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Experiments with Entangled Photons : Bell Inequalities, Non-local Games and Bound Entanglement

Muhammad Sadiq

Published Jan 1, 2016• 2 citations
OpenAlex

Abstract

Quantum mechanics is undoubtedly a weird field of science, which violates many deep conceptual tenets of classical physics, requiring reconsideration of the concepts on which classical physics is based. For instance, it permits persistent correlations between classically separated systems, that are termed as entanglement. To circumvent these problems and explain entanglement, hidden variables theories--based on undiscovered parameters--have been devised. However, John S. Bell and others invented inequalities that can distinguish between the predictions of local hidden variable (LHV) theories and quantum mechanics. The CHSH-inequality (formulated by J. Clauser, M. Horne, A. Shimony and R. A. Holt), is one of the most famous among these inequalities. In the present work, we found that this inequality actually contains an even simpler logical structure, which can itself be described by an inequality and will be violated by quantum mechanics. We found 3 simpler inequalities and were able to violate them experimentally. Furthermore, the CHSH inequality can be used to devise games that can outperform classical strategies. We explore CHSH-games for biased and unbiased cases and present their experimental realizations. We also found a remarkable application of CHSH-games in real life, namely in the card game of duplicate Bridge. In this thesis, we have described this application along with its experimental realization. Moreover, non-local games with quantum inputs can be used to certify entanglement in a measurement device independent manner. We implemented this method and detected entanglement in a set of two-photon Werner states. Our results are in good agreement with theory. A peculiar form of entanglement that is not distillable through local operations and classical communication (LOCC) is known as bound entanglement (BE). In the present work, we produced and studied BE in four-partite Smolin states and present an experimental violation of a Bell inequality by such states. Moreover we produced a three-qubit BE state, which is also the first experimental realization of a tripartite BE state. We also present its activation, where we experimentally demonstrate super additivity of quantum information resources.

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Quantum mechanics is undoubtedly a weird field of science, which violates many deep conceptual tenets of classical physics, requiring reconsideration of the concepts on which classical physics is based. For instance, it permits persistent correlations between classically separated systems, that are termed as entanglement. To circumvent these problems and explain entanglement, hidden variables theories--based on undiscovered parameters--have been devised. However, John S. Bell and others invented inequalities that can distinguish between the predictions of local hidden variable (LHV) theories and quantum mechanics. The CHSH-inequality (formulated by J. Clauser, M. Horne, A. Shimony and R. A. Holt), is one of the most famous among these inequalities. In the present work, we found that this inequality actually contains an even simpler logical structure, which can itself be described by an inequality and will be violated by quantum mechanics. We found 3 simpler inequalities and were able to violate them experimentally. Furthermore, the CHSH inequality can be used to devise games that can outperform classical strategies. We explore CHSH-games for biased and unbiased cases and present their experimental realizations. We also found a remarkable application of CHSH-games in real life, namely in the card game of duplicate Bridge. In this thesis, we have described this application along with its experimental realization. Moreover, non-local games with quantum inputs can be used to certify entanglement in a measurement device independent manner. We implemented this method and detected entanglement in a set of two-photon Werner states. Our results are in good agreement with theory. A peculiar form of entanglement that is not distillable through local operations and classical communication (LOCC) is known as bound entanglement (BE). In the present work, we produced and studied BE in four-partite Smolin states and present an experimental violation of a Bell inequality by such states. Moreover we produced a three-qubit BE state, which is also the first experimental realization of a tripartite BE state. We also present its activation, where we experimentally demonstrate super additivity of quantum information resources.
This thesis is the synthesis of theoretical and experimental works performed in the area of quantum foundations, particularly on quantum correlations and experimental tests of multiplicative Bell inequalities. First we begin with a comprehensive theoretical work performed on the foundations of quantum mechanics, focusing on the puzzling concepts of quantum entanglement, and hidden variable theories. Specifically, we present a broad overview of different classes of hidden variable theories such as local, crypto-nonlocal, contextual and non-local theories, along with several Bell like inequalities for these theories, providing theoretical proofs based on quantum mechanics for the falsification of some of these theories. Second we present a body of experimental, and theoretical works performed on a new class of Bell inequalities, i.e., the multiplicative Bell inequalities. We experimentally report the observation of the Bell parameters close to the Tsirelson (quantum) limit, upto a large number of measurement devices (n)(n)(n), and compare the results with a particular deterministic strategy. We also obtain classical bounds for some nnn, and report the experimental violation of these classical limits. We theoretically derive new richer bounds on the CHSH inequality (named after John Clauser, Michael Horne, Abnor Shimony and Richard Holt) and the multiplicative Bell parameter for n=2n=2n=2, based on the principle of ``relativistic independence'', and experimentally observe the distribution of Bell parameters as predicted by these bounds.
Bell nonlocality is the experimentally testable incompatibility between quantum correlations and explanations based on local hidden variables. Its significance now extends beyond the foundations of quantum mechanics: a Bell-inequality violation can certify entanglement, randomness, measurement incompatibility, and cryptographic security without requiring a detailed model of the devices producing the observed data. This article develops the mathematical structure of Bell experiments and explains its role in device-independent quantum information. Conditional probability distributions are classified into local, quantum, and no-signalling sets; the Clauser-Horne-Shimony-Holt inequality is derived, and its classical, quantum, and algebraic limits are distinguished. Tsirelson’s bound is obtained from the CHSH operator, while Popescu-Rohrlich correlations demonstrate that no-signalling alone does not identify the quantum set. The relation between entanglement and nonlocality is examined through local entangled states, hidden nonlocality, and activation. Nonlocal games, semidefinite relaxations, self-testing, certified randomness, and device-independent quantum key distribution are treated as operational consequences of Bell violation. Particular attention is given to entropy accumulation, finite-data security, loophole-free experiments, and the limitations of device independence. Bell nonlocality emerges as both a foundational separation between classical and quantum causal models and a quantitative resource for cryptographic and informational tasks.
Entanglement, describing the inseparability of a quantum multiparty system, is one of the most intriguing features of quantum mechanics. Violation of Bell inequality, for ruling out the possibility of local hidden variable theories, is commonly used as a strong witness for quantum entanglement. In previous Bell test experiments with photonic entanglement based on two-photon coincidence measurement, the photon temporal wave packets are absorbed completely by the detectors. That is, the photon coherence time is much shorter than the detection time window. Here we demonstrate generation of frequency-bin entangled narrowband biphotons, and for the first time, test the Clauser-Horne-Shimony-Holt (CHSH) Bell inequality |S|<= 2 for their nonlocal temporal correlations with time-resolved detection. We obtain a maximum |S| value of 2.52+/-0.48 that violates the CHSH inequality. Our result will have applications in quantum information processing involving time-frequency entanglement.
Quantum nonlocality is presented often as the most remarkable and inexplicable phenomenon known to modern science. It has been known already for a long time that the probabilistic models used to prove Bell and Clauser-Horn-Shimony-Holt inequalities (BI-CHSH) for spin polarization correlation experiments (SPCE) are incompatible with the experimental protocols of SPCE. In particular these models use the same common probability space, joint probability distributions and/or conditional independence to describe coincidence experiments in incompatible experimental settings. Strangely enough these results are not known or simply neglected. This is why we will once again reanalyze Bell locality assumptions and show that they have nothing to do with the notion of Einsteinian locality therefore their violation should not be called quantum nonlocality but rather quantum non-Kolmogorovness or quantum contextuality. Moreover if local variables describing the measuring instruments are correctly taken into account then BI-CHSH can no longer be proven and one can easily construct non-signaling probabilistic models able to reproduce the predictions of QT. The violation of BI-CHSH is considered usually as a proof that a quantum state is entangled. Since BI-CHSH are violated also in some experiments from outside the domain of quantum physics therefore the entanglement is not exclusively a quantum phenomenon. In order to further demystify these notions we show that one can prepare two macroscopic systems in such a way that simple realizable local experiments on these systems violate BI. In view of these arguments the further testing of BI-CHSH inequalities in search for the loopholes does not seem to be necessary.
The rapidly developing interdisciplinary field of quantum information, which merges quantum and information science, studies non-classical aspects of quantum systems. These studies are motivated by the promise that the non-classicality can be used to solve tasks more efficiently than classical methods would allow. In many quantum informational studies, non-classical behaviour is attributed to the notion of entanglement. In this thesis we use photons to experimentally investigate fundamental questions such as: What happens to the entanglement in a system when it is affected by noise? In our study of noisy entanglement we pursue the challenging task of creating bound entanglement. Bound entangled states are created through an irreversible process that requires entanglement. Once in the bound regime, entanglement cannot be distilled out through local operations assisted by classical communication. We show that it is possible to experimentally produce four-photon bound entangled states and that a violation of a Bell inequality can be achieved. Moreover, we demonstrate an entanglement-unlocking protocol by relaxing the condition of local operations. We also explore the non-classical nature of quantum mechanics in several single-photon experiments. In these experiments, we show the violation of various inequalities that were derived under the assumption of non-contextuality. Using qutrits we construct and demonstrate the simplest possible test that offers a discrepancy between classical and quantum theory. Furthermore, we perform an experiment in the spirit of the Kochen-Specker theorem to illustrate the state-independence of this theorem. Here, we investigate whether or not measurement outcomes exhibit fully contextual correlations. That is, no part of the correlations can be attributed to the non-contextual theory. Our results show that only a small part of the experimental generated correlations are amenable to a non-contextual interpretation.
Quantum mechanics is nonlocal, meaning it cannot be described by any classical local hidden variable model. In this thesis we study two aspects of quantum nonlocality. Part I addresses the question of what classical resources are required to simulate nonlocal quantum correlations. We start by constructing new local models for noisy entangled quantum states. These constructions exploit the connection between nonlocality and Grothendieck's inequality, first noticed by Tsirelson. Next, we consider local models augmented by a limited amount of classical communication. After generalizing Bell inequalities to this setting, we show that (i) one bit of communication is sufficient to simulate the correlations of projective measurements on a maximally entangled state of two qubits, and (ii) five bits of communication are sufficient to simulate the joint correlation of two-outcome measurements on any bipartite quantum state. The latter result can be interpreted as a stronger (constrained) version of Grothendieck's inequality. In part II, we investigate the monogamy of nonlocal correlations. In a setting where three parties, A, B, and C, share an entangled quantum state of arbitrary dimension, we: (i) bound the trade-off between AB's and AC's violation of the CHSH inequality, obtaining an intriguing generalization of Tsirelson's bound, and (ii) demonstrate that forcing B and C to be classically correlated prevents A and B from violating certain Bell inequalities. We study not only correlations that arise within quantum theory, but also arbitrary correlations that do not allow signaling between separate groups of parties. These results are based on new techniques for obtaining Tsirelson bounds, or bounds on the quantum value of a Bell inequality, and have applications to interactive proof systems and cryptography.