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Journal of Experimental and Theoretical Physics

Multiphoton dynamics of qutrits in the ultrastrong coupling regime with a quantized photonic field

H. K. Avetissian, A. K. Avetissian, G. F. Mkrtchian, Oleg V. Kibis

Published Dec 1, 2015• 1 citation
Publisher

Abstract

Multiphoton resonant excitation of a three-state quantum system (a qutrit) with a single-mode photonic field is considered in the ultrastrong coupling regime, when the qutrit–photonic field coupling rate is comparable to appreciable fractions of the photon frequency. For ultrastrong couplings, the obtained solutions of the Schrödinger equation that reveal multiphoton Rabi oscillations in qutrits with the interference effects leading to the collapse and revival of atomic excitation probabilities at the direct multiphoton resonant transitions.

DOI
10.1134/s1063776115120018

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Multiphoton resonant excitation of a three-state quantum system (a qutrit) with a single-mode photonic field is considered in the ultrastrong coupling regime, when the qutrit–photonic field coupling rate is comparable to appreciable fractions of the photon frequency. For ultrastrong couplings, the obtained solutions of the Schrödinger equation that reveal multiphoton Rabi oscillations in qutrits with the interference effects leading to the collapse and revival of atomic excitation probabilities at the direct multiphoton resonant transitions.
We consider the multiphoton dynamics of a quantum system composed of a three-state atom (a qutrit) and a single-mode photonic field in the ultrastrong and deep strong coupling regimes, when the coupling strength is comparable to or larger than the oscillator energy scale. We assume a qutrit to be in a L configuration, where an upper level is coupled to a twofold degenerate lower level. Direct multiphoton resonant transitions revealing generalized Rabi oscillations, collapse, and revivals in atomic excitation probabilities for the ultrastrong couplings are studied. In the deep strong coupling regime, particular emphasis is placed on the ground state of the considered system which strictly exhibits nonclassical properties.
When an atom is strongly coupled to a cavity, the two systems can exchange a single photon through a coherent Rabi oscillation. This process enables precise quantum-state engineering and manipulation of atoms and photons in a cavity, which play a central role in quantum information and measurement. Recently, a new regime of cavity QED was reached experimentally where the strength of the interaction between light and artificial atoms (qubits) becomes comparable to the atomic transition frequency or the resonance frequency of the cavity mode. Here we show that this regime can strongly modify the concept of vacuum Rabi oscillations, enabling multiphoton exchanges between the qubit and the resonator. We find that experimental state-of-the-art circuit-QED systems can undergo two- and three-photon vacuum Rabi oscillations. These anomalous Rabi oscillations can be exploited for the realization of efficient Fock-state sources of light and complex entangled states of qubits.
We compare the semiclassical and quantum predictions for the unitary dynamics of a two-level atom interacting with a single-mode electromagnetic field under parametric modulation of the atomic parameters in the regime of multiphoton atom–field resonances. We derive approximate analytic solutions for the semiclassical Rabi model when the atomic transition frequency and the atom–field coupling strength undergo harmonic external modulations. These solutions are compared to the predictions of the quantum Rabi model, which we solve numerically for an initial coherent state with a large average photon number (on the order of 104), in the regime of three-photon resonance. We show that, for short enough times and sufficiently intense coherent states, the semiclassical dynamics agrees quite well with the quantum dynamics, although it inevitably fails at longer times due to the absence of collapse–revival behavior. Furthermore, we describe how the field state evolves throughout the interaction, presenting numerical results for the average photon number, entropies (related to atom–field entanglement), and other quantities characterizing the photon number statistics of the electromagnetic field.
Damping of multiphoton Rabi oscillations due to a finite lifetime of photons is investigated using an algebraic method of the solution of the master equation. The time dependence of the probability of electron transitions between atomic levels is evaluated. In a regime of weak atom–photon coupling (a coupling constant smaller than the photon decay rate), the spontaneous emission of many photons from a single electron transition due to the interaction with a resonant light is found. Thus, a multiphoton counterpart of the Purcell effect is predicted.
Within the Rabi quantum model, it has been shown theoretically that a two-level atom ultrastrongly coupled to an electromagnetic field generates or absorbs photons. Photons can be generated if the field is initially in the vacuum state. Under certain initial states of the atom + field system, the absorption of photons is possible in the field mode in the ultrastrong atom–field coupling regime. If the atom is initially in the ground (unexcited) state and the field is in the vacuum state, photons can be generated under resonance condition ωa ≈ ωf or ξ ≡ ωa/ωf ≈ 1, where ωa and ωf are the atomic transition and field frequencies, respectively, in the ultrastrong coupling regime. At the negative detuning when ξ ≪ \ll ≪ 1 or ωa ≪ \ll ≪ ωf, Rabi oscillations of the average number of photons ⟨n^⟩t{{\langle \hat {n}\rangle }_{t}}⟨n^⟩t​ with 0⩽⟨n^⟩t⩽nmax⁡≫10 \leqslant {{\langle \hat {n}\rangle }_{t}} \leqslant {{n}_{{\max }}} \gg 10⩽⟨n^⟩t​⩽nmax​≫1 are observed in the case of the ultrastrong coupling with the atom–field coupling constant g~≡|g|/ωf∼1\tilde {g} \equiv {\text{|}}g{\text{|/}}{{\omega }_{{\text{f}}}} \sim 1g~​≡|g|/ωf​∼1 ; in this case, the population of the excited atomic state is Pe(t) ≈ 0.5. At a large positive detuning when ξ ≫ \gg ≫ 1, photons are not generated, i.e., ⟨n^⟩≈0\langle \hat {n}\rangle \approx 0⟨n^⟩≈0 , and the atom remains in the initial state, i.e., Pe(t) ≈ 0. The statistics of photons in the generation regime is nearly chaotic: the variance of photons is much larger than the level of the coherent field state (i.e., is super-Poisson). Field photons are absorbed without the excitation of the atom in the ultrastrong coupling regime in the case of the coherent initial state of the field (⟨n^(t=0⟩>0)(\langle \hat {n}(t = 0\rangle > 0)(⟨n^(t=0⟩>0) for certain positive detuning values. In this case, the field becomes sub-Poisson.