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ACTA PHOTONICA SINICA

Coherent Population Trapping of a Three-level Atom Interacting with Few Cycle Pulse Train

蔡勋明 CAI Xun-minga, 范梦慧 FAN Meng-huib

Published Jan 1, 2013• 0 citations
Publisher

Abstract

The poulation transfer and coherent population trapping of a three-level atom interacting with few cycle pulse train are studied.The density matrix equation in interation picture is numerical solved without rotating wave approximation.The research indicates that if a three-level atom interacts with a few cycle pulse train,the population transfer of level and the coherence of ground state will be gradual accumulated.When the repetition frequency of pulses is integer points of the ground-state splitting,the three atom interacts with pulse train can be seen as the atom interacts with two tenoning frequency of the frequency comb.So the system will be in the dark state and reach coherent population trapping.If the parameters of few-cycle pulse are appropriately selected,the coherence of three-level system will evolute into stable value in 0.5 nanosecond.The coherent population trapping in the three-level is generated.Comparing with the pulse that the pulse width is 100 femtoseconds,the build-up time of coherent population trapping by few cycle pulse train is shortened two orders of magnitude.When the ground-state splitting is wided enough and the carrier frequency of pulse is ω=(ω1+ω2)/2,where,are the atomic transition frequency,the doppler frequency shift that is aroused by the movement of atom won't destroy the coherent population trapping of atom.The reason is that all tenoning frequencies of the frequency comb have the same frequency shift,so the condition of coherent population trapping is still meeted.

DOI
10.3788/gzxb20134202.0209

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The poulation transfer and coherent population trapping of a three-level atom interacting with few cycle pulse train are studied.The density matrix equation in interation picture is numerical solved without rotating wave approximation.The research indicates that if a three-level atom interacts with a few cycle pulse train,the population transfer of level and the coherence of ground state will be gradual accumulated.When the repetition frequency of pulses is integer points of the ground-state splitting,the three atom interacts with pulse train can be seen as the atom interacts with two tenoning frequency of the frequency comb.So the system will be in the dark state and reach coherent population trapping.If the parameters of few-cycle pulse are appropriately selected,the coherence of three-level system will evolute into stable value in 0.5 nanosecond.The coherent population trapping in the three-level is generated.Comparing with the pulse that the pulse width is 100 femtoseconds,the build-up time of coherent population trapping by few cycle pulse train is shortened two orders of magnitude.When the ground-state splitting is wided enough and the carrier frequency of pulse is ω=(ω1+ω2)/2,where,are the atomic transition frequency,the doppler frequency shift that is aroused by the movement of atom won't destroy the coherent population trapping of atom.The reason is that all tenoning frequencies of the frequency comb have the same frequency shift,so the condition of coherent population trapping is still meeted.
In this paper, we investigate numerically the modeled density matrix equations for the interaction of a three-level atomic system in V-configuration with a train of chirped optical n-pulses (up to n = 10) within and without the rotating wave approximation. For adopted data of Rb 87, maximal population transfer to either of the upper levels is achieved with n > 1 pulse via variation of chirp parameter/frequency mismatch of the closely lying upper levels. Optimal steady population transfer and maximum atomic coherence of the upper levels are predicted for non-zero chirp parameter and train of n = 1 - 10, 30 pulses.
The interactions of sub-cycle and single-cycle pulses with two- or three-level quantum systems are studied, respectively. For the two-level quantum system, two cases in which the carrier frequency of pulses is in resonance and far from resonance with the atom are analysed. The ultrafast complete population transfer can be obtained. The sub-cycle pulse with a far off-resonant carrier frequency is found to be more suitable for the population transfer. The relation between the area of pulses and population transfer is clarified in the sub-cycle and single-cycle domain. For the Lambda-type three-level quantum system, more than 90% of population transfer can be achieved from one level to another. The scheme is insensitive to the variation of the laser parameters such as the peak Rabi frequency and the carrier frequency for both two- and three-level quantum systems.
The excitation of room-temperature four-level 87Rb^{87}\mathrm{Rb}87Rb atoms by a train of ultrashort pulses is investigated theoretically in the conditions when the pulse repetition period is shorter than the characteristic atomic relaxation times. It is shown that coherent accumulation of excitation leads to coherent population trapping and electromagnetically induced transparency of the excitation pulses when the pulse repetition rate is a subharmonic of the ground-state hyperfine splitting. It is illustrated how the judicious choice for the frequency comb parameters can provide a means to effectively control the degree of coherence between the ground-state hyperfine levels for selective atomic groups, and even transfer the whole atomic distribution to the dark state with up to 9595%95 efficiency.
We report a study on the ultrafast coherent population oscillations (UCPOs) in two-level atoms induced by a frequency-modulated few-cycle optical pulse train. The phenomenon of UCPOs is investigated by numerically solving the optical Bloch equations beyond the rotating wave approximation. We demonstrate that the quantum state of the atoms and the frequency of the UCPOs may be controlled by controlling the number of pulses in the pulse trains and the pulse repetition time, respectively. Moreover, the robustness of the population inversion against the variation of the laser pulse parameters is also investigated. The proposed scheme may be useful for the creation of atoms in selected quantum states for desired time duration and may have potential applications in ultrafast optical switching. The scheme may also be used to measure pulse repetition rate.
We consider the case of interaction of a three-level atom with a high intensity pulse electromagnetic field. Rabi frequencies are assumed to be of the order of the transition frequency or greater. We demonstrate that coherent population trapping exists even in such a case when the usual rotating-wave approximation is no longer valid. However, a certain condition on the phases of electromagnetic wave components has to be satisfied in order to make coherent population trapping possible. This condition is specific for the strong field case in contrast to the case where the rotating-wave approximation is valid. Also we point out some elements for which a model of an atom with a finite number of levels may still be valid while the rotating-wave approximation breaks down.
We present an experimental and theoretical study of the carrier-envelope phase effects on population transfer between two bound atomic states interacting with intense ultrashort pulses. Radio frequency pulses are used to transfer population among the ground state hyperfine levels in rubidium atoms. These pulses are only a few cycles in duration and have Rabi frequencies of the order of the carrier frequency. The phase difference between the carrier and the envelope of the pulses has a significant effect on the excitation of atomic coherence and population transfer. We provide a theoretical description of this phenomenon using density matrix equations. We discuss the implications and possible applications of our results.