Using modern micro and nano-fabrication techniques combined with superconducting materials we realize quantum electronic circuits in which we create, store, and manipulate individual microwave photons. The strong interaction of photons with superconducting quantum two-level systems allows us to probe fundamental quantum effects of microwave radiation and also to develop components for applications in quantum technology. Previously we have realized on-demand single photon sources which we have characterized using correlation function measurements [1] and full quantum state tomography [2]. For this purpose we have developed efficient methods to separate the quantum signals of interest from the noise added by the linear amplifiers used for quadrature amplitude detection [3]. We now regularly employ superconducting parametric amplifiers [4] to perform nearly quantum limited detection of propagating electromagnetic fields. These enable us to probe the entanglement which we generate on demand between stationary qubits and microwave photons freely propagating down a transmission line [5]. Using two independent microwave single photon sources, we have recently performed Hong-Ou-Mandel experiments at microwave frequencies [6] and have probed the coherence of two-mode multi-photon states at the out-put of a beam-splitter. The non-local nature of such states may prove to be useful for distributing entanglement in future small-scale quantum networks.
Using modern micro and nano-fabrication techniques combined with superconducting materials we realize quantum electronic circuits in which we create, store, and manipulate individual microwave photons. The strong interaction of photons with superconducting quantum two-level systems allows us to probe fundamental quantum effects of microwave radiation and also to develop components for applications in quantum technology. Previously we have realized on-demand single photon sources which we have characterized using correlation function measurements [1] and full quantum state tomography [2]. For this purpose we have developed efficient methods to separate the quantum signals of interest from the noise added by the linear amplifiers used for quadrature amplitude detection [3]. We now regularly employ superconducting parametric amplifiers [4] to perform nearly quantum limited detection of propagating electromagnetic fields. These enable us to probe the entanglement which we generate on demand between stationary qubits and microwave photons freely propagating down a transmission line [5]. Using two independent microwave single photon sources, we have recently performed Hong-Ou-Mandel experiments at microwave frequencies [6] and have probed the coherence of two-mode multi-photon states at the out-put of a beam-splitter. The non-local nature of such states may prove to be useful for distributing entanglement in future small-scale quantum networks.
Two-photon quantum interference at a beam splitter, commonly known as Hong–Ou–Mandel interference, is a fundamental demonstration of the quantum mechanical nature of electromagnetic fields and a key component of various quantum information processing protocols. The phenomenon was recently demonstrated with microwave-frequency photons by Lang et al (2013 Nature Phys. 9 345–8). This experiment employed circuit QED systems as sources of microwave photons, and was based on the measurement of second-order cross-correlation and auto-correlation functions of the microwave fields at the outputs of the beam splitter using linear detectors. Here we present the calculation of these correlation functions for the cases of inputs corresponding to: (i) trains of pulsed Gaussian or Lorentzian single microwave photons and (ii) resonant fluorescent microwave fields from continuously driven circuit QED systems. In both cases, the signature of two-photon quantum interference is a suppression of the second-order cross-correlation function for small delays. The experiment described in Lang et al (2013) was performed with trains of Lorentzian single photons, and very good agreement with experimental data is obtained. The results are relevant not only to interference experiments using circuit QED systems, but any such setup with highly controllable sources and time-resolved detection.
Two-photon quantum interference at a beam splitter, commonly known as Hong–Ou–Mandel interference, is a fundamental demonstration of the quantum mechanical nature of electromagnetic fields and a key component of various quantum information processing protocols. The phenomenon was recently demonstrated with microwave-frequency photons by Lang et al (2013 Nature Phys. 9 345–8). This experiment employed circuit QED systems as sources of microwave photons, and was based on the measurement of second-order cross-correlation and auto-correlation functions of the microwave fields at the outputs of the beam splitter using linear detectors. Here we present the calculation of these correlation functions for the cases of inputs corresponding to: (i) trains of pulsed Gaussian or Lorentzian single microwave photons and (ii) resonant fluorescent microwave fields from continuously driven circuit QED systems. In both cases, the signature of two-photon quantum interference is a suppression of the second-order cross-correlation function for small delays. The experiment described in Lang et al (2013) was performed with trains of Lorentzian single photons, and very good agreement with experimental data is obtained. The results are relevant not only to interference experiments using circuit QED systems, but any such setup with highly controllable sources and time-resolved detection.
The flexible engineering of superconducting circuits, together with the nonlinearity available from Josephson junctions, have made microwave quantum optics a blooming research field in the past decade. Key experiments originally performed in the optical domain have become very accessible on this microwave-frequency, such that strong atom-field interactions and optical parametric interactions in microwave. From the latter, one example is the implementation of spontaneous parametric downconversion (SPDC). This process is particularly interesting as it can act as a nonclassical radiation source which give a number of potential applications in quantum information processing. We will focus on studying SPDC in microwave throughout this thesis. \n \nIn the first half of this thesis, from designs to measurements, we will explore the well-known two-photon parametric processes, SPDC and coherent coupling, which are generated by quadratic Hamiltonians. Using three resonant modes of a SQUID-terminated parametric cavity, we proceeded to combine different two-photon processes in an effort to demonstrate a multipartite nonclassical radiation source. With detailed system gain and noise calibration of our cryogenic microwave network, we confirmed our implementation by experimentally verifying that the generated states contain genuine tripartite entanglement. This multimode entangled radiation source can be an important resource for future experiments on quantum networking. \n \nWhile two-photon parametric processes have found numerous important applications, they have also been the limit of experiments for over three decades, with higher-order parametric processes seemingly out of reach. In the second half of this thesis, we explore the potential of parametric resonators for achieving such higher-order processes. To do this, we first studied the necessary conditions for accessing cubic Hamiltonians through our SQUID-based interactions. We then fabricated a device dedicated to performing three-photon processes through these cubic Hamiltonians. For the first time, we observed a direct generation of photon triplets by a single SPDC process in microwave . The generation rate can exceed a photon flux density of 60 photon per second per Hertz at the device output, far surpassing any record to date for photon triplets. We studied various pump configurations corresponding to different three-photon SPDC processes starting from a cold vacuum state. Pumping at triple the frequency of a single mode, we observed a phase-space distribution with a non-Gaussian profile which shows strong skewness (third moment) in the quadrature amplitude distribution. We reconstruct the Wigner function of the propagating states from the directly measured moment matrix, demonstrating Wigner negativity. Pumping at the sum frequency of three modes, we observed non-zero coskewness between the quadrature amplitudes of the modes. By analysing the output signals and comparing their characteristics to the predicted theoretical signatures, we confirm our implementation of three-photon SPDC processes generated by specific cubic Hamiltonians. These types of non-Gaussian states have been suggested as a resource enabling universal quantum computation with continuous variables. Our results thus open up the realm of three-photon quantum optics, enabling a wealth of novel experimental and theoretical studies.
In this thesis, I demonstrate and evaluate an on-demand source of single propagating microwaves photons. Working in the context of a quantum network, nodes are connected via propagating, nonclassical states of the electromagnetic field. As such, preparing and detecting propagating quantum states is an essential task. I work with one particular node consisting of a microfabricated, effective two level system coupled to a microwave resonator and study its ability to produce propagating nonclassical states, such as single photon states. In principle, states generated by this node could be sent to other such nodes. However, I send them into a Josephson parametric amplifier (JPA) to characterize the source. In particular, I discuss how to design and couple the two components that form my source: a fixed frequency transmon qubit and a 3D superconducting waveguide cavity. I demonstrate the ability to control of the dynamics of this combined system and implement a single photon generation protocol, which utilizes a single microwave control field that is far detuned from the photon emission frequency. To characterize the generation, I perform tomography on the propagating photon state to determine its density matrix ρ. I perform repeated JPA-backed, linear measurements of the propagating state. Based on the histograms of my measurements, I infer a maximum single photon component ρ₁₁ = 0.36 ± 0.01. I characterize the imperfections of the photon generation and detection, including detection inefficiency and measurement backaction. I find that within uncertainty my measurements match my expectation.
Quantum optics in superconducting circuits, known as circuit QED, studies the interaction of photons at microwave frequencies with artificial atoms made of Josephson junctions. Although quite young, remarkable progress has been made in this field over the past decade, especially given the interest in building a quantum computer using superconducting circuits. In this thesis based on the appended papers, we look at generation, engineering and detection of microwave photons using superconducting circuits. We do this by taking advantage of the strong coupling, on-chip tunability and huge nonlinearity available in superconducting circuits. First, we present the strong photon-photon interaction measured experimentally, as shown in the giant cross-Kerr effect. In this work, conditional phase shift of about 20 degrees per photon was measured between two coherent fields at single photon level. Given this strong interaction, we propose and analyze a cascaded setup based on the cross-Kerr effect to detect itinerant microwave photons, a long outstanding problem with only recent experimental realizations. We show that a nondestructive detection of microwave photons is possible with few cascaded transmons. The on-chip tunability of Superconducting Quantum Interference Device (SQUID) is exploited to create a tunable superconducting resonator in the next presented experimental work. Finally, we show that by placing the atom at the end of a transmission line, microwave photons can be generated efficiently and on-demand. We also present a setup that can generate the photons in arbitrary wave packets.
Atoms and photons, two things so different but yet so alike. The former, the building block of matter, something we learn about in school and imagine it as some tiny marbles encircled by other tinier marbles. The latter, an electromagnetic wave, a light particle or an excitation of the electromagnetic field. Quantum mechanics tells us about the properties of these two entities. And even if it sounds, looks and writes counter-intuitive, it has proven right for over a century now. In this work, I elaborate on how we tested the laws of quantum mechanics and how we used them learn more about the tiny building blocks of nature and the fields they use to talk to each other. The atoms we use, are artificial. Superconducting qubits, small electrical circuits with quantized energy levels behave like electrons that transition between different orbitals in an atom. One of the qubits' advantages, is also a big disadvantage. We design the circuits' energy levels and fabricate them in a cleanroom. This allows for arbitrary spaced energy levels but in contrast to real atoms, prevents two superconducting qubits from being alike. Still, this qubit platform is one of the frontrunners for future quantum computing technology and testing fundamental physics due to their scalability. We interface superconducting qubits, which operate in the GHz regime, with microwave photons. We use 3D aluminum cavities as mediators between qubits and photons. The cavities allow for non-destructive readout of the qubit state, they shield the qubits from noise at the qubit frequency and they give us an easy way to frequency-tune these joint systems. We need to operate superconducting qubits and their cavities at millikelvin temperatures in dilution refrigerators. At higher temperatures, superconductivity suffers and even worse, the environment is filled with thermal noise photons. This poses a fundamental limitation on the scalability of superconducting qubit devices. Also connecting multiple devices in different fridges does not work over room temperature links because the microwave photons used for this purpose will be covered in noise and the quantum information they carry, will be unusable. Infrared photons do not suffer from this noise problem since there are close to zero thermal noise photons at their frequencies at room temperature. We cannot simply interface superconducting devices with optical photons due their frequency mismatch and the destructive effect of optical photons on superconductors. Therefore, we use microwave-to-optics transducers that allow to convert microwave photons into optical ones and vice-versa. The transducers that we use are macroscopic electro-optic transducers using the Pockels effect in a disk-shaped Lithium Niobate whispering gallery mode resonator. By using a strong optical pump, photons from the two frequency domains experience a beam-splitter interaction and get converted from one to the other. We measure the generated optical photons using elaborate optical setups, optical heterodyning and single photon detectors to gain knowledge about the qubit state or the converted microwave photons. Bridging the microwave and the optical world allows us to take advantage of both of their strengths but it also requires deep knowledge about both of their working principles. In this work, we describe two experiments that our group conducted to showcase the opportunities that arise from interfacing superconducting qubits with optical photons but also the pitfalls, one may encounter on the way. In the first experiment, we managed to all-optically read out a superconducting qubit. We show that the assignment fidelity, the probability that a measurement of the qubit state matches the prepared state, is close to equal for all-optical, microwave-to-optics and conventional microwave readout. We show T1 and T2 measurements for all three readout types and give an analysis of the noise caused by the optics. Finally, we show that the infrared light does not affect the qubit performance in a negative way but that the heating it causes does. This is an important insight that we used in the next experiment. The second experiment is the upconversion of itinerant single microwave photons to the optical domain. We show that we can generate single microwave photons from a qubit-cavity system. We upconvert these single photons, measure them with a single photon detector and reconstruct their shape. By conducting a single photon Rabi measurement, we show correlations between the microwave and the optical domain. And by thorough signal-to-noise measurements and noise analysis, we find that we can generate single infrared photons with high signal-to-noise ratio 5.1 and low transducer added noise (<0.012 quanta). We show that this measurement creates a path towards entanglement of a superconducting qubit and an optical photon and what parameters need to be improved to achieve it. Additionally, this experiment is a proof of principle for an on-demand infrared single photon source. More generally, it allows to link microwave quantum technology in general to the optical domain.