The flexible engineering of superconducting circuits, together with the nonlinearity available from Josephson junctions, have made microwave quantum optics a blooming research field in the past decade. Key experiments originally performed in the optical domain have become very accessible on this microwave-frequency, such that strong atom-field interactions and optical parametric interactions in microwave. From the latter, one example is the implementation of spontaneous parametric downconversion (SPDC). This process is particularly interesting as it can act as a nonclassical radiation source which give a number of potential applications in quantum information processing. We will focus on studying SPDC in microwave throughout this thesis. \n \nIn the first half of this thesis, from designs to measurements, we will explore the well-known two-photon parametric processes, SPDC and coherent coupling, which are generated by quadratic Hamiltonians. Using three resonant modes of a SQUID-terminated parametric cavity, we proceeded to combine different two-photon processes in an effort to demonstrate a multipartite nonclassical radiation source. With detailed system gain and noise calibration of our cryogenic microwave network, we confirmed our implementation by experimentally verifying that the generated states contain genuine tripartite entanglement. This multimode entangled radiation source can be an important resource for future experiments on quantum networking. \n \nWhile two-photon parametric processes have found numerous important applications, they have also been the limit of experiments for over three decades, with higher-order parametric processes seemingly out of reach. In the second half of this thesis, we explore the potential of parametric resonators for achieving such higher-order processes. To do this, we first studied the necessary conditions for accessing cubic Hamiltonians through our SQUID-based interactions. We then fabricated a device dedicated to performing three-photon processes through these cubic Hamiltonians. For the first time, we observed a direct generation of photon triplets by a single SPDC process in microwave . The generation rate can exceed a photon flux density of 60 photon per second per Hertz at the device output, far surpassing any record to date for photon triplets. We studied various pump configurations corresponding to different three-photon SPDC processes starting from a cold vacuum state. Pumping at triple the frequency of a single mode, we observed a phase-space distribution with a non-Gaussian profile which shows strong skewness (third moment) in the quadrature amplitude distribution. We reconstruct the Wigner function of the propagating states from the directly measured moment matrix, demonstrating Wigner negativity. Pumping at the sum frequency of three modes, we observed non-zero coskewness between the quadrature amplitudes of the modes. By analysing the output signals and comparing their characteristics to the predicted theoretical signatures, we confirm our implementation of three-photon SPDC processes generated by specific cubic Hamiltonians. These types of non-Gaussian states have been suggested as a resource enabling universal quantum computation with continuous variables. Our results thus open up the realm of three-photon quantum optics, enabling a wealth of novel experimental and theoretical studies.
The flexible engineering of superconducting circuits, together with the nonlinearity available from Josephson junctions, have made microwave quantum optics a blooming research field in the past decade. Key experiments originally performed in the optical domain have become very accessible on this microwave-frequency, such that strong atom-field interactions and optical parametric interactions in microwave. From the latter, one example is the implementation of spontaneous parametric downconversion (SPDC). This process is particularly interesting as it can act as a nonclassical radiation source which give a number of potential applications in quantum information processing. We will focus on studying SPDC in microwave throughout this thesis. \n \nIn the first half of this thesis, from designs to measurements, we will explore the well-known two-photon parametric processes, SPDC and coherent coupling, which are generated by quadratic Hamiltonians. Using three resonant modes of a SQUID-terminated parametric cavity, we proceeded to combine different two-photon processes in an effort to demonstrate a multipartite nonclassical radiation source. With detailed system gain and noise calibration of our cryogenic microwave network, we confirmed our implementation by experimentally verifying that the generated states contain genuine tripartite entanglement. This multimode entangled radiation source can be an important resource for future experiments on quantum networking. \n \nWhile two-photon parametric processes have found numerous important applications, they have also been the limit of experiments for over three decades, with higher-order parametric processes seemingly out of reach. In the second half of this thesis, we explore the potential of parametric resonators for achieving such higher-order processes. To do this, we first studied the necessary conditions for accessing cubic Hamiltonians through our SQUID-based interactions. We then fabricated a device dedicated to performing three-photon processes through these cubic Hamiltonians. For the first time, we observed a direct generation of photon triplets by a single SPDC process in microwave . The generation rate can exceed a photon flux density of 60 photon per second per Hertz at the device output, far surpassing any record to date for photon triplets. We studied various pump configurations corresponding to different three-photon SPDC processes starting from a cold vacuum state. Pumping at triple the frequency of a single mode, we observed a phase-space distribution with a non-Gaussian profile which shows strong skewness (third moment) in the quadrature amplitude distribution. We reconstruct the Wigner function of the propagating states from the directly measured moment matrix, demonstrating Wigner negativity. Pumping at the sum frequency of three modes, we observed non-zero coskewness between the quadrature amplitudes of the modes. By analysing the output signals and comparing their characteristics to the predicted theoretical signatures, we confirm our implementation of three-photon SPDC processes generated by specific cubic Hamiltonians. These types of non-Gaussian states have been suggested as a resource enabling universal quantum computation with continuous variables. Our results thus open up the realm of three-photon quantum optics, enabling a wealth of novel experimental and theoretical studies.
Multimode superconducting parametric cavity is a flexible platform that has been used to study a variety of topics in microwave quantum optics ranging from parametric amplification, entanglement generation to higher order spontaneous parametric downconversion (SPDC). \nLeveraging the extensive toolbox of interactions available in this system, we can look to explore exciting applications in quantum computation and simulation. \nIn this thesis, we study the use of the parametric cavity to realize continuous variable (CV) quantum computation. \nWe propose and examine in detail the scheme to compute with the microwave photons in the orthogonal frequency modes of the cavity via successive application of parametric pump pulses or cavity drives. \nThe family of all Gaussian transformations can be accomplished easily with interactions already demonstrated in this system. \nFrom recent results and proposals involving higher order SPDC, there are also clear pathways towards realizing the non-Gaussian resources necessary for universal computation. \nCommon measurements on the system are accomplished with standard measurement techniques on the output state of the cavity and additional useful measurements may be implemented using available parametric interactions or new device designs involving a qubit as a nonlinear probe. \nUsing the parametric cavity, we experimentally implemented a hybrid quantum-classical machine learning algorithm called the Quantum Kitchen Sinks (QKS) as the first step towards developing this platform for quantum computation. \nThe algorithm is studied over two sets of experiments starting from partial experimental implementation of the quantum variational circuits to fully experimental implementation using multiple simultaneous continuous wave (CW) pumps. \nIn both cases, we find that the quantum part of the algorithm implemented in the parametric cavity improved the classification accuracy on a difficult synthetic data set up to 90.1% and 99.5% respectively when compared to a classical linear machine learning algorithm.
The generation of entangled photons through spontaneous parametric down-conversion (SPDC) is a critical resource for many key experiments and technologies in the domain of quantum optics. Historically, SPDC was limited to the generation of photon pairs. However, the use of the strong nonlinearities in circuit quantum electrodynamics has recently enabled the observation of three-photon SPDC (3P-SPDC). Despite great interest in the entanglement structure of the resultant states, entanglement between photon triplets produced by a 3P-SPDC source has still not been confirmed. Here, we report on the observation of genuine tripartite non-Gaussian entanglement in the steady-state output field of a 3P-SPDC source consisting of a superconducting parametric cavity coupled to a transmission line. We study this non-Gaussian tripartite entanglement using an entanglement witness built from three-mode correlation functions, observing a maximum violation of the bound by 15 standard deviations of the statistical noise. Furthermore, we find strong agreement between the observed and the analytically predicted scaling of the entanglement witness. We then explore the impact of the temporal function used to define the photon mode on the observed value of the entanglement witness.
Quantum optics in superconducting circuits, known as circuit QED, studies the interaction of photons at microwave frequencies with artificial atoms made of Josephson junctions. Although quite young, remarkable progress has been made in this field over the past decade, especially given the interest in building a quantum computer using superconducting circuits. In this thesis based on the appended papers, we look at generation, engineering and detection of microwave photons using superconducting circuits. We do this by taking advantage of the strong coupling, on-chip tunability and huge nonlinearity available in superconducting circuits. First, we present the strong photon-photon interaction measured experimentally, as shown in the giant cross-Kerr effect. In this work, conditional phase shift of about 20 degrees per photon was measured between two coherent fields at single photon level. Given this strong interaction, we propose and analyze a cascaded setup based on the cross-Kerr effect to detect itinerant microwave photons, a long outstanding problem with only recent experimental realizations. We show that a nondestructive detection of microwave photons is possible with few cascaded transmons. The on-chip tunability of Superconducting Quantum Interference Device (SQUID) is exploited to create a tunable superconducting resonator in the next presented experimental work. Finally, we show that by placing the atom at the end of a transmission line, microwave photons can be generated efficiently and on-demand. We also present a setup that can generate the photons in arbitrary wave packets.
One of the primary requirements for superconducting quantum information processors is high-fidelity, quantum non-demolition qubit readout. In superconducting circuits, we perform measurements with quantum-limited microwave amplifiers. These amplifiers are based on microwave cavities and powered by Josephson-junction based nonlinearities, which we drive to parametrically modulate the circuit and generate gain. However, cavity-based amplifiers generally suffer from a fixed gain-bandwidth product, a limited dynamic range, and the absence of directionality, and so they must be operated with external lossy microwave commercial components such as circulators. Many of these limitations can be circumvented by combining multiple parametric processes in a few-mode device, in particular by combining parametric drives which produce gain and those which produce gainless photon conversion. By combining balanced gain and conversion processes between a pair of modes, we have demonstrated transmission-only, phase-sensitive, gain-bandwidth-free amplification. We have also used measurements of transmon qubits with this mode of amplification to demonstrate its practical utility. More, by combining multiple instances of imbalanced gain and conversion processes among three modes, we have realized devices with non-reciprocal, transmission-only amplification, matched ports, and a large, gain-independent bandwidth. One of the biggest challenges in tuning multiple parametric processes is both inherent and dynamically-generated higher order nonlinearities in the device, which shift mode frequencies and parametric coupling strengths with pump power, preventing accurate balancing of the parametric processes. These can be controlled through engineering the Hamiltonian of the nonlinear element, in this thesis either a linearly-shunted Josephson Ring Modulator or SNAIL (Superconducting Nonlinear Asymmetric Inductive eLements), which for certain applied flux values can minimize or even change the sign of higher-order even nonlinearities. Additionally, we have explored a range of circuit parameters, allowing us to also control the relative size of odd-order nonlinearities. We have developed a series of prototypes which implement these concepts, and have achieved both high-dynamic range singly pumped amplifiers, and a promising platform for multi-parametric devices. We conclude by presenting recent progress towards implementing multiple parametric schemes that generates a practical directional amplifier, and discuss the remaining obstacles to a truly ideal parametric amplifiers.
Over the past decade, much effort has been made in identifying and characterizing systems that can form a building block of quantum networks, among which semiconductor quantum dots (QD) and spontaneous parametric down-conversion (SPDC) source are two of the most promising candidates. The work presented in this thesis will be centered on investigating and engineering the mentioned systems for generating customizable single photons. A type-II SPDC source can generate a highly flexible pair of entangled photons that can be used to interface disparate quantum systems. In this thesis, we have successfully implemented a cavity-SPDC source that emits polarization correlated photons at 942 nm with a lifetime of 950-1050ps that mode matches closely with InAs/GaAs QD photons. The source emits 80 photon pairs per second per mW pump power within the 150MHz bandwidth. Though the detection of idler photons, the source is capable of emitting heralded photons with g2≤0.5 for up to 40 mW pump power. For a low pump power of ~5 mW, the heralded g2 is 0.06, indicating that the system is an excellent heralded single photon source. By directly exciting a single QD with cavity-SPDC photons, we have demonstrated a heralded-absorption of SPDC photons by QD, resulting in the coupling of the two systems. Due to the large pump bandwidth, the emitted source is highly multimode in nature, requiring us to post-filter the downconverted field, resulting in a lower photon pair emission rate. We propose placing an intra-cavity etalon to suppress the multi-mode emissions and increase the photon count rate. Understanding and experimentally implementing two-photon interference (HOM) measurements will be crucial for building a scalable quantum network. A detailed theoretical description of HOM measurements is given and is experimentally demonstrated using photons emitted by QD. Through HOM measurements we demonstrated that the QD sample in the study is capable of emitting indistinguishable photons, with the visibility exceeding 95%. As an alternative approach to modifying the spectral mode of single photons, we performed phase modulation of photons emitted by a QD to generate additional sidebands that are separated by several GHz. By performing HOM measurements, we have shown that the central component and the sidebands are in the superposition states and the spectrally modified photons have a well-preserved indistinguishability. Such spectrally engineered photons can be used for phase-encoded cryptography applications. These experimental results should lay the foundations towards building a scalable hybrid quantum network.
Artificially engineered atoms, built using superconducting electrical circuits, have had a broad impact on the field of quantum information and quantum computing. Based on the Josephson effect, superconducting qubits have provided a robust platform for engineering light-matter interactions at the single-photon level. The ability to precisely control and manipulate single photons using superconducting qubits and cavities, a field now popularly known as circuit quantum electrodynamics (circuit QED), has enabled new and novel regimes in quantum physics, which previously remained inaccessible. For instance, the coupling between individual photons and artificial atoms have been shown to reach the ultrastrong and deep-strong regimes, a feat which is difficult to achieve with natural atoms. The superconducting circuit platform is now a promising contender for building large-scale quantum processors, attracting large investments from academic, industry and government players. \n \nThis thesis uses superconducting circuits to engineer photon interactions in two separate studies. The first is aimed at studying the physics of ``giant" artificial-atoms. The second study explores the route towards building a quantum heat engine using two parametrically-coupled, superconducting microwave cavities. We review the theoretical ideas and concepts which motivate our work, along with discussions of the design methodology, simulations, fabrication, measurement setup and the experimental findings. \n \nIn the first study, we explore a giant artificial atom, formed from a transmon qubit, which is coupled to propagating microwaves at multiple points along an open transmission line. The multipoint coupling nature of the transmon allows its radiated field to interfere with itself leading to some striking ``giant" atom effects. For instance, we observe strong frequency dependent couplings of the transmon's transition levels to its electromagnetic environment, a feature which is not observed with ordinary artificial atoms. We measure large on/off ratios, as high as 380, for the coupling rate of the ket0−ket1 transition. Furthermore, we show that we can enhance or suppress the coupling rate of the ket1−ket2 transition relative to the ket0−ket1 transition, by more than a factor of 200. The relative modulation of the coupling rates was exploited to engineer a metastable state in the giant transmon and demonstrate electromagnetically-induced transparency (EIT), a typical signature of a lambda system. Our results show that we can transform the ladder structure of an ordinary transmon into a more interesting lambda system using a giant transmon, thereby paving the way for exploring new possibilities to study three-level physics in a waveguide-QED setting. \n \nExtending giant atom physics to multiple giant atoms, we then explore a device with two giant artificial atoms connected in a braided configuration to a transmission line. The braided topology of the qubits, offers an interesting regime where the qubits can interact with each other in a decoherence-free environment, where the interaction is mediated by virtual photons in the transmission line. We probe the resonant behavior of the qubits at two different frequency bias points, where we observe qualitatively different scattering behavior. Furthermore, when probing for the Autler-Townes Splitting (ATS), multiple resonances are observed for both resonant and off-resonant cases instead of the familiar doublet in the ATS spectroscopy. This comes as a surprise as the frequency-level spacings in both qubits are nominally identical. We believe these features could be an indication of a novel resonant interaction between the qubits facilitated by the braided topology. An effort to understand this theoretically is underway. \n \nFor our second study, we explore a system with two parametrically-coupled superconducting resonators, which implements an optomechanical-like interaction in an all-electrical network. The nonlinear nature of this interaction is mediated by a superconducting quantum interference device (SQUID), where the current in one resonator couples to the photon number in the other resonator. We propose to use this system to build a ``photonic piston" engine in the quantum regime. We motivate the feasibility of the proposal by reviewing key theoretical results which demonstrate an Otto-cycle by appropriately driving the system with noise. Our experimental findings demonstrate the crucial nonlinear coupling that is required for the engine to work. We also show that we can increase the coupling strength between the resonators depending on the chosen flux operating point.