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Optics Express

Ultrashort coherence times in partially polarized stationary optical beams measured by two-photon absorption

Andriy Shevchenko, M. Roussey, Ari T. Friberg, Tero Setälä

Published Nov 20, 2015• 18 citations
Publisher

Abstract

We measure the recently introduced electromagnetic temporal degree of coherence of a stationary, partially polarized, classical optical beam. Instead of recording the visibility of intensity fringes, the spectrum, or the polarization characteristics, we introduce a novel technique based on two-photon absorption. Using a Michelson interferometer equipped with polarizers and a specific GaAs photocount tube, we obtain the two fundamental quantities pertaining to the fluctuations of light: the degree of coherence and the degree of polarization. We also show that the electromagnetic intensity-correlation measurements with two-photon absorption require that the polarization dynamics, i.e., the time evolution of the instantaneous polarization state, is properly taken into account. We apply the technique to unpolarized and polarized sources of amplified spontaneous emission (Gaussian statistics) and to a superposition of two independent, narrow-band laser beams of different mid frequencies (non-Gaussian statistics). For these two sources femtosecond-range coherence times are found that are in good agreement with the traditional spectral measurements. Although previously employed for laser pulses, two-photon absorption provides a new physical principle to study electromagnetic coherence phenomena in classical and quantum continuous-wave light at extremely short time scales.

DOI
10.1364/oe.23.031274

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We study the probabilities for two-photon absorption processes induced by both coherent and thermal light when acting on an atomic system. Calculations are performed with quantum electrodynamics, and we find results similar to those obtained with semiclassical methods; that is, the two-photon absorption probability depends on the statistical properties of the light used. This probability assumes its maximum value for coherent light.

Physical Review•May 25, 1967•34 citations
We measure the recently introduced electromagnetic temporal degree of coherence of a stationary, partially polarized, classical optical beam. Instead of recording the visibility of intensity fringes, the spectrum, or the polarization characteristics, we introduce a novel technique based on two-photon absorption. Using a Michelson interferometer equipped with polarizers and a specific GaAs photocount tube, we obtain the two fundamental quantities pertaining to the fluctuations of light: the degree of coherence and the degree of polarization. We also show that the electromagnetic intensity-correlation measurements with two-photon absorption require that the polarization dynamics, i.e., the time evolution of the instantaneous polarization state, is properly taken into account. We apply the technique to unpolarized and polarized sources of amplified spontaneous emission (Gaussian statistics) and to a superposition of two independent, narrow-band laser beams of different mid frequencies (non-Gaussian statistics). For these two sources femtosecond-range coherence times are found that are in good agreement with the traditional spectral measurements. Although previously employed for laser pulses, two-photon absorption provides a new physical principle to study electromagnetic coherence phenomena in classical and quantum continuous-wave light at extremely short time scales.
Recently some novel two-photon interference experiments have been performed, where quantities such as the field coherence time and the beat spacing between light beams with different frequencies were measured with high time resolution1. These experiments have overcome the traditional limits on time resolution by combining a Mach-Zehnder interferometer configuration with the two-photon correlation technique. All of these experiments, however, have been performed with cw light sources, and no attempt has yet been made to measure the temporal variation of the field intensity.
Statistical properties of partially polarized Gaussian light were studied experimentally for degrees of polarization PPP from 0.03 to 1 by a standard technique of photon counting. The Gaussian light with an arbitrary degree of polarization was obtained from Rayleigh scattering of orthogonally polarized laser beams. The factorial moments up to sixth order of the photoelectron distribution were measured with an arbitrary temporal and spatial coherence. After corrections were taken for the experimental conditions, the theoretical values of these factorial moments were compared with the experimental results. It is shown that the theoretical predictions were quantitatively well verified by the present measurements. The microscopic process is discussed from the standpoint of the light scattering system used in the present measurements, and it is shown that the orthogonally polarized components of the scattered light observed are statistically independent.
In this work, interference of independent polychromatic waves with different center frequencies and polarizations is studied experimentally using intensity interferometry and two-photon detection. The intensity and polarization beatings of such interfering waves depend on the wave spectra and fluctuation statistics. The authors introduce an experimental technique to characterize the beating harmonicity time and the randomness of the polarization beating for light beams obeying Gaussian and/or Poissonian statistics.
We study the photon correlation properties of broadband parametric down-converted light. The measurement of the photon correlation is carried out thanks to a modified Hanbury Brown-Twiss interferometer based on two photon absorption in GaAs detector. Since this method is not affected by the phase matching conditions of the detecting apparatus (so called "final state post-selection"), the detection bandwidth can be extremely large. This is illustrated by studying, with the same apparatus, the degree of second order coherence of parametric light in both degenerate and non-degenerate cases. We show that our experiment is able to determine the coherent as well as the incoherent contributions to the degree of second order coherence of parametric light with a time resolution in the fs range scale.
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Non-Critical Rayleigh Scattering from Pure Liquids.- T5 Coherence Effects in Spontaneous Emission II.- T5-1 Cooperative Effects in Spontaneous Emission.- T5-2 Amplified Spontaneous Emission.- T5-3 Non-Gaussian Statistics of Superradiant Radiation from Saturated Xenon 3.5?m Laser Amplifier.- T5-4 On the Theory of Radiating Electrons.- T6 Coherent Light Interactions.- T6-1 Atomic and Molecular Spectroscopy by Saturation with Coherent Light.- T6-2 Response Functions for Strongly Driven Systems.- T6-3 Mechanism of Interaction of Picosecond Light Pulses with Matter Yielding Self-Trapping.- T6-4 Resonance Fluorescence Lineshapes with Intense Applied Fields.- T6-5 Electron Beams as Carriers of Optical Coherence.- T7 Lasers.- T7-1 Detuned Single Mode Laser and Detailed Balance.- T7-2 Tunable Raman Lasers.- T7-3 Dye Lasers: Recent Advances in Tunable Systems.- F1 Quantum Electrodynamics and Alternative Theories III.- F1-1 A Theory of Light without Photons: Implications from Fermis to Light Years.- F1-2 Blackbody Heat Capacity and Action-at-a-Distance Electrodynamics.- F1-3 The Implications of Radiative Equilibrium in Jaynes' Extension of Semiclassical Radiation Theory.- F1-4 A Quantum Electrodynamic Investigation of the Jaynes-Crisp-Stroud Approach to Spontaneous Emission.- F1-5 Critical Comments on Radiation Theory.- F2 Resonant Pulse Propagation II.- F2-1 Cooperative Phenomena in Resonant Propagation.- F2-2 Theory of Sub-Cooperation-Limit Optical Pulses in Resonant Absorbers.- F2-3 Multiple Pulse Chirping in Self-Induced Transparency.- F2-4 Coupled Superradiance Master Equations: Application to Fluctuations in Coherent Pulse Propagation in Resonant Media.- F3 Coherence II.- F3-1 The Laser-Phase Transition Analogy - Recent Developments.- F3-2 Multiple-Time-Scale Analysis of Coherent Radiation.- F3-3 Orthogonal Operators and Phase Space Distributions in Quantum Optics.- F4 Coherence Effects in Spontaneous Emission III.- F4-1 Radiation by Many Excited Atoms between Mirrors.- F4-2 Transient Coherent Emission.- F4-3 Superradiance from a System of 3-Level Particles.- F4-4 A Quantum Electrodynamic View of Superradiance as a Competition between Stimulated and Spontaneous Atomic Decay.- F5 Post Deadline Session.- F5-1 Third- and Higher-Order Intensity Correlations in Laser Light.- F5-2 Correlation Function of a Laser Beam near Threshold.- F5-3 Localization of Photons.- F5-4 Adiabatic Following and the Self-Defocusing of Light in Rubidium Vapor.- F5-5 Experimental Evidence of an X-Ray Laser.- F5-6 Quantum Theory of Photodetection and Coherence Properties of Electrons.- F5-7 Statistics of Light Scattered by Non-Gaussian Fluctuations.- F6 Quantum Noise.- F6-1 Unified Thermodynamics of Dissipative Structures and Coherence in Nonlinear Optics.- F6-2 The Approach to Thermal Equilibrium in Systems of Coupled Quantum Oscillators Initially in a Generalized Gaussian State.- F6-3 Comparison between Incoherent and Chaotic Sources: Contribution to the Study of the Origin of Bunching Effect.- F6-4 Self-Pulsing in Laser Amplification of Broadband Noise.- Author Index.