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Chinese Physics B

Spontaneous emission of two quantum dots in a single-mode cavity

Liu Qiu, Ke Zhang, Zhiyuan Li

Published Sep 1, 2013• 4 citations
Publisher

Abstract

The spontaneous emission spectrum from two quantum dots (QDs) that are strongly coupled with a single-mode nanocavity is investigated using rigorous numerical calculations and simple analytical solutions of quantum dynamics. The emission spectra both from the side and along the axis of the cavity are considered. Modification of two parameters, the coupling strength and the detuning between the transition frequencies of the two quantum dots, allows us to efficiently control the shape of the spontaneous emission spectrum. Different profiles and their physical origins can be well understood in the dressed-state picture for the light—QD interaction in the on-resonance and off-resonance situations. In the on-resonance situation, the emission spectra exhibit symmetric features, and they are not altered by the asymmetry in the coupling parameters. The axis spectra show two emission peaks while the side spectra have three emission peaks. In the off-resonance situation, the emission spectra always show an asymmetrical three-peak feature. When the two QDs have different decay parameters, singular features (a peak or a dip) can take place at the frequency of the cavity mode, and this is attributed to the unbalanced process of the emission and absorption of a single photon.

DOI
10.1088/1674-1056/22/9/094207

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The spontaneous emission spectrum from two quantum dots (QDs) that are strongly coupled with a single-mode nanocavity is investigated using rigorous numerical calculations and simple analytical solutions of quantum dynamics. The emission spectra both from the side and along the axis of the cavity are considered. Modification of two parameters, the coupling strength and the detuning between the transition frequencies of the two quantum dots, allows us to efficiently control the shape of the spontaneous emission spectrum. Different profiles and their physical origins can be well understood in the dressed-state picture for the light—QD interaction in the on-resonance and off-resonance situations. In the on-resonance situation, the emission spectra exhibit symmetric features, and they are not altered by the asymmetry in the coupling parameters. The axis spectra show two emission peaks while the side spectra have three emission peaks. In the off-resonance situation, the emission spectra always show an asymmetrical three-peak feature. When the two QDs have different decay parameters, singular features (a peak or a dip) can take place at the frequency of the cavity mode, and this is attributed to the unbalanced process of the emission and absorption of a single photon.
In this work, we theoretically analyze the few-photon emissions generated in a coupled double quantum dots (CDQDs)-single mode microcavity system, under continuous wave and pulse excitation. Compared with the uncoupled case, strong sub-Poissonian character is achieved in a CDQDs–cavity system at a certain laser frequency. Based on the proposed scheme, single photon generation can be obtained separately under QD–cavity resonant condition and off-resonant condition. For different cavity decay rates, we reveal that laser frequency detunings of minimum second-order autocorrelation function are discrete and can be divided into three regions. Moreover, the non-ideal situation where two QDs are not identical is discussed, indicating the robustness of the proposed scheme, which possesses sub-Poissonian character in a large QD difference variation range.
In 1946, E. M. Purcell predicted that the radiative lifetime of an emitter is not an intrinsic property but can be modified by structuring the surrounding electromagnetic field [36]. By inserting a semiconductor quantum dot (QD) in an optical cavity, one can accelerate or inhibit its spontaneous emission. In the present article, we show that the QD spontaneous emission can be deterministically controlled to fabricate bright sources of quantum light. QDs in cavities: basics, motivation, first demonstrations Light-matter coupling We note f the ground state of the QD and e its excited state. For a cavity mode close to resonance with the QD optical transition, we consider only the states with 0 or 1 photon in the cavity mode. The states ∣ e, 0〉 and ∣ f, 1〉 are coupled through light–matter interaction, with a constant g , where h g = ∣〈 e, 0∣ Ed ∣ f, 1∣, with d the dipole of the optical transition e → f and E the electric field at the QD position. Each of the states ∣ e, 0 > and ∣ f, 1 > are also coupled to continua of states: continuum of the free-space optical mode, phonons of the semiconductor matrix, etc. [4]. Here, we consider only the coupling to the continuum of the free-space optical mode, related to the cavity losses, with a constant γ c . When g << γ c , the photon emitted by the recombination of an exciton efficiently escapes outside the cavity. The QD optical transition radiative recombination rate can be accelerated (Purcell effect) or inhibited.
We present a study of the strong coupling between radiation and matter, considering a system of two quantum dots, which are in mutual interaction and interact with a single mode of light confined in a semiconductor nanocavity. We take into account dissipative mechanisms such as the escape of the cavity photons, decay of the quantum dot excitons by spontaneous emission, and independent exciton pumping. It is shown that the mutual interaction between the dots can be measured off-resonance only if the strong coupling condition is reached. Using the quantum regression theorem, a reasonable definition of the dynamical coupling regimes is introduced in terms of the complex Rabi frequency. Finally, the emission spectrum for relevant conditions is presented and compared with the above definition, demonstrating that the interaction between the excitons does not affect the strong coupling.
We study the dynamics of a quantum dot embedded in a three-dimensional microcavity in the strong coupling regime in which the quantum dot exciton has an energy close to the frequency of a confined cavity mode. Under the continuous pumping of the system, the confined electron and hole can recombine either by spontaneous emission through a leaky mode or by stimulated emission of a cavity mode that can escape from the cavity. The numerical integration of a master equation including all these effects gives the dynamics of the density matrix. By using the quantum regression theorem, we compute the first- and second-order coherence functions required to calculate the photon statistics and the spectrum of the emitted light. Our main result is the determination of a range of parameters in which a state of cavity modes with Poissonian or sub-Poissonian (nonclassical) statistics can be built up within the microcavity. Depending on the relative values of pumping and rate of stimulated emission, either one or two peaks close to the excitation energy of the dot and/or to the natural frequency of the cavity are observed in the emission spectrum. The physics behind these results is discussed.
We theoretically discuss spontaneous emission properties of a quantum dot embedded in an ultrahigh-QQQ microcavity, where a detuning between an excitation in the quantum dot and the cavity mode is taken into account. Both weak- and strong-coupling states are obtained under the ultrahigh-QQQ condition. In the high-QQQ weak-coupling case, the spontaneous emission spectrum shows a sharp dip, whose origin is a quantum interference. In the strong-coupling case, there is a region where both the Rabi splitting and the quantum interference contribute on an equal footing, referred to as a crossover region, where the spontaneous emission spectral shape is quite similar to that of the high-QQQ weak-coupling state. The quantum interference is robust against the detuning.
The time-dependent spectral properties and nonlinear dynamics of a spontaneous photon emitted by two level atom, trapped in damped nanocavity and coupled to a single resonance mode, have been investigated. The results have been obtained with the help of new nonperturbative approach by solving exactly the Schrödinger equation. The theory accounts exactly and simultaneously processes of emission, reabsorptions and leakage of photon. The solution was found with the Green functions formalism, supplemented with the novel algorithm in operating causal singular functions and fundamentals of the theory of quasi-stationary systems. The obtained distributions and emission dynamics are presented with plots as functions of photon frequency detuning and time for various value Γ/4g. For Γ/4g <1 the spectrum is a triplet inside the cavity and doublet outside it. In this case the total emission probability is described by decaying oscillations. For Γ/4g ≥ 1 and Γ/4g >> 1 the spectrum consists of a single central line decaying exponentially with profile depending on value Γ/4g.