high-cost, custom-manufactured lenses, and in-vacuum optical systems, I have designed and bench-tested an objective lens with a high numerical aperture (0.36) and a long working distance (35 mm) consisting of standard catalogue lenses. Using 780 nm light, suitable for imaging rubidium condensates, this objective can achieve a resolution of 1.3 μm across a diffraction-limited field of view of 360 μm through a 5 mm thick glass window of a science cell. By changing the spacing between the lens elements, this objective lens can compensate for the aberrations produced by a glass window up to 15 mm thick, and by changing the aperture size the objective becomes suitable for diffraction-limited monochromatic imaging on the D2 line of all the alkalis. Before performing proof-of-principle magnetic resonance control experiments on real Bose–Einstein condensates, we needed to construct an experimental apparatus capable of producing spinor Bose–Einstein condensates. In this thesis I summarise my main contributions to this group endeavour, including: constructing the ultra-high vacuum system; supervising the bakeout of our vacuum system; designing and aligning the optical systems to produce laser beams of different, tunable frequencies to trap, cool, and image rubidium gas; trapping a cloud of rubidium atoms in a magneto-optical trap; constructing laser beam shutters, photodetectors, and photodetector signal filters; and designing and constructing our side imaging and top imaging systems. Using our spinor Bose–Einstein condensate apparatus, I performed the first proof-of-principle magnetic resonance control experiments. With a pair of condensates side-by-side, separated by 200 μm, we can use magnetic resonance control to invert the spin of one condensate only, while leaving the other condensate unaffected. We anticipate magnetic resonance control being used in the laboratory to engineer the first black soliton in a Bose–Einstein condensate. Looking beyond solitons, magnetic resonance control could have applications to the field of magnon spintronics, and extending the technique to higher dimensions could enable the study of exotic topological defects such as spin knots in a quantum fluid.
This thesis presents the development of an experimental apparatus to produce Bose-Einstein condensates (BECs) with tunable interparticle interactions. The ability to precisely control the strength of these interactions, and even to switch them from repulsive to attractive, allows one to probe novel regimes of condensate physics, from the collapse of attractively interacting BECs and the formation of solitary matter-waves to the observation of beyond mean-field effects in strongly repulsive condensates. The construction and characterisation of both a single and crossed beam optical dipole trap is presented. In the single beam case we develop a technique allowing the guided transport of atoms along the beam and up to a room-temperature surface; a technique which can be used to evaporatively cool the trapped atomic cloud. We produce Bose-Einstein condensates of 87Rb in the F=1, mF=-1 state in this trap, comparing the effect of beam waist on the evaporation trajectory. In the crossed beam trap Bose-Einstein condensation of 87Rb is realised in three distinct trapping configurations, along with a 1D optical lattice formed by changing the polarisation of the beams. A method of direct cooling of 85Rb atoms in the crossed trap is developed using a magnetic Feshbach resonance to precisely tune both the elastic and inelastic scattering properties of the atoms. The resonance used for this work occurs at 155G in collisions between atoms in the F=2, mF=-2 state of 85Rb. Bose-Einstein condensates of up to 40,000 85Rb atoms are formed in this trap and we demonstrate the presence of tunable interatomic interactions, exploring the collapse phenomenon associated with attractive condensates. By loading the 85Rb condensate into a quasi-1D waveguide we show that stable attractive condensates can be created, taking the form of bright solitary matter-waves. We observe a solitary wave of ~2,000 atoms which propagates, without dispersion, along the waveguide over a distance of ~1.1mm. The particle-like nature of the solitary wave is demonstrated by classical reflection of the wavepacket from a repulsive Gaussian barrier.
Summary form only given. Bose-Einstein condensates (BEC) of weakly interacting gases allow for the new regime of nonlinear atom optics. Of special interest are macroscopically excited states like dark solitons or vortices. Solitons, as particle like excitations of matter wave fields, provide a link from condensate physics to fluid mechanics, nonlinear optics and fundamental particle physics. Dark solitons in matter waves are characterized by a local density minimum and, a steep phase gradient of the wavefunction at the position of the minimum. We report on experimental and theoretical investigation of dark solitons in BECs of /sup 87/Rb which are produced by the method of phase imprinting. A highly anisotropic confining potential allows us to be close to the (quasi) 1D situation where dark solitons are expected to be dynamically stable. By monitoring the evolution of the density profile we observe the evolution of density minima travelling at a smaller velocity than the speed of sound. By comparison to analytical and numerical solutions of the 3D Gross-Pitaevskii equation for our experimental conditions we identify these density minima to be moving dark solitons. We have studied in detail the creation and the dynamics of dark solitons as a function of evolution time and imprinted phase.
We present experiments investigating different aspects concerning the coherent manipulation of a Bose-Einstein condensate wavefunction with far blue detuned dipole potentials. In a first set of experiments we study a waveguide for matter waves as an important atom optical element allowing to hold and guide the atoms for long observation times. We present a flexible realization of this waveguide based on a tube shaped Laguerre Gaussian laser beam and investigate the dynamics of a Bose condensed ensemble transferred into this guide. In a second set of experiments we study the dynamics of dark solitons created by the manipulation of the phase of the condensate wave function by temporally applied dipole potentials. This method of phase imprinting represents a powerful tool for the design of matter waves and the controlled creation of various excitations. The dynamics of dark solitons in matter waves is investigated in detail by experimentally and numerically studying the temporal evolution of the condensate density as well as by mapping the velocity field of the excited condensate wavefunction. In these measurements we directly detect the flux of the wave function associated with the dark soliton using spatially resolved Bragg scattering. Experiments investigating the creation and interaction of several dark solitons conclude this chapter.
In this habilitation-thesis a collection of 14 experiments is presented. In these experiments we have developed and used novel techniques to control ultracold gases on the quantum level. In brief, Bose-Einstein condensates (BEC) and degenerate Fermi gases of laser-cooled alkali atoms are subjected to specially designed optical and magnetic fields. The fields influence in a coherent way the behavior, properties and dynamics of the gases. On this basis we developed tools to prepare, coherently manipulate, and analyze pre-defined quantum states. With this high level of control, it was possible to investigate interesting physics phenomena, and we were able to achieve several breakthroughs in the field of ultracold atoms. Highlights of our experimental results include the demonstration of phase engineering of a BEC wavefunction where we created solitons in a BEC and studied their propagation. In another experiment we constructed a spatially resolved matter wave interferometer with which we mapped out the phase distribution on a condensate. Illuminating the BEC with a periodic pattern, i.e. an optical lattice, allowed us to study solid states physics phenomena. In a second set of experiments we demonstrated optically tuning of the interaction between atoms with optical Feshbach resonances. Employing either magnetically tunable Feshbach resonances or laser radiation, we were able to produce ground state molecules in well defined quantum states. This led to the production of the first molecular BEC. By tuning the coupling of atom pairs in a Fermi gas of atoms, we could for the first time investigate the so-called BEC-BCS crossover which describes the continuous change from a BEC superfluid to a Bardeen-Cooper Schrieffer (BCS) superfluid. Due to the excellent control on the quantum level, the developed cold atom techniques open up intriguing prospects for future applications and experiments. They represent a general tool box to investigate fundamental physical phenomena in a pure and undisturbed environment. In the future, cold atoms might serve as a testing ground for fundamental theories or as quantum simulators for complex systems.
Bose–Einstein Condensation (BEC) of atomic gases has attracted a renewed theoretical and experimental interest in quantum many-body systems at extremely low temperatures (Pethick & Smith; 2002). This excitement stems from two favorable features: (1) by applying magnetic fields and lasers, most of the system parameters, such as the shape, dimensionality, internal states of the condensates, and even the strength of the interatomic interactions, are controllable; (2) due to the diluteness, the mean-field theory explains experiments quite well. In particular, the Gross–Pitaevskii (GP) equation demonstrates its validity as a basic equation for the condensate dynamics. The GP equation is the counterpart of the nonlinear Schrodinger (NLS) equation in nonlinear optics. Thus, a study based on nonlinear analysis is possible and important. In nonlinear physics, a soliton is remarkable object not only for the fact that exact solutions can be obtained but also for its usefulness as a communications tool due to its robustness. In general, solitons are formed under the balance between nonlinearity and dispersion. For atomic condensates, the former is attributed to the interatomic interactions, while the latter comes from the kinetic energy. Either dark or bright solitons are allowable depending on the positive or negative sign of the interatomic coupling constants g, respectively, and indeed have been observed in a quasione-dimensional (q1D) optically constructed waveguide (Strecker et al.; 2002) (Khaykovich et al.; 2002). Such matter-wave solitons are expected in atom optics for applications in atom laser, atom interferometry, and coherent atom transport (Meystre; 2002). In this chapter, we extend the analysis of the matter-wave solitons to a multicomponent case by considering the so-called spinor condensate (Stenger et al.; 1998) whose spin degrees of freedom are liberated under optical traps. Based on theoretical and experimental results, we introduce a new integrable model which describes the dynamical properties of the matter-wave soliton of spinor condensates (Ieda et al.; 2004a). We employ the inverse scattering method to solve this model exactly. As a result, we predict the occurrence of undiscovered physical phenomena such as macroscopic spin precession and spin switching. The chapter is organized as follows. In Sec. 2, the mean field theory of condensate is briefly reviewed. Section 3 introduces an effective interatomic coupling in a q1D condensate. Using these results, we consider a spinor condensate in q1D regime in Sec. 4. Then, in Sec. 5, we