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On optical self-phase modulation via collective atomic excitations in a Bose-Einstein condensate

Khulud Almutairi

Published Jan 1, 2014• 0 citations
Publisher

Abstract

This thesis presents a method for generating nonlinear phase shifts on superpositions of photon number states. Light is stored in a Bose-Einstein condensate (BEC) via electromagnetically induced transparency (EIT) memory techniques. Atomic collisions are exploited to generate a nonlinear phase shift of the stored state. The stored light is then revived with the nonlinear phase shift imprinted upon it. We show that this method can be used to develop a nonlinear-sign gate in the regime where the Thomas-Fermi and mean-field approximations are valid. We test these approximations using realistic parameters to find that these approximations pass the standard tests for validity in a single-component condensate. However, for the two-component condensates considered here, we find that these conditions are not sufficiently strict. Therefore, we find a stronger set of conditions and show for the same set of parameters that the approximations are invalid.

DOI
10.11575/prism/27183

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This thesis presents a method for generating nonlinear phase shifts on superpositions of photon number states. Light is stored in a Bose-Einstein condensate (BEC) via electromagnetically induced transparency (EIT) memory techniques. Atomic collisions are exploited to generate a nonlinear phase shift of the stored state. The stored light is then revived with the nonlinear phase shift imprinted upon it. We show that this method can be used to develop a nonlinear-sign gate in the regime where the Thomas-Fermi and mean-field approximations are valid. We test these approximations using realistic parameters to find that these approximations pass the standard tests for validity in a single-component condensate. However, for the two-component condensates considered here, we find that these conditions are not sufficiently strict. Therefore, we find a stronger set of conditions and show for the same set of parameters that the approximations are invalid.
We investigate a method for generating nonlinear phase shifts on superpositions of photon number states. The light is stored in a Bose-Einstein condensate via electromagnetically induced transparency memory techniques. The atomic collisions are exploited to generate a nonlinear phase shift of the stored state. The stored light is then revived with the nonlinear phase shift imprinted upon it. We show that this method can be used as a nonlinear-sign gate in the regime where the Thomas-Fermi and mean-field approximations are valid. We test these approximations using realistic parameters and find that these approximations pass the standard tests for validity in a single-component condensate. However, for the two-component condensates considered here, we find that these conditions are insufficiently strict. We find a stronger set of conditions and show for the same set of parameters that the approximations are invalid.
We propose and analyze a scheme to generate squeezed light by storing a classical probe pulse in a Bose--Einstein condensate (BEC) and exploiting the nonlinear evolution caused by atom--atom collisions during the storage time. A ΛΛΛ-type optical memory interface maps a chosen temporal probe mode onto a single phase-matched collective spin wave; for a coherent input this prepares a tunable coherent spin state of a two-component BEC, with its initial spin orientation set by the stored mean excitation number and the phase relation between the probe and control fields. Collisional interactions during storage then implement one-axis-twisting dynamics and generate spin squeezing in the atomic ensemble. We account for realistic loss and finite memory and retrieval efficiencies, and model readout as a single-mode beam-splitter mapping that transfers the atomic quadrature squeezing onto a propagating optical mode. We identify optimal storage times and predict that, under realistic conditions, several dB of squeezing can be transferred to the retrieved light.
Large nonlinearity at the single-photon level can pave the way for the implementation of universal quantum gates. However, realizing large and noiseless nonlinearity at such low light levels has been a great challenge for scientists in the past decade. Here, we propose a scheme that enables substantial nonlinear interaction between two light fields that are both stored in an atomic memory. Semiclassical and quantum simulations demonstrate the feasibility of achieving large cross-phase modulation (XPM) down to the single-photon level. The proposed scheme can be used to implement parity gates from which CNOT gates can be constructed. Furthermore, we present a proof of principle experimental demonstration of XPM between two optical pulses: one stored and one freely propagating through the memory medium. Researchers have developed a new technique that shows promise for constructing optical quantum logic gates. Theoretical simulations performed by Mahdi Hosseini and co-workers from the Australian National University and Macquarie University in Australia show that inducing cross-phase modulation between two single-photon light fields stored in a rubidium atomic memory should provide large phase shifts and thus allow the realization of parity gates and CNOT gates, both of which are needed for quantum computing. The researchers estimate that using cold atoms confined in a dipole trap and short-duration single-photon wavepackets should make it possible to realize phase shifts of the order of 10 mrad — orders of magnitude larger than schemes that employ electromagnetically induced transparency.
We theoretically explore coherent information transfer between ultraslow light pulses and Bose-Einstein condensates (BEC's) and find that storing light pulses in BEC's allows the coherent condensate dynamics to process optical information. We consider BEC's of alkali atoms with a $\ensuremath{\Lambda}$ energy level configuration. In this configuration, one laser (the coupling field) can cause a pulse of a second pulsed laser (the probe field) to propagate with little attenuation (electromagnetically induced transparency) at a very slow group velocity $(\ensuremath{\sim}10\phantom{\rule{0.3em}{0ex}}\mathrm{m}∕\mathrm{s})$ and be spatially compressed to lengths smaller than the BEC. These pulses can be fully stopped and later revived by switching the coupling field off and on. Here we develop a formalism, applicable in both the weak- and strong-probe regimes, to analyze such experiments and establish several results: (1) We show that the switching can be performed on time scales much faster than the adiabatic time scale for electromagnetically induced transparancy even in the strong-probe regime. We also study the behavior of the system changes when this time scale is faster than the excited state lifetime. (2) Stopped light pulses write their phase and amplitude information onto spatially dependent atomic wave functions, resulting in coherent two-component BEC dynamics during long storage times. We investigate examples relevant to 87Rb^{87}\mathrm{Rb}87Rb experimental parameters and see a variety of novel dynamics occur, including interference fringes, gentle breathing excitations, and two-component solitons, depending on the relative scattering lengths of the atomic states used and the probe to coupling intensity ratio. We find that the dynamics when the levels $\ensuremath{\mid}F=1,{M}_{F}=\ensuremath{-}1⟩$ and $\ensuremath{\mid}F=2,{M}_{F}=+1⟩$ are used could be well suited to designing controlled processing of the information input on the probe. (3) Switching the coupling field on after the dynamics writes the evolved BEC wave functions density and phase features onto a revived probe pulse, which then propagates out. We establish equations linking the BEC wave function to the resulting output probe pulses in both the strong- and weak-probe regimes. We then identify sources of deviations from these equations due to absorption and distortion of the pulses. These deviations result in imperfect fidelity of the information transfer from the atoms to the light fields and we calculate this fidelity for Gaussian-shaped features in the BEC wave functions. In the weak-probe case, we find that the fidelity is affected both by absorption of very-small-length-scale features and absorption of features occupying regions near the condensate edge. We discuss how to optimize the fidelity using these considerations. In the strong-probe case, we find that when the oscillator strengths for the two transitions are equal the fidelity is not strongly sensitive to the probe strength, while when they are unequal the fidelity is worse for stronger probes. Applications to distant communication between BEC's, squeezed light generation, and quantum information are anticipated.
Photons are good candidates for carrying quantum information because they are very stable particles: they interact weakly with the medium and barely with each other. However, this has drawbacks when you want to process the information because, in this case, it is preferable to have photon-photon interactions. For example, for applications in quantum repeaters, such interactions would allow deterministic Bell state measurements, increasing the entanglement distribution rate between two remote nodes. Getting two photons to interact with each other efficiently requires mapping them into a nonlinear medium at the single-photon level, that is, a medium that reacts differently when it interacts with a single photon than when it does with two. Such strong nonlinearity has been demonstrated with Rydberg atoms, which are atoms excited to a state with a high principal quantum number. In this thesis we have performed nonlinear quantum optics experiments using an ensemble of cold Rydberg atoms, where we have studied the properties of the quantum light emitted by these atoms. First, we demonstrated nonlinearities at the single-photon level. To reach this stage, we made several improvements to the previous experimental setup available in the group, of which the implementation of a dipole trap was especially relevant. We evidence quantum nonlinearity by measuring photon antibunching for the transmitted light after interacting with the Rydberg state under electromagnetically induced transparency (EIT). We also showed the generation of single photons on-demand after storing weak coherent states of light pulses as collective Rydberg excitations. Then, we studied the variation of the light statistic throughout the output pulse after propagating through the medium as Rydberg polaritons, which are superposition states of light and Rydberg excitations. We showed that the properties at the beginning and the end of the pulse were different from those of the steady state. In particular, the light detected after the input pulse was abruptly turned off gave much stronger suppression of two-photon events. Then, we investigated how to exploit this effect to generate single photons on demand. To do this, we analyzed the quality of the single photons detected at the end of the pulse as a function of the detection probability and compared the results with those obtained by storing the input pulse as collective Rydberg excitations. We showed that the photons were generated more efficiently when increasing the detection window at the cost of deteriorating the single photons statistics. Finally, we investigated the indistinguishability of the photons emitted by our Rydberg atomic ensemble, a crucial property for using Rydberg atoms as nodes in quantum networks. We also compared the single photons generated after storage under EIT conditions with those obtained using a two-photon Raman excitation to the Rydberg state. We measured the indistinguishability by making them interfere with weak coherent states of light in a Hong-Ou-Mandel experiment. And we showed that, although we obtained better photon statistics under EIT conditions, the indistinguishability from those obtained with Raman excitation was significantly higher.